Related papers: Hot-Band Absorption Can Mimic Entangled Two-Photon…
Resonant intermediate states have been proposed to increase the efficiency of entangled two-photon absorption (ETPA). Although resonance-enhanced ETPA (r-ETPA) has been demonstrated in atomic systems using bright squeezed vacuum, it has not…
We investigate the nonlinear optical response of a commercial extended-wavelength In$_{0.81}$Ga$_{0.19}$As photodetector. Degenerate two-photon absorption in the mid-infrared range is observed at room temperature using a quantum cascade…
This study delves into the enhancement of two-photon absorption (2PA) properties in diazaacene-bithiophene derivatives through a synergistic approach combining theoretical analysis and experimental validation. By investigating the…
Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption…
We report the measurement of the entangled two photon absorption cross section, $\sigma_E$, at 808 nm on organic chromophores in solution in a low photon flux regime. We performed measurements on Zinc tetraphenylporphyrin (ZnTPP) in Toluene…
Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…
The phenomena of subthreshold photoemission and absorption under coherent and entangled-photon-pair illumination are reviewed, and the generation and properties of entangled-photon pairs are surveyed. Three prominent forms of subthreshold…
We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and…
We propose a compact high-intensity room-temperature source of entangled photons based on the efficient second-order process of two-photon spontaneous emission from electrically-pumped semiconductor quantum wells in a photonic microcavity.…
Electronic 2D spectroscopy allows nontrivial quantum effects in chemistry and biology to be explored in unprecedented detail. Here, we apply recently developed fluorescence detected coherent 2D spectroscopy to study the light harvesting…
We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with conventional absorption peak at frequency close to intersubband…
Inspired by the unique nonclassical character of two-photon interactions induced by entangled photons, we develop a new comprehensive F\"orster-type formulation for entangled two-photon resonance energy transfer (E2P-RET) mediated by…
For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon…
Entangling microwave and optical photons is one of the promising ways to realize quantum transduction through quantum teleportation. This paper investigates the entanglement of microwave-optical photon pairs generated from an…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Particle entanglement is a fundamental resource upon which are based many quantum technologies. However, the up-to-now best sources of entangled photons rely on parametric down-conversion processes, which are optimal only at certain…
Quantum entanglement offers an incredible resource for enhancing the sensing and spectroscopic probes. Here we develop a microscopic theory for the stimulated Raman scattering (SRS) using entangled photons. We demonstrate that the…
We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered…
We recently demonstrated orders of magnitude enhancement of two-photon absorption (2PA) in direct gap semiconductors due to intermediate state resonance enhancement for photons of very different energies. It can be expected that further…
Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the…