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The new family of superconducting nickelates centered around La$_{3}$Ni$_{2}$O$_{7}$ possesses attractive features, such as the high transition temperature and the presence of an antiferromagnetic ground state at ambient pressure,…

High-transition-temperature ($T_{C}$) superconductivity is recently discovered in Ruddlesden-Popper (RP) nickelate films with extraordinarily strong oxidation. While investigating phase diagrams is essential for uncovering the…

A new frontier in condensed matter physics is to stack atomically thin layered-materials with different properties and create intriguing phenomena which do not exist in any of the constituent layers. Transition metal dichalcogenide…

$R_2BaNiO_5$ ($R=$ rare earth) quasi-1-D antiferromagnets are structurally equivalent to the well-studied 1-D S=1 Haldane-gap compound Y_2BaNiO_5. Unlike the Y-nickelate though, these materials undergo 3-D magnetic ordering at finite…

Condensed Matter · Physics 2016-03-23 A. Zheludev

The status of nickelate superconductors in relation to cuprate high temperature superconductors is one of the concepts being discussed in high temperature superconductivity in correlated transition metal oxides. New additions to the class…

Strongly Correlated Electrons · Physics 2022-04-14 Hyo-Sun Jin , W. E. Pickett , K. -W. Lee

An effective two-dimensional two-band model for infinite-layer nickelates consists of bands obtained from $d_{x^2-y^2}$ and $s$--like orbitals. We investigate whether it could be mapped onto a single-band Hubbard model and the filling of…

Strongly Correlated Electrons · Physics 2023-04-12 Tharathep Plienbumrung , Maria Daghofer , Michael T. Schmid , Andrzej M. Oleś

The electronic structure of the new superconducting material LaNiPO experimentally probed by soft X-ray spectroscopy and theoretically calculated by the combination of local density approximation with Dynamical Mean-Field Theory (LDA+DMFT)…

Recently superconductivity at 9 - 15 K was discovered in an infinite-layer nickelate (Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ films), which has received enormous attention. Since the $Ni^{1+}$ ionic state in NdNiO$_2$ may have the $3d^9$ outer-shell…

Superconductivity · Physics 2020-04-06 Qing Li , Chengping He , Jin Si , Xiyu Zhu , Yue Zhang , Hai-Hu Wen

Starting from an effective two-dimensional two-band model for infinite layered nickelates, consisting of bands obtained from $d$ and $s$--like orbitals, we investigate to which extend it can be mapped onto a single-band Hubbard model. We…

Strongly Correlated Electrons · Physics 2023-02-13 Tharathep Plienbumrung , Maria Daghofer , Michael Schmid , Andrzej M. Oleś

In the present study, we explore superconductivity in NdNiO$_2$ and LaNiO$_2$ employing a first-principles derived low-energy model Hamiltonian, consisting of two orbitals: Ni $x^{2}$-$y^{2}$, and an {\it axial} orbital. The {\it axial}…

Atomic structure and electronic band structure are fundamental properties for understanding the mechanism of superconductivity. Motivated by the discovery of pressure-induced high-temperature superconductivity at 80 K in the bilayer…

The consequences of varying the rare-earth element in the superconducting infinite-layer nickelates have been much debated. Here we show striking differences in the magnitude and anisotropy of the superconducting upper critical field across…

Motivated by the recently reported signatures of superconductivity in trilayer La$_4$Ni$_3$O$_{10}$ under pressure, we comprehensively study this system using {\it ab initio} and random-phase approximation techniques. Without electronic…

Superconductivity · Physics 2024-09-24 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

We suggest that a family of Ni-based compounds, which contain [Ni$_2$M$_2$O]$^{2-}$(M=chalcogen) layers with an antiperovskite structure constructed by mixed-anion Ni complexes, NiM$_4$O$_2$, can be potential high temperature…

Superconductivity · Physics 2018-08-06 Congcong Le , Jinfeng Zeng , Guang-Han Cao , Jiangping Hu

We theoretically study quasi-two-dimensional nickel compounds, where the nickel ions assume Ni$^{2+}$ $d^8$ valence state and feature a low-spin $S=0$ ground state quasidegenerate with $S=1$ ionic excitations. Such a level structure is…

Strongly Correlated Electrons · Physics 2025-09-16 Jiří Chaloupka , Giniyat Khaliullin

Motivated by the high temperature superconductivity observed in the bilayer nickelate La$_3$Ni$_2$O$_7$ and the spectroscopic evidences of strong electron correlations in this compound, we address the role of its multiorbital electron…

Superconductivity · Physics 2024-12-31 Zhiguang Liao , Yiming Wang , Lei Chen , Guijing Duan , Rong Yu , Qimiao Si

The 122$^{*}$ series of iron-chalcogenide superconductors, for example K$_x$Fe$_{2-y}$Se$_{2}$, only possesses electron Fermi pockets. Their distinctive electronic structure challenges the picture built upon iron pnictide superconductors,…

Motivated by the recent activities on the Ni-based diamond lattice antiferromagnet NiRh$_2$O$_4$, we theoretically explore on a general ground the unique spin and orbital physics for the Ni$^{2+}$ ions with a $3d^8$ electron configuration…

Strongly Correlated Electrons · Physics 2019-07-10 Fei-Ye Li , Gang Chen

The discovery of superconductivity with a critical temperature of about 80~K in La$_{3}$Ni$_{2}$O$_{7}$ single crystals under pressure has received enormous attention. La$_{3}$Ni$_{2}$O$_{7}$ is not superconducting under ambient pressure…

Superconductivity · Physics 2024-09-12 Zhe Liu , Mengwu Huo , Jie Li , Qing Li , Yuecong Liu , Yaomin Dai , Xiaoxiang Zhou , Jiahao Hao , Yi Lu , Meng Wang , Hai-Hu Wen

Very recently, a new superconductor with Tc = 80 K was reported in nickelate (La3Ni2O7) at around 15 - 40 GPa conditions (Nature, 621, 493, 2023) [1], which is the second type of unconventional superconductor, beside the cuprates, with Tc…

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