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Related papers: Interlayer exciton valley polarization dynamics in…

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We perform photoluminescence experiments at 4K on two different transition metal diselenide monolayers, namely MoSe2 and WSe2 in magnetic fields $B_z$ up to 9T applied perpendicular to the sample plane. In MoSe2 monolayers the valley…

Materials Science · Physics 2015-06-12 G. Wang , L. Bouet , M. M. Glazov , T. Amand , E. L. Ivchenko , E. Palleau , X. Marie , B. Urbaszek

We investigate the valley depolarization due to the electron-hole exchange interaction in monolayer MoS$_{2}$. Both the long- and short-range parts of the intra- and inter-valley electron-hole exchange interactions are calculated. We find…

Mesoscale and Nanoscale Physics · Physics 2014-05-13 T. Yu , M. W. Wu

In this paper, we employ a fully microscopic approach to the study of interlayer excitons in hetero-bilayers. We use Fowler's and Karplus' method to access the dynamical polarizability of non--interacting interlayer excitons in a…

Mesoscale and Nanoscale Physics · Physics 2021-12-30 M. F. C. Martins Quintela , J. C. G. Henriques , N. M. R. Peres

Van der Waals heterostructures (vdWHs) composed of transition-metal dichalcogenides (TMDs) and layered magnetic semiconductors offer great opportunities to manipulate exciton and valley properties of TMDs. Here, we present…

We investigate the optical properties of spin-triplet interlayer excitons in heterobilayer transition metal dichalcogenides in comparison with the spin-singlet ones. Surprisingly, the optical transition dipole of the spin-triplet exciton is…

Mesoscale and Nanoscale Physics · Physics 2018-05-15 Hongyi Yu , Gui-Bin Liu , Wang Yao

We study experimentally and theoretically the hybridization among intralayer and interlayer moir\'e excitons in a MoSe$_2$/WS$_2$ heterostructure with antiparallel alignment. Using a dual-gate device and cryogenic white light reflectance…

Novel excitonic phenomena emerging in transition metal dichalcogenide (TMDC) heterostructures belong to the most exciting topics in contemporary physics of van der Waals materials. Interlayer excitons (IXs) stand out among those due to…

In van der Waals (vdW) heterostructures formed by stacking two monolayer semiconductors, lattice mismatch or rotational misalignment introduces an in-plane moir\'e superlattice. While it is widely recognized that a moir\'e superlattice can…

The atomic-level vdW heterostructures have been one of the most interesting quantum material systems, due to their exotic physical properties. The interlayer coupling in these systems plays a critical role to realize novel physical…

Strongly Correlated Electrons · Physics 2021-03-16 Xiaoli Ma , Shaohua Fu , Jianwei Ding , Meng Liu , Ang Bian , Fang Hong , Jia-Tao Sun , Xiaoxian Zhang , Xiaohui Yu , Dawei He

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation…

Materials Science · Physics 2015-11-05 G. Wang , I. C. Gerber , L. Bouet , D. Lagarde , A. Balocchi , M. Vidal , E. Palleau , T. Amand , X. Marie , B. Urbaszek

Coupling between exciton states across the Brillouin zone in monolayer transition metal dichalcogenides can lead to ultrafast valley depolarization. Using time- and angle-resolved photoemission, we present momentum- and energy-resolved…

High degree of valley polarization of optically active excitons in transition-metal dichalcogenide monolayers (TMD-MLs) is vital in valley-based photonic applications but known to be likely spoiled by the intrinsic electron-hole exchange…

Mesoscale and Nanoscale Physics · Physics 2021-06-15 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

Strong magnetic fields quench the kinetic energy of electrons, leading to the formation of flat energy bands, known as Landau levels (LLs). In this situation, even weak interactions can drive the emergence of various ordered phases. The…

We argue that the layer electric polarization of noncentrosymmetric layered heterostructures can be generically controlled by light yielding a layer photovoltaic effect (LPE). The LPE possesses a rich phenomenology and can arise from myriad…

Mesoscale and Nanoscale Physics · Physics 2025-01-29 Oles Matsyshyn , Ying Xiong , Arpit Arora , Justin C. W. Song

Heterobilayers formed by stacking two-dimensional atomic crystals are particularly promising for low-dimensional semiconductor optics, as they host interlayer excitons, bound states of electrons and holes residing in different layers. They…

Mesoscale and Nanoscale Physics · Physics 2025-07-31 Suvadip Masanta , Chumki Nayak , Premananda Chatterjee , Atindra Nath Pal , Indrani Bose , Achintya Singha

Optical orientation of localized/bound excitons is shown to be effectively enhanced by the application of magnetic fields as low as 20 mT in monolayer WS$_2$. At low temperatures, the evolution of the polarization degree of different…

We identify an optical excitation mechanism that transfers a valley polarization from photo-excited electron-hole pairs to free charge carriers in twisted WSe$_2$/MoSe$_2$ heterobilayers. For small twist angles, the valley lifetimes of the…

We developed a comprehensive theoretical framework focusing on many-body effects of exciton species in monolayer WS$_2$, including bright and dark excitons, and intra- and inter-valley biexcitons, to investigate valley dynamics in monolayer…

Mesoscale and Nanoscale Physics · Physics 2020-04-17 Fanyao Qu , Helena Bragança , Railson Vasconcelos , Fujun Liu , S-J Xie , Hao Zeng

Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling…

Mesoscale and Nanoscale Physics · Physics 2019-05-20 M. Król , K. Lekenta , R. Mirek , K. Łempicka , D. Stephan , K. Nogajewski , M. R. Molas , A. Babiński , M. Potemski , J. Szczytko , B. Piętka

We report magneto-absorption spectroscopy of gated WSe$_2$ monolayers in high magnetic fields up to 60~T. When doped with a 2D Fermi sea of mobile holes, well-resolved sequences of optical transitions are observed in both $\sigma^\pm$…

Mesoscale and Nanoscale Physics · Physics 2020-10-07 Jing Li , Mateusz Goryca , Nathan P. Wilson , Andreas V. Stier , Xiaodong Xu , Scott A. Crooker