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In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar…

We have investigated the effect of imperfect circular polarization on the angle-resolved photoemission spectroscopy signal, using graphene as a prototypical system that can be understood within tight-binding formalism. We found that perfect…

Materials Science · Physics 2015-04-28 Hwihyeon Hwang , Choongyu Hwang

We describe a new experimental setup for the detection of magnetic circular dichroism with fast electrons (EMCD). As compared to earlier findings the signal is an order of magnitude higher, while the probed area could be significantly…

The ability to differentiate chiral molecules of different handedness is of great importance for chemical and life sciences. Since most of the relevant chiral molecules have their chiral transitions in the UV region, detecting their…

Circular dichroism (CD), i.e. the differential response of a system to left and right circularly polarized light, is one of the only techniques capable of providing morphological information of certain samples. In biology, for instance, CD…

Elliptical dichroism is known in atomic photoionization as the difference in the photoelectron angular distributions produced in nonlinear ionization of atoms by left- and right-handed elliptically polarized light. We theoretically…

Atomic Physics · Physics 2018-08-07 J. Hofbrucker , A. V. Volotka , S. Fritzsche

DNA and proteins are chiral: their three-dimensional structure cannot be superimposed with its mirror image. Circular dichroism spectroscopy is widely used to characterize chiral compounds, but data interpretation is difficult in the case…

Biomolecules · Quantitative Biology 2020-09-09 Steven Daly , Frederic Rosu , Valerie Gabelica

Photoelectron diffraction (PED) is a powerful and essential experimental technique for resolving the structure of surfaces with sub-angstrom resolution. In the high energy regime, researchers in angle-resolved photoemission spectroscopy…

We demonstrate that an effect phenomenologically analogous to circular dichroism can arise even for dielectric and isotropic chiral spherical particles. By analyzing the polarimetry of light scattered from a chiral, lossless microsphere…

Altermagnets are a new class of magnetic materials that are promising for spintronics technology. Here it is shown that in altermagnets, the circular dichroism (CD) in resonant photoelectron diffraction (RPED) contains a time-reversal odd…

Materials Science · Physics 2025-09-26 Peter Krüger

We calculate the circular dichroism (CD) for absorption of the twisted photons, or optical vortices, by atoms, caused by atomic excitation into discrete energy levels. The effects of photon spin on the rates and cross sections of atomic…

Quantum Physics · Physics 2017-10-02 Andrei Afanasev , Carl E. Carlson , Maria Solyanik

3D photoelectron angular distributions (PADs) are measured from an atomic target ionized by ultrafast, elliptical fields of opposite handedness. Comparing these PADs to one another and to numeric simulations, a difficult to avoid systematic…

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

We review the recent experimental and theoretical progress in $K$-shell detachment studies of atomic anions. On the experimental side, this field has largely benefitted from technical advances at 3rd generation synchrotron radiation…

Atomic Physics · Physics 2020-08-28 S. Schippers , A. Perry-Sassmannshausen , T. Buhr , M. Martins , S. Fritzsche , A Müller

Chiral light-matter interactions have been investigated for two centuries, leading to the discovery of many chiroptical processes used for discrimination of enantiomers. Whereas most chiroptical effects result from a response of bound…

Molecular chirality is a key design property for many technologies including bioresponsive imaging, circularly polarized light detection and emission, molecular motors and switches. Imaging and manipulating the primary steps of transient…

Shadow X-ray Magnetic Circular Dichroism Photo-Emission Electron Microscopy (XMCD-PEEM) is a recent technique, in which the photon intensity in the shadow of an object lying on a surface, may be used to gather information about the…

Circular Dichroism (CD) can distinguish the handedness of chiral molecules. However, it is typically very weak due to vanishing absorption at low molecular concentrations. Here, we suggest Thermal Circular Dichroism (TCD) for chiral…

Optics · Physics 2024-07-19 Ershad Mohammadi , Giulia Tagliabue

We investigate few-photon ionization of lithium atoms prepared in the polarized 2$p$($m_\ell=\!+1$) state when subjected to femtosecond light pulses with left- or right-handed circular polarization at wavelengths between 665 nm and 920 nm.…

Circular dichroism covering the telecommunication band is experimentally demonstrated in a semiconductor-based three-dimensional chiral photonic crystal (PhC). We design a rotationally-stacked woodpile PhC structure where neighboring layers…

Optics · Physics 2015-06-22 S. Takahashi , T. Tajiri , Y. Ota , J. Tatebayashi , S. Iwamoto , Y. Arakawa