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The structural stability and phonon properties of SnSe/SnS superlattices at finite temperatures have been studied using machine learning force field molecular dynamics and the anharmonic phonon approach. The vertical SnSe/SnS superlattice…

Materials Science · Physics 2025-02-13 Feng-ning Xue , Wei Li , Zi Li , Yong Lu

Spectacular quantum phenomena such as superconductivity often emerge in flat-band systems where Coulomb interactions overpower electron kinetics. Engineering strategies for flat-band physics is therefore of great importance. Here, using…

Motivated by the recently discovered high-$T_c$ superconductor La$_3$Ni$_2$O$_7$, we comprehensively study this system using density functional theory and random phase approximation calculations. At low pressures, the Amam phase is stable,…

Superconductivity · Physics 2024-03-27 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

Superconductivity in nickelates apparently takes place in two different Ni oxidation regimes, namely either for infinite-layer-type compounds close to Ni$^{+}$, or for Ruddlesden-Popper materials close to Ni$^{2+}$. The reduced…

Strongly Correlated Electrons · Physics 2025-12-12 Frank Lechermann , Steffen Bötzel , Ilya M. Eremin

We theoretically investigate a freestanding membrane of infinite-layer nickelate Nd$_{0.85}$Sr$_{0.15}$NiO$_2$ under pressure by constructing a seven-orbital effective model based on first-principles calculations. By performing the…

Infinite-layer nickelates present a new family of potential unconventional superconductors. A key open question is the superconducting pairing symmetry. We present low-temperature measurements of the London penetration depth in optimally…

The recent discovery of superconductivity in Sr-doped NdNiO$_2$, with a critical temperature of $10-15$ K suggests the possibility of a new family of nickel-based high-temperature superconductors (HTS). NdNiO$_{2}$ is the $n=\infty$ member…

Strongly Correlated Electrons · Physics 2021-09-15 Harrison LaBollita , Antia S. Botana

Inelastic neutron scattering is used to measure the temperature dependent phonon dispersion in Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ ($x=0.4$, 0.6). The in-plane $\Sigma_{4}$ octahedral tilt mode softens significantly at the zone boundary of the high…

Strongly Correlated Electrons · Physics 2015-05-13 R. G. Moore , M. D. Lumsden , M. B. Stone , Jiandi Zhang , Y. Chen , J. W. Lynn , R. Jin , D. Mandrus , E. W. Plummer

Infinite-layer nickelate superconductors are typically synthesized as thin films and thus include, besides the more bulk-like inner layers, distinct surface and interface layers in contact with the vacuum and substrate, respectively. Here,…

Strongly Correlated Electrons · Physics 2025-11-26 Leonard M. Verhoff , Liang Si , Karsten Held

Recent works[1-3] reported evidence for charge density waves (CDWs) in infinite layer nickelates (112 structure) based on resonant diffraction at the Ni $L_3$ edge measured at fixed scattering angle. We have found that a measurement with…

Superconductivity · Physics 2023-06-28 J. Pelliciari , N. Khan , P. Wasik , A. Barbour , Y. Li , Y. Nie , J. M. Tranquada , V. Bisogni , C. Mazzoli

Guided by experiment and band structure, we introduce and study a phenomenological Landau theory for the unusual charge and spin ordering associated with the Mott transition in the perovskite nickelates, with chemical formula RNiO$_3$,…

Strongly Correlated Electrons · Physics 2015-05-19 SungBin Lee , Ru Chen , Leon Balents

The discovery that Nd$_{1-x}$Sr$_x$NiO$_2$, with the CaCuO$_2$ infinite-layer structure, superconducts up to 15 K around the hole-doping level $x$=0.2 raises the crucial question of its fundamental electronic and magnetic processes. The…

Superconductivity · Physics 2020-09-22 Mi-Young Choi , W. E. Pickett , K. -W. Lee

Despite exhibiting a similar $d_{x^2-y^2}$ band character to cuprates, infinite-layer nickelates host additional electron pockets that distinguish them from single-band cuprates. The elusive orbital origin of these electron pockets has led…

The metal-insulator transition (MIT) of VO2 is discussed with particular emphasis on the structural instability of the rutile compounds toward dimerization. Ti substitution experiments reveal that the MIT is robust up to 20% Ti…

Strongly Correlated Electrons · Physics 2022-02-01 Zenji Hiroi

The layered square-planar nickelates, Nd$_{n+1}$Ni$_{n}$O$_{2n+2}$, are an appealing system to tune the electronic properties of square-planar nickelates via dimensionality; indeed, superconductivity was recently observed in…

Using advanced dynamical mean-field theory on a realistic level we study the normal-state correlated electronic structure of the high-pressure superconductor La$_3$Ni$_2$O$_7$ and compare the features of the conventional bilayer (2222)…

Strongly Correlated Electrons · Physics 2024-07-26 Frank Lechermann , Steffen Bötzel , Ilya M. Eremin

Controlled introduction of oxygen vacancies offers an effective route to induce metal-to-insulator transition in strongly correlated rare-earth nickelates ($R$NiO$_3$) at room temperature. However, the role played by the rare-earth cations…

Materials Science · Physics 2024-12-30 Devang Bhagat , Ranga Teja Pidathala , Badri Narayanan

The two-dimensional (2D) IV-V semiconductors have attracted much attention due to their fascinating electronic and optical properties. In this work, we predicted three phases of silicon nitrides, denoted $\alpha$-Si$_{2}$N$_{2}$,…

Materials Science · Physics 2024-04-02 Jiesen Li , Wanxing Lin , Junjun Shi , Feng Zhu , Haiwen Xie , Dao-Xin Yao

The discovery of superconductivity in bulk Ruddlesden-Popper La$_3$Ni$_2$O$_7$(LNO327) under high hydrostatic pressure has redefined the recent experimental consensus that nickelate superconductivity is restricted to systems with a $3d^9$…

An extensive theoretical study is performed for wide bandgap crystalline oxides and nitrides, namely, SiO_{2}, GeO_{2}, Al_{2}O_{3}, Si_{3}N_{4}, and Ge_{3}N_{4}. Their important polymorphs are considered which are for SiO_{2}:…

Materials Science · Physics 2009-11-11 C. Sevik , C. Bulutay
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