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In this work, we present a stochastic variational calculation (SVM) of energies and wave functions of few particle systems coupled to quantum fields in cavity QED. The light-matter coupled system is described by the Pauli-Fierz Hamiltonian.…

Mesoscale and Nanoscale Physics · Physics 2022-01-05 Alexander Ahrens , Chenhang Huang , Matt Beutel , Cody Covington , Kalman Varga

We study a system consisting of a superconducting flux qubit strongly coupled to a microwave cavity. The fundamental cavity mode is externally driven and the response is investigated in the weak nonlinear regime. We find that near the…

Quantum Physics · Physics 2016-09-14 Eyal Buks , Chunqing Deng , Jean-Luc F. X. Orgazzi , Martin Otto , Adrian Lupascu

A quantum electrodynamical time-dependent density functional theory framework is applied to describe strongly coupled light--matter interactions in cavity environments. The formalism utilizes a tensor product approach, coupling real-space…

Chemical Physics · Physics 2025-11-27 Yetmgeta Aklilu , Matthew Shepherd , Cody L. Covington , Kalman Varga

This chapter provides a basic introduction to excited-state extensions of density functional theory (DFT), including time-dependent (TD-)DFT in both its linear-response and its explicitly time-dependent formulations. As applied to the…

Chemical Physics · Physics 2023-05-02 John M. Herbert

In this work, we illustrate the recently introduced concept of the cavity Born-Oppenheimer approximation for correlated electron-nuclear-photon problems in detail. We demonstrate how an expansion in terms of conditional electronic and…

Quantum Physics · Physics 2017-04-12 Johannes Flick , Heiko Appel , Michael Ruggenthaler , Angel Rubio

Strong quantum correlations in matter are responsible for some of the most extraordinary properties of material, from magnetism to high-temperature superconductivity, but their integration in quantum devices requires a strong, coherent…

Quantum Gases · Physics 2020-07-15 Kevin Roux , Hideki Konishi , Victor Helson , Jean-Philippe Brantut

We study a two-level system (atom, superconducting qubit or quantum dot) strongly coupled to the single photonic mode of a cavity, in the presence of incoherent pumping and including detuning and dephasing. This system displays a striking…

Quantum Physics · Physics 2011-10-12 E. del Valle , F. P. Laussy

The interaction between the electromagnetic field inside a cavity and natural or artificial atoms has played a crucial role in developing our understanding of light-matter interaction, and is central to various quantum technologies.…

Recent experimental advances in strongly coupled light-matter systems has sparked the development of general ab-initio methods capable of describing interacting light-matter systems from first principles. One of these methods,…

Chemical Physics · Physics 2022-10-12 Johannes Flick

Quantum-electrodynamical density-functional theory (QEDFT) provides a promising avenue for exploring complex light-matter interactions in optical cavities for real materials. Similar to conventional density-functional theory, the Kohn-Sham…

Computational Physics · Physics 2024-02-16 I-Te Lu , Michael Ruggenthaler , Nicolas Tancogne-Dejean , Simone Latini , Markus Penz , Angel Rubio

Time-Dependent Density Functional Theory (TDDFT) has recently been extended to describe many-body open quantum systems (OQS) evolving under non-unitary dynamics according to a quantum master equation. In the master equation approach,…

Chemical Physics · Physics 2015-05-18 David G. Tempel , Mark A. Watson , Roberto Olivares-Amaya , Alán Aspuru-Guzik

The description of excited state dynamics in multichromophoric systems constitutes both a theoretical and experimental challenge in modern physical chemistry. An experimental protocol which can systematically characterize both coherent and…

Quantum Physics · Physics 2011-10-31 Joel Yuen-Zhou , Jacob J. Krich , Masoud Mohseni , Alán Aspuru-Guzik

Cavity quantum electrodynamics (QED) studies the interaction between a quantum emitter and a single radiation-field mode. When an atom is in strong coupling with a cavity mode1,2, it is possible to realize key quantum information processing…

Quantum Physics · Physics 2009-11-13 K. Hennessy , A. Badolato , M. Winger , D. Gerace , M. Atature , S. Gulde , S. Falt , E. L. Hu , A. Imamoglu

Achieving strong coupling between light and matter is usually a challenge in Cavity Quantum Electrodynamics (cQED), especially in solid state systems. For this reason is useful taking advantage of alternative approaches to reach this…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 J. E. Ramírez-Muñoz , J. P. Restrepo Cuartas , H. Vinck-Posada

The hybridization between light and matter forms the basis to achieve cavity control over quantum materials. In this work we investigate a cavity coupled to an XXZ quantum chain of interacting spinless fermions by numerically exact…

Strongly Correlated Electrons · Physics 2023-07-17 Giacomo Passetti , Christian J. Eckhardt , Michael A. Sentef , Dante M. Kennes

Intense laser-matter interactions are at the center of interest in research and technology since the development of high power lasers. They have been widely used for fundamental studies in atomic, molecular, and optical physics, and they…

Time-dependent response theories are foundational to the development of algorithms that determine quantum properties of electronic excited states of molecules and periodic systems. They are employed in wave-function, density-functional, and…

Chemical Physics · Physics 2022-11-23 Martín A. Mosquera

Strong-field quantum-state control is investigated, taking advantage of the full---amplitude and phase---characterization of the interaction between matter and intense ultrashort pulses via transient-absorption spectroscopy. A sequence of…

Atomic Physics · Physics 2017-04-26 Stefano M. Cavaletto , Zoltán Harman , Thomas Pfeifer , Christoph H. Keitel

A reduced-density-matrix (RDM)-based approach to {\em ab initio} cavity quantum electrodynamics (QED) is developed. The expectation value of the Pauli-Fierz Hamiltonian is expressed in terms of one- and two-body electronic and photonic…

Chemical Physics · Physics 2022-11-23 Joel D. Mallory , A. Eugene DePrince

A quantitative and predictive theory of quantum light-matter interactions in ultra thin materials involves several fundamental challenges. Any realistic model must simultaneously account for the ultra-confined plasmonic modes and their…