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Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

We present a theoretical study of the local optical conductivity, plasmon spectra, and thermoelectric properties of twisted bilayer graphene (TBG) at different filling factors and twist angles $\theta$. Our calculations are based on the…

Mesoscale and Nanoscale Physics · Physics 2020-09-04 Pietro Novelli , Iacopo Torre , Frank H. L. Koppens , Fabio Taddei , Marco Polini

We report on the dynamics of coherent phonons in semimetal 1T'-MoTe2 using femtosecond pump-probe spectroscopy. On an ultrafast sub-picosecond time scale at room temperature, a low frequency and long-lifetime shear phonon mode was observed…

Materials Science · Physics 2020-03-09 T. Fukuda , K. Makino , Y. Saito , P. Fons , A. V. Kolobov , K. Ueno , M. Hase

Motivated by recent experimental progress we revisit the theory of pump-probe time- and angle-resolved photoemission spectroscopy (trARPES), which is one of the most powerful techniques to trace transient pump-driven modifications of the…

Mesoscale and Nanoscale Physics · Physics 2022-01-14 Michael Schüler , Michael A. Sentef

The transient-absorption spectrum of a $V$-type three-level system is investigated, when this is periodically excited by a train of equally spaced, $\delta$-like pump pulses as, e.g., from an optical-frequency-comb laser. We show that, even…

Atomic Physics · Physics 2019-01-30 Juliane Haug , Stefano M. Cavaletto

Van der Waals heterostructures obtained by artificially stacking two-dimensional crystals represent the frontier of material engineering, demonstrating properties superior to those of the starting materials. Fine control of the interlayer…

We investigate experimentally the ultrafast changes in the spectral response of the Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl ($\kappa$-Cl) upon photodoping with intense excitation at 1.6 eV and probing with continuum pulses…

Strongly Correlated Electrons · Physics 2023-10-31 Konstantin Warawa , Yassine Agarmani , Harald Schubert , Martin Dressel , Michael Lang , Hartmut G. Roskos , Mark D. Thomson

Time-resolved optical spectroscopy (TR-OS) has emerged as a fundamental spectroscopic tool for probing complex materials, to both investigate ground-state-related properties and trigger phase transitions among different states with peculiar…

Time-resolved multi-terahertz (THz) spectroscopy is used to observe pump fluence-dependent dynamics in the optical conductivity of photoexcited tin selenide (SnSe) over an ultrabroadband spectral range of 0.5 - 11 THz at fluences from 0.1 -…

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

Materials Science · Physics 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

We report the observation of the resonant excitation of edge photocurrents in bilayer graphene subjected to terahertz radiation and a magnetic field. The resonantly excited edge photocurrent is observed for both inter-band (at low carrier…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 S. Candussio , M. V. Durnev , S. Slizovskiy , T. Jötten , J. Keil , V. V. Bel'kov , J. Yin , Y. Yang , S. -K. Son , A. Mishchenko , V. Fal'ko , S. D. Ganichev

We have made a detailed temperature-dependent photoemission study of VO_2/TiO_2(001) thin films, which show a metal-insulator transition at \sim 300 K. Clean surfaces were obtained by annealing the films in an oxygen atmosphere. Spectral…

Strongly Correlated Electrons · Physics 2009-11-10 K. Okazaki , H. Wadati , A. Fujimori , M. Onoda , Y. Muraoka , Z. Hiroi

Femtosecond core-level transient absorption spectroscopy is utilized to investigate photoinduced dynamics of the charge density wave in 1T-TiSe2 at the Ti M2,3 edge (30-50 eV). Photoexcited carriers and phonons are found to primarily induce…

Materials Science · Physics 2022-11-08 Tobias Heinrich , Hung-Tzu Chang , Sergey Zayko , Kai Rossnagel , Murat Sivis , Claus Ropers

Bismuth, with its rhombohedral crystalline structure and two Raman active phonon modes corresponding to the internal displacement ($A_{1g}$) and shear ($E_{g}$) ionic motions, offers an ideal target for the investigation of the…

Materials Science · Physics 2024-07-31 Kunie Ishioka , Oleg V. Misochko

1$T$-TaSe$_{2}$ is host to coexisting strongly-correlated phases including charge density waves (CDWs) and an unusual Mott transition at low temperature. Here, we investigate coherent phonon oscillations in 1$T$-TaSe$_{2}$ using a…

Strongly Correlated Electrons · Physics 2023-10-26 C. J. Sayers , H. Hedayat , A. Ceraso , F. Museur , M. Cattelan , L. S. Hart , L. S. Farrar , S. Dal Conte , G. Cerullo , C. Dallera , E. Da Como , E. Carpene

Degenerate pump-probe reflectivity experiments have been performed on a single crystal of bismuth telluride (Bi$_2$Te$_3$) as a function of sample temperature (3K to 296K) and pump intensity using $\sim$ 50 femtosecond laser pulses with…

Materials Science · Physics 2015-05-20 N. Kamaraju , Sunil Kumar , A. K. Sood

Carrier dynamics in monolayer MoS2 have been investigated using broadband femtosecond transient absorption spectroscopy (FTAS). A tunable pump pulse was used while a broadband probe pulse revealed ground and excited state carrier dynamics.…

Mesoscale and Nanoscale Physics · Physics 2016-08-24 Shrouq H. Aleithan , Maksim Y. Livshits , Sudiksha Khadka , Jeffrey J. Rack , Martin Kordesch , Eric Stinaff

Photosensitive proteins embedded in the cell membrane (about 5 nm thickness) act as photoactivated proton pumps, ion gates, enzymes, or more generally, as initiators of stimuli for the cell activity. They are composed of a protein backbone…

In this study, we experimentally investigate the photonic dispersion in one-dimensional moir\'e structures formed by stacking two photonic crystal slabs with slightly different periods, separated by a carefully controlled subwavelength…

The strong interlayer coupling in black phosphorus (BP), arising from wavefunction overlap between layers, is critical for understanding its electronic and optical properties. Here, we utilize terahertz (THz) spectroscopy to study phonon…

Strongly Correlated Electrons · Physics 2025-09-08 Haiyun Huang , Cheng Chen , Yuxin Zhai , Xiu Zhang , Junzhi Zhu , Junyong Wang , Kai Zhang , Qihua Xiong , Haiyun Liu