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Porous materials are widely used for applications in gas storage and separation. The diffusive properties of a variety of gases in porous media can be modeled using molecular dynamics simulations that can be computationally demanding…

Chemical Physics · Physics 2023-09-19 Gastón González , Rubén A. Fritz , Yamil J. Colón , Felipe Herrera

The problem of diffusion in a porous medium with a spatially varying porosity is considered. The particular microstructure analyzed comprises a collection of impenetrable spheres, though the methods developed are general. Two different…

Fluid Dynamics · Physics 2017-10-12 Maria Bruna , S. Jonathan Chapman

An atomistic study of the order-effect occurring in Li$_{x}$CoO$_{2}$ at $x=0.5$ is presented and an explanation for the computationally and experimentally observed dip in the Li diffusivity is proposed. Configurations where a single…

Materials Science · Physics 2016-05-04 Teutë Bunjaku , Andreas Pedersen , Mathieu Luisier

Aims. We probe the effect of turbulent diffusion on the chemistry at the interface between a cold neutral medium (CNM) cloudlet and the warm neutral medium (WNM). Methods. We perform moving grid, multifluid, 1D, hydrodynamical simulations…

Astrophysics · Physics 2009-11-13 P. Lesaffre , M. Gerin , P. Hennebelle

The time dependency of the diffusion coefficient of particles in porous media is an efficient probe of their geometry. The analysis of this quantity, measured e.g. by nuclear magnetic resonance (PGSE-NMR), can provide rich information…

Soft Condensed Matter · Physics 2013-02-13 Maximilien Levesque , Olivier Bénichou , Benjamin Rotenberg

The aqueous proton displays an anomalously large diffusion coefficient that is up to 7 times that of similarly sized cations. There is general consensus that the proton achieves its high diffusion through the Grotthuss mechanism, whereby…

Chemical Physics · Physics 2018-12-18 Sean A. Fischer , Brett I. Dunlap , Daniel Gunlycke

We present a combined experimental and theoretical study of the self-diffusion of ammonia on exfoliated graphite. Using neutron time-of-flight spectroscopy we are able to resolve the ultrafast diffusion process of adsorbed ammonia, NH$_3$,…

The properties of amorphous solid water at and near the calorimetric glass transition temperature, $T_{g}$, of 136 K have been debated for years. One hypothesis is that water turns into a "true" liquid at $T_{g}$ (i.e., it becomes ergodic)…

Soft Condensed Matter · Physics 2025-03-03 Greg A. Kimmel , Megan K. Dunlap , Kirill Gurdumov , R. Scott Smith , Loni Kringle , Bruce D. Kay

While the energy-dependent neutron diffusion equation is widely employed in nuclear engineering, its status as an approximation to the transport equation is not yet completely understood, and several different approximations are in use to…

Computational Physics · Physics 2025-12-22 Gabriele Burgio , Christian Reiter , Stefano Lorenzi

The diffusion coefficient of a circular shaped inclusion in a liquid membrane is investigated by taking into account the interaction between membranes and bulk solvents of arbitrary thickness. As illustrative examples, the diffusion…

Soft Condensed Matter · Physics 2015-05-28 Kazuhiko Seki , Sanoop Ramachandran , Shigeyuki Komura

Although real surfaces exhibit intricate topologies at the nanoscale, rough surface consideration is often overlooked in nanoscale heat transfer studies. Superimposed sinusoidal functions effectively model the complexity of these surfaces.…

To simulate the transient enhanced diffusion near the surface or interface, a set of equations describing the impurity diffusion and quasichemical reactions of dopant atoms and point defects in ion-implanted layers is proposed and analyzed.…

Materials Science · Physics 2007-05-23 O. I. Velichko , Yu. P. Shaman , A. K. Fedotov , A. V. Masanik

Long-timescale simulations of the diffusion of a H$_2$O admolecule on the (0001) basal plane of ice Ih were carried out over a temperature range of 100 to 200 K using the adaptive kinetic Monte Carlo method and TIP4P/2005f interaction…

Computational Physics · Physics 2015-08-04 Andreas Pedersen , Leendertjan Karssemeijer , Herma M. Cuppen , Hannes Jónsson

In this work, a new algorithm is proposed to compute single particle (infinite dilution) thermodiffusion using Non-Equilibrium Molecular Dynamics simulations through the estimation of the thermophoretic force that applies on a solute…

Statistical Mechanics · Physics 2009-11-13 Guillaume Galliéro , S. Volz

Carbon dioxide (CO$_2$) sequestration in saline aquifers has been introduced as one of the most practical, long-term, and safe solutions to tackle a growing threat originating from the emission of CO$_2$. Successfully executing and planning…

Mesoscale and Nanoscale Physics · Physics 2021-09-07 Sina Omrani , Mehdi Ghasemi , Saeed Mahmoodpour , Ali Shafiei , Behzad Rostami

We investigate water and deuterated water chemistry in turbulent protoplanetary disks. Chemical rate equations are solved with the diffusion term, mimicking turbulent mixing in vertical direction. Water near the midplane is transported to…

Astrophysics of Galaxies · Physics 2015-06-17 Kenji Furuya , Yuri Aikawa , Hideko Nomura , Franck Hersant , Valentine Wakelam

Molecular dynamics simulations are used to study the mechanism and kinetics of hydrated electron diffusion. The electron center of mass is found to exhibit Brownian-type behavior with a diffusion coefficient considerably greater than that…

Chemical Physics · Physics 2012-11-06 Kafui A. Tay , François-Xavier Coudert , Anne Boutin

Translational diffusion coefficients are routinely estimated from molecular dynamics simulations. Linear fits to mean squared displacement (MSD) curves have become the de facto standard, from simple liquids to complex biomacromolecules.…

Computational Physics · Physics 2020-11-20 Jakob Tómas Bullerjahn , Sören von Bülow , Gerhard Hummer

Context: Diffusion of species on the dust surface is a key process for determining the chemical composition of interstellar ices. On the dust surface, adsorbed species diffuse from one potential well to another and react with other adsorbed…

Astrophysics of Galaxies · Physics 2018-12-12 Wasim Iqbal , Valentine Wakelam , Pierre Gratier

Using a continuum bead-spring Monte Carlo model, we study the anomalous diffusion dynamics of a self-avoiding tethered membrane by means of extensive computer simulations. We focus on the subdiffusive stochastic motion of the membrane's…

Soft Condensed Matter · Physics 2008-05-14 Hristina Popova , Andrey Milchev