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Maximum Elliptical Dichroism in Atomic Two-Photon Ionization

Atomic Physics 2018-08-07 v1

Abstract

Elliptical dichroism is known in atomic photoionization as the difference in the photoelectron angular distributions produced in nonlinear ionization of atoms by left- and right-handed elliptically polarized light. We theoretically demonstrate that the maximum dichroism |{\Delta}_{ED}|=1 always appears in two-photon ionization of any atom if the photon energy is tuned in so that the electron emission is dominantly determined by two intermediate resonances. We propose the two-photon ionization of atomic helium in order to demonstrate this remarkable phenomenon. The maximum elliptical dichroism could be used as a sensitive tool for analyzing the polarization state of photon beams produced by free-electron lasers.

Keywords

Cite

@article{arxiv.1808.01860,
  title  = {Maximum Elliptical Dichroism in Atomic Two-Photon Ionization},
  author = {J. Hofbrucker and A. V. Volotka and S. Fritzsche},
  journal= {arXiv preprint arXiv:1808.01860},
  year   = {2018}
}
R2 v1 2026-06-23T03:25:24.529Z