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Motivated by the recently reported signatures of superconductivity in trilayer La$_4$Ni$_3$O$_{10}$ under pressure, we comprehensively study this system using {\it ab initio} and random-phase approximation techniques. Without electronic…

Superconductivity · Physics 2024-09-24 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

Using DFT+DMFT we study the normal-state electronic structure and magnetic correlations of the recently discovered alternating single-layer bilayer Raddlesden-Popper nickelate La$_5$Ni$_3$O$_{11}$ (1212-LNO). Our results exhibit qualitative…

Strongly Correlated Electrons · Physics 2026-04-30 I. V. Leonov

Superconductivity is one of the most intriguing properties of matter described by an attractive interaction that bounds electrons into Cooper pairs. To date, the highest critical temperature at ambient conditions is achieved in copper…

Motivated by the report of superconductivity in bilayer La$_3$Ni$_2$O$_7$ at high pressure, we examine the interacting electrons in this system. First-principles many-body theory is utilized to study the normal-state electronic properties.…

Strongly Correlated Electrons · Physics 2023-12-04 Frank Lechermann , Jannik Gondolf , Steffen Bötzel , Ilya M. Eremin

Motivated by the recently reported high-temperature superconductivity in the bilayer La$_3$Ni$_2$O$_7$ (LNO) under pressure, here we comprehensively study this system using {\it ab initio} techniques. The Ni $3d$ orbitals have a large…

Superconductivity · Physics 2023-11-29 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

The discovery of nickelate superconductivity provided the first example of a non-copper-based material with superconductivity strongly analogous to the cuprates, but recent findings raise questions and inconsistencies around the electron…

Superconductivity · Physics 2024-11-05 Y. N. Huang , D. J. Singh

We conduct first-principles simulations of La$_3$Ni$_2$O$_7$, a nickelate in which recent experiments have shown signs of high-temperature superconductivity. Within the hydrostatic pressure range where superconductivity is observed, we find…

Superconductivity · Physics 2026-02-25 Daan Verraes , Tom Braeckevelt , Nick Bultinck , Veronique Van Speybroeck

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in…

We present a comparative density-functional theory plus dynamical mean-field theory (DFT+DMFT) study of the two known superconducting members of the rare-earth (R) layered nickelate family: hole-doped RNiO$_{2}$ ($n=\infty$) and…

Strongly Correlated Electrons · Physics 2022-03-01 Harrison LaBollita , Antia S. Botana

Superconductivity in nickelates apparently takes place in two different Ni oxidation regimes, namely either for infinite-layer-type compounds close to Ni$^{+}$, or for Ruddlesden-Popper materials close to Ni$^{2+}$. The reduced…

Strongly Correlated Electrons · Physics 2025-12-12 Frank Lechermann , Steffen Bötzel , Ilya M. Eremin

Recent experiments have shown that the reduced multilayer rare-earth (RE) nickel oxides of form RE$_{p+1}$Ni$_p$O$_{2p+2}$ may belong to the novel family of superconducting lanthanide nickelates. Here, the correlated electronic structure of…

Strongly Correlated Electrons · Physics 2022-04-07 Frank Lechermann

Using the DFT+dynamical mean-field theory approach we study the effects of electronic correlations and doping on the normal state electronic structure of the double-layer nickelate superconductor La$_3$Ni$_2$O$_7$ under pressure. In…

Strongly Correlated Electrons · Physics 2026-04-27 I. V. Leonov

Motivated by the recent discovery of superconductivity in the Sr-doped layered nickelate NdNiO$_2$, we perform a systematic computational materials design of layered nickelates that are dynamically stable and whose electronic structure…

Superconductivity · Physics 2020-02-12 Motoaki Hirayama , Terumasa Tadano , Yusuke Nomura , Ryotaro Arita

Motivated by the high temperature superconductivity observed in the bilayer nickelate La$_3$Ni$_2$O$_7$ and the spectroscopic evidences of strong electron correlations in this compound, we address the role of its multiorbital electron…

Superconductivity · Physics 2024-12-31 Zhiguang Liao , Yiming Wang , Lei Chen , Guijing Duan , Rong Yu , Qimiao Si

Systematically controlling the superconducting transition temperature ($T_\text{c}$) in the bilayer Ruddlesden-Popper nickelate La$_3$Ni$_2$O$_7$ remains a significant challenge. Here, we address this by synthesizing high-quality…

In this paper we investigate the electronic and superconducting properties in nickelate compounds of NiO2 through Perturbative Density Functional Theory (P-DFT) and multi-band BCS theory. We consider three different cases of study (i) the…

Superconductivity · Physics 2021-12-16 Julian Faundez , C. A. Aguirre , S. G. Magalhães , J. Barba-Ortega

The recent discovery of ambient-pressure superconductivity in thin-film bilayer nickelates opens new possibilities for investigating electronic structures in this new class of high-transition temperature $T_C$ superconductors. Here, we…

We investigate the electronic structure of nickelate superconductor NdNiO2 upon hole doping, by means of density-functional theory and dynamical mean-field theory. We demonstrate the strong intrinsic hybridization between strongly…

Strongly Correlated Electrons · Physics 2021-01-13 Zhao Liu , Chenchao Xu , Chao Cao , W. Zhu , Z. F. Wang , Jinlong Yang

Superconductivity has been demonstrated in the family of multi-layered nickelates La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$. Key questions remain open regarding the low-energy electronic states that support superconductivity in these…

The predominant Ni-multiorbital nature of infinite-layer neodynium nickelate at stoichiometry and with doping is revealed. We investigate the correlated electronic structure of NdNiO$_2$ at lower temperatures and show that first-principles…

Strongly Correlated Electrons · Physics 2020-10-06 Frank Lechermann