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A combined experimental and theoretical study of the layered antiferromagnetic compound DyRh$_2$Si$_2$ in the ThCr$_2$Si$_2$-type structure is presented. The heat capacity shows two transitions upon cooling, the first one at the N{\'e}el…

Strongly Correlated Electrons · Physics 2023-07-05 Kristin Kliemt , Michelle Ocker , Sarah Krebber , Susanne Schulz , Denis V. Vyalikh , Cornelius Krellner , Dmitry Yu. Usachov

A new mononuclear Dysprosium based Coordination Polymer {Dy-CP} was investigated magnetically using dc and ac magnetic susceptibility. The dc magnetic susceptibility does not exhibit any long-range ordering down to 1.8 K and the negative…

Materials Science · Physics 2020-08-26 Suraj Singh , Sheetal , Bandhana Devi , R. R. Koner , Aditi Haldar , C. S. Yadav

We present a first principles LSDA+U study of the magnetic coupling constants in the spinel magnets CoCr_2O_4 and MnCr_2O_4. Our calculated coupling constants highlight the possible importance of AA interactions in spinel systems with…

Materials Science · Physics 2007-08-09 Claude Ederer , Matej Komelj

Comprehensive muon spin rotation/relaxation (muSR) and neutron powder diffraction (NPD) studies supported via bulk measurements have been performed on the ordered double perovskite Sr2YbRuO6 to investigate the nature of the magnetic ground…

The magnetic properties and the spin dynamics of two molecular magnets have been investigated by magnetization and d.c. susceptibility measurements, Electron Paramagnetic Resonance (EPR) and proton Nuclear Magnetic Resonance (NMR) over a…

Materials Science · Physics 2017-12-06 P. Khuntia , M. Mariani , M. C. Mozzati , L. Sorace , F. Orsini , A. Lascialfari , F. Borsa , M. Andruh , C. Maxim

An extensive {\it ab initio} study of the physical properties of both linear and zigzag atomic chains of all 4$d$ and 5$d$ transition metals (TM) within the GGA by using the accurate PAW method, has been carried out. All the TM linear…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 J. C. Tung , G. Y. Guo

Co$_{1-x}$Mn$_x$Cr$_2$O$_4$ crystallizes as a normal spinel in the cubic $Fd \overline{3}m$ space group, and the end members have been reported to display a region of collinear ferrimagnetism as well as a low-temperature spin-spiral state…

Magnetic properties of a sigma-phase Fe60V40 intermetallic compound were studied by means of ac and dc magnetic susceptibility and magnetocaloric effect measurements. The compound is a soft magnet yet it was found to behave like a…

Strongly Correlated Electrons · Physics 2017-02-28 M. Balanda , S. M. Dubiel , R. Pelka

This study presents the first-ever investigation of spin-phonon coupling mechanisms in fullerene-based single-molecule magnets (SMMs) using ab initio CASSCF combined with DFT calculations. While lanthanide-based SMMs, particularly those…

Single crystals of Fe$_{1/4}$TaS$_{2}$ have been studied by using magneto-optical (MO) imaging and radio-frequency (rf) magnetic susceptibility, $\chi$. Real time MO images reveal unusual, slow dynamics of dendritic domain formation, the…

Strongly Correlated Electrons · Physics 2009-10-28 M. D. Vannette , S. Yeninas , E. Morosan , R. J. Cava , R. Prozorov

The hyperfine coupling constants of neutron deficient $^{37}$Ca were deduced from the atomic hyperfine spectrum of the $4s~^2S_{1/2}$ $\leftrightarrow$ $4p~^2P_{3/2}$ transition in Ca II, measured using the collinear laser spectroscopy…

Dynamic magnetic properties of $\mathrm{Y_{0.7}Ca_{0.3}MnO_{3}}$ are reported. The system appears to attain local ferromagnetic order at $T_{\mathrm{SRF}} \approx 70$ K. Below this temperature the low field magnetization becomes history…

Materials Science · Physics 2009-10-31 R. Mathieu , P. Nordblad , D. N. H. Nam , N. X. Phuc , N. V. Khiem

In order to probe the magnetic ground state, we have carried out temperature dependent magnetic Compton scattering experiments on an oriented single crystal of magnetite (Fe$_3$O$_4$), together with the corresponding first-principles band…

Strongly Correlated Electrons · Physics 2007-10-11 Yinwan Li , P. A. Montano , B. Barbiellini , P. E. Mijnarends , S. Kaprzyk , A. Bansil

Motivated by the observation of biskyrmions in centrosymmetric magnetic films (Yu et al. Nature Communications 2014, Wang et al. Advanced Materials 2016), we investigate analytically and numerically the stability of biskyrmions in films of…

Mesoscale and Nanoscale Physics · Physics 2019-07-31 Daniel Capic , Dmitry A. Garanin , Eugene M. Chudnovsky

We present a theoretical approach to calculate the molecular magnetic anisotropy parameters, $D_M$ and $E_M$ for single molecule magnets in any eigenstate of the exchange Hamiltonian, treating the anisotropy Hamiltonian as a perturbation.…

Strongly Correlated Electrons · Physics 2009-11-13 Rajamani Raghunathan , S. Ramasesha , Diptiman Sen

The intermediate valence of Ce in CeCo$_5$ challenges standard density functional theory (DFT) and static DFT+$U$ approaches, which fail to capture its magnetic properties. By combining DFT+$U$ with exact diagonalization of the Anderson…

Strongly Correlated Electrons · Physics 2026-04-21 Alexander B. Shick , Evgenia A. Tereshina-Chitrova

The magnetic ground state is crucial for the applications of the two-dimension magnets as it decides fundamental magnetic properties of the material, such as magnetic order, magnetic transition temperature, and low-energy excitation of the…

Materials Science · Physics 2024-12-06 Yue-Fei Hou , Shujing Li , Xinlong Yang , Wei Jiang , Qiuhao Wang , Fawei Zheng , Zhen-Guo Fu , Ping Zhang

A systematic study of magnetocrystalline anisotropy is performed for R(La/Ce/Nd)2Fe14B tetragonal compound with the site substitution mechanism. Theoretical calculation suggests the 50% doping with Ce at 4f-site can lead to competitive…

Materials Science · Physics 2018-06-07 Rajiv K. Chouhan , Arjun K. Pathak , D. Paudyal , V. K. Pecharsky

The debate whether uranium 5f electrons are closer to being localized or itinerant in the ferromagnetic compound UGa2 is not yet fully settled. The experimentally determined magnetic moments are large, approximately 3 Bohr magnetons,…

Strongly Correlated Electrons · Physics 2021-07-14 Banhi Chatterjee , Jindrich Kolorenc

The understanding of coercivity mechanism in high performance Nd-Fe-B permanent magnets relies on the analysis of the magnetic properties of all phases present in the magnets. By adding Cu in such compounds, a new Nd6Fe13Cu grain boundary…