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We propose a new self-consistent field (SCF) algorithm based on an iterative, partially stochastic \textit{``Divide \& Conquer''}-type approach. This new SCF algorithm is a simple variant of the usual SCF procedure and can be easily…

Chemical Physics · Physics 2021-08-04 Pierre-François Loos , Jean-Louis Rivail , Xavier Assfeld

We describe a version of an algorithm for evolving self-gravitating collections of particles that should be nearly ideal for parallel architectures. Our method is derived from the ``self-consistent field'' (SCF) approach suggested…

Astrophysics · Physics 2016-08-30 Lars Hernquist , Steinn Sigurdsson , Greg L. Bryan

In this paper, we present a local convergence analysis of the self-consistent field (SCF) iteration using the density matrix as the state of a fixed-point iteration. Sufficient and almost necessary conditions for local convergence are…

Numerical Analysis · Mathematics 2018-11-26 Parikshit Upadhyaya , Elias Jarlebring , Emanuel H. Rubensson

Self-consistent field theory (SCFT) is one of the most widely-used framework in studying the equilibrium phase behaviors of inhomogenous polymers. For liquid crystalline polymeric systems, the main numerical challenges of solving SCFT…

Numerical Analysis · Mathematics 2024-09-16 Zhijuan He , Kai Jiang , Liwei Tan , Xin Wang

We propose a novel adaptive damping algorithm for the self-consistent field (SCF) iterations of Kohn-Sham density-functional theory, using a backtracking line search to automatically adjust the damping in each SCF step. This line search is…

Materials Science · Physics 2022-03-14 Michael F. Herbst , Antoine Levitt

We present a comprehensive convergence analysis for Self-Consistent Field (SCF) iteration to solve a class of nonlinear eigenvalue problems with eigenvector-dependency (NEPv). Using a tangent-angle matrix as an intermediate measure for…

Numerical Analysis · Mathematics 2020-09-22 Zhaojun Bai , Ren-Cang Li , Ding Lu

The inherently high computational cost of iterative self-consistent-field (SCF) methods proves to be a critical issue delaying visual and haptic feedback in real-time quantum chemistry. In this work, we introduce two schemes for SCF…

Chemical Physics · Physics 2016-03-10 Adrian H. Mühlbach , Alain C. Vaucher , Markus Reiher

The convergence property of a stochastic algorithm for the self-consistent field (SCF) calculations of electron structures is studied. The algorithm is formulated by rewriting the electron charges as a trace/diagonal of a matrix function,…

Numerical Analysis · Mathematics 2023-04-20 Taehee Ko , Xiantao Li

Spectral clustering is one of the most popular methods for community detection in graphs. A key step in spectral clustering algorithms is the eigen decomposition of the $n{\times}n$ graph Laplacian matrix to extract its $k$ leading…

Machine Learning · Statistics 2018-09-10 Muni Sreenivas Pydi , Ambedkar Dukkipati

We formulate and implement the Variational Quantum Eigensolver Self Consistent Field (VQE-SCF) algorithm in combination with polarizable embedding (PE), thereby extending PE to the regime of quantum computing. We test the resulting…

We propose an efficient algorithm for solving orthogonal canonical correlation analysis (OCCA) in the form of trace-fractional structure and orthogonal linear projections. Even though orthogonality has been widely used and proved to be a…

Machine Learning · Computer Science 2019-09-26 Leihong Zhang , Li Wang , Zhaojun Bai , Ren-cang Li

It is well known that the self-consistent field (SCF) iteration for solving the Kohn-Sham (KS) equation often fails to converge, yet there is no clear explanation. In this paper, we investigate the SCF iteration from the perspective of…

Computational Physics · Physics 2013-12-02 Xin Liu , Xiao Wang , Zaiwen Wen , Yaxiang Yuan

We introduce a self-consistent mean-field quantum optimization algorithm that approximates the ground state of classical Ising Hamiltonians. The algorithm decomposes the problem into independent subproblems and treats the interactions…

Quantum Physics · Physics 2026-03-11 Maxime Dupont , Bhuvanesh Sundar , Meenambika Gowrishankar

The Hartree-Fock equation is a fundamental equation in many-electron problems. It is of practical importance in quantum chemistry to find solutions to the Hartree-Fock equation. The self-consistent field (SCF) method is a standard numerical…

Analysis of PDEs · Mathematics 2023-11-17 Sohei Ashida

Semi-supervised learning is highly useful in common scenarios where labeled data is scarce but unlabeled data is abundant. The graph (or nonlocal) Laplacian is a fundamental smoothing operator for solving various learning tasks. For…

Computer Vision and Pattern Recognition · Computer Science 2023-04-20 Or Streicher , Guy Gilboa

The common spatial pattern analysis (CSP) is a widely used signal processing technique in brain-computer interface (BCI) systems to increase the signal-to-noise ratio in electroencephalogram (EEG) recordings. Despite its popularity, the…

Numerical Analysis · Mathematics 2023-11-23 Dong Min Roh , Zhaojun Bai

We present a simple spectral approach to the well-studied constrained clustering problem. It captures constrained clustering as a generalized eigenvalue problem with graph Laplacians. The algorithm works in nearly-linear time and provides…

Social and Information Networks · Computer Science 2016-01-20 Mihai Cucuringu , Ioannis Koutis , Sanjay Chawla , Gary Miller , Richard Peng

Semi-supervised Laplacian regularization, a standard graph-based approach for learning from both labelled and unlabelled data, was recently demonstrated to have an insignificant high dimensional learning efficiency with respect to…

Machine Learning · Computer Science 2020-06-16 Xiaoyi Mai , Romain Couillet

We present a self consistent field approach (SCF) within the Adaptive Derivative-Assembled Problem-Tailored Ansatz Variational Quantum Eigensolver (ADAPT-VQE) framework for efficient quantum simulations of chemical systems on near-term…

Consistency is a key property of all statistical procedures analyzing randomly sampled data. Surprisingly, despite decades of work, little is known about consistency of most clustering algorithms. In this paper we investigate consistency of…

Statistics Theory · Mathematics 2008-12-18 Ulrike von Luxburg , Mikhail Belkin , Olivier Bousquet
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