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We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Femtosecond high-order harmonic transient absorption spectroscopy is used to observe electromagnetically induced transparency-like behavior as well as induced absorption in the extreme ultraviolet by laser dressing of the He 2s2p (1Po) and…

Atomic Physics · Physics 2009-11-13 Zhi-Heng Loh , Chris H. Greene , Stephen R. Leone

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

The study of entangled states has greatly improved the basic understanding about two-photon interferometry. Two-photon interference is not the interference of two photons but the result of superposition among indistinguishable two-photon…

Quantum Physics · Physics 2009-11-10 Giuliano Scarcelli , Alejandra Valencia , Yanhua Shih

We present a 1 GHz-clocked, maximally entangled and on-demand photon pair source based on droplet etched GaAs quantum dots using two-photon excitation. By employing these GaP microlensenhanced devices in conjunction with their substantial…

Quantum Physics · Physics 2021-06-29 Caspar Hopfmann , Weijie Nie , Nand Lal Sharma , Carmen Weigelt , Fei Ding , Oliver G. Schmidt

We introduce a generalized theoretical approach to study action signals induced by the absorption of two-photons from two phase modulated laser beams and subject it to experimental testing for two types of photoactive samples, solution of…

We study in this paper the efficiency of different two-photon states of light to induce the simultaneous excitation of two atoms of different kinds when the sum of the energies of the two photons matches the sum of the energies of the two…

Quantum Physics · Physics 2013-03-21 Zhan Zheng , Pablo L. Saldanha , Jose R. Rios Leite , Claude Fabre

We show that many-body correlations among excitons originating from the Pauli exclusion principle in a quantum well embedded inside a microcavity provide a possibility to produce pairs of entangled photons by ultrashort laser pulses with a…

Mesoscale and Nanoscale Physics · Physics 2015-06-02 Mikhail Erementchouk , Michael N. Leuenberger

Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…

We propose the generation of attosecond entangled bi-photons in the extreme-ultraviolet regime by two-photon decay of a metastable atomic state as a source similar to spontaneous parametric down-conversion photons. The 1s2s $^1S_0$…

Quantum Physics · Physics 2025-11-25 Yimeng Wang , Siddhant Pandey , Chris H. Greene , Niranjan Shivaram

We analytically derive transfer probabilities and efficiencies for an artificial light-harvesting photosynthetic system, which consists of a ring coupled to a central acceptor. For an incident photon pair, we find near-perfect single…

Chemical Physics · Physics 2025-04-22 Stephon Alexander , Roger Andrews , Oliver Fox , Sarben Sarkar

A pulsed source of energy-time entangled photon pairs pumped by a standard laser diode is proposed and demonstrated. The basic states can be distinguished by their time of arrival. This greatly simplifies the realization of 2-photon quantum…

Quantum Physics · Physics 2016-09-08 J. Brendel , N. Gisin , W. Tittel , H. Zbinden

Unwanted multiphoton emission commonly reduces the degree of entanglement of photons generated by non-classical light sources and, in turn, hampers their exploitation in quantum information science and technology. Quantum emitters have the…

Photon blockade (PB) is a quantum effect in strongly nonlinear systems where a single photon prevents the system from being excited to a higher level, generating anti-bunched light fields. It enables the generation of single-photon sources…

Quantum Physics · Physics 2026-01-05 Weiyi An , Jie Zhu

Quantum entanglement among multiple spatially separated particles is of fundamental interest, and can serve as central resources for studies in quantum nonlocality, quantum-to-classical transition, quantum error correction, and quantum…

Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…

Quantum Physics · Physics 2020-11-03 Haowei Shi , Zheshen Zhang , Stefano Pirandola , Quntao Zhuang

Twin entangled beams produced by single-pass parametric down-conversion (PDC) offer the opportunity to detect weak amount of absorption with an improved sensitivity with respect to standard techniques which make use of classical light…

Quantum Physics · Physics 2009-11-13 E. Brambilla , L. Caspani , O. Jedrkiewicz , L. A. Lugiato , A. Gatti

The simplest approach to deal with light excitations in direct-gap semiconductors is to model them as a two-band system: one conduction and one valence band. For such models, particularly simple analytical expressions are known to exist for…

Materials Science · Physics 2022-10-12 W. -R. Hannes , M. F. Ciappina

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

We present a novel quantum phenomenon named electromagnetically induced entanglement in the conventional Lambda-type three-level atomic system driven by a strong pump field and a relatively weak probe field. Nearly perfect entanglement…

Quantum Physics · Physics 2015-05-19 Xihua Yang , Min Xiao