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This article summarizes recent work on the many-body (beyond density functional theory) electronic structure of layered rare-earth nickelates, both in the context of the materials themselves and in comparison to the high-temperature…

Strongly Correlated Electrons · Physics 2022-02-03 Hanghui Chen , Alexander Hampel , Jonathan Karp , Frank Lechermann , Andrew Millis

The discovery of superconductivity in Sr-doped NdNiO$_{2}$ is a crucial breakthrough in the long pursuit for nickel oxide materials with electronic and magnetic properties similar to those of the cuprates. NdNiO$_2$ is the infinite-layer…

Superconductivity · Physics 2020-08-05 Emilian M. Nica , Jyoti Krishna , Rong Yu , Qimiao Si , Antia S. Botana , Onur Erten

The square-planar layered nickelates R$_{n+1}$Ni$_n$O$_{2n+2}$ (R= Nd, $n=4-7$) have been recently shown to be superconducting without the need for chemical doping or pressure. Here, we examine the electronic structure of the analog…

Strongly Correlated Electrons · Physics 2026-03-31 Alexander K. Gavrilov , Lidia C. Santander , Antia S. Botana

In strongly correlated materials, lattice, charge, spin and orbital degrees of freedom interact with each other, leading to emergent physical properties such as superconductivity, colossal magnetic resistance and metal-insulator transition.…

Superconductivity · Physics 2021-08-04 Junjie Zhang , Xutang Tao

The discovery of superconductivity in Ruddlesden-Popper nickelates has established a new frontier in the study of high-temperature superconductors. However, the underlying pairing mechanism and its relationship to the material's electronic…

The discovery of superconductivity in hole-doped infinite layer nickelates, RNiO2 (R = Nd, Pr, La) has garnered sustained interest in the field. A definitive picture of low-energy many-body states has not yet emerged. We provide new…

Strongly Correlated Electrons · Physics 2023-03-28 Gheorghe Lucian Pascut , Lucian Cosovanu , Kristjan Haule , Khandker F. Quader

Motivated by the report of superconductivity in bilayer La$_3$Ni$_2$O$_7$ at high pressure, we examine the interacting electrons in this system. First-principles many-body theory is utilized to study the normal-state electronic properties.…

Strongly Correlated Electrons · Physics 2023-12-04 Frank Lechermann , Jannik Gondolf , Steffen Bötzel , Ilya M. Eremin

The discovery of infinite-layer nickelate superconductors has spurred enormous interest. While the Ni$^{1+}$ cations possess nominally the same 3$d^9$ configuration as Cu$^{2+}$ in cuprates, the electronic structure variances remain…

After the significant discovery of the hole-doped nickelate compound Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, an analysis of the electronic structure, orbital components, Fermi surfaces and band topology could be helpful to understand the mechanism of…

Materials Science · Physics 2021-03-18 Jiacheng Gao , Zhijun Wang , Chen Fang , Hongming Weng

Rare-earth nickelates RNiO$_2$ adopting an infinite-layer phase show superconductivity once La, Pr or Nd are substituted by a divalent cation. Either in the pristine or doped form, these materials are reported to adopt a high symmetry,…

The discovery of superconductivity in infinite-layer nickelates has added a new family of materials to the fascinating growing class of unconventional superconductors. By incorporating the strongly correlated multi-orbital nature of the…

Superconductivity · Physics 2022-08-15 Andreas Kreisel , Brian M. Andersen , Astrid T. Rømer , Ilya M. Eremin , Frank Lechermann

Effective models are constructed for a newly discovered superconductor (Nd,Sr)NiO2, which has been considered as a possible nickelate analogue of the cuprates owing to the d9 electron configuration. Estimation of the effective interaction,…

Superconductivity · Physics 2020-08-14 Hirofumi Sakakibara , Hidetomo Usui , Katsuhiro Suzuki , Takao Kotani , Hideo Aoki , Kazuhiko Kuroki

Motivated by recent photoemission measurements on the La$_{0.8}$Sr$_{0.2}$NiO$_2$, we carry out a systematic study of the infinite-layer nickelate using both dynamical mean-field theory and density matrix embedding theory. The renormalized…

Strongly Correlated Electrons · Physics 2024-11-07 Ziyan Chen , Yuxin Wang , Kun Jiang , Jiangping Hu

We demonstrate in this paper that the recently discovered infinite-layer (IL) nickelates have much in common with a class of materials known as electrides. Oxide based electrides are compounds in which topotactic removal of loosely bound…

Superconductivity · Physics 2023-11-30 Kateryna Foyevtsova , Ilya Elfimov , George A. Sawatzky

Recently discovered superconducting infinite-layer nickelates $R$NiO$_2$ ($R$=Nd, La, Pr) attract increasing attention due to their similarities to cuprates. Both $R$NiO$_2$ and YBCO cuprates exhibit the non-Fermi-liquid transport behavior,…

Strongly Correlated Electrons · Physics 2025-12-10 Shinichi Hiragami , Seiichiro Onari

The series of nickel-oxide compounds LaNiO$_3$ (formal Ni$(d^7)$), La$_2$NiO$_4$ (formal Ni$(d^8)$) and LaNiO$_2$ (formal Ni$(d^9)$) is investigated by first-principles many-body, using a combination of density functional theory,…

Strongly Correlated Electrons · Physics 2022-04-07 Frank Lechermann

Motivated by the recently reported high-temperature superconductivity in the bilayer La$_3$Ni$_2$O$_7$ (LNO) under pressure, here we comprehensively study this system using {\it ab initio} techniques. The Ni $3d$ orbitals have a large…

Superconductivity · Physics 2023-11-29 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

The newly synthesized strontium doped RNiO$_2$ (R=Nd, La) superconductors have stimulated extensive interests in understanding their pairing mechanism and pairing nature. Here we study the pairing mechanism in this family from a two-orbital…

Strongly Correlated Electrons · Physics 2022-03-14 Chen Lu , Lun-Hui Hu , Yu Wang , Fan Yang , Congjun Wu

Recently, superconductivity was discovered in the infinite layer of hole-doped nickelates NdNiO$_{2}$. Contrary to this, superconductivity in LaNiO$_{2}$ is still under debate. This indicates the crucial role played by the $f$ electrons on…

Strongly Correlated Electrons · Physics 2023-02-09 Andrzej Ptok , Surajit Basak , Przemysław Piekarz , Andrzej M. Oleś

The discovery of unconventional superconductivity in hole doped NdNiO2, similar to CaCuO2, has received enormous attention. However, different from CaCuO2, RNiO2 (R = Nd, La) has itinerant electrons in the rare-earth spacer layer. Previous…

Strongly Correlated Electrons · Physics 2020-05-18 Yuhao Gu , Sichen Zhu , Xiaoxuan Wang , Jiangping Hu , Hanghui Chen