English

Electronic instability, layer selectivity and Fermi arcs in La$_3$Ni$_2$O$_7$

Strongly Correlated Electrons 2024-07-26 v3 Superconductivity

Abstract

Using advanced dynamical mean-field theory on a realistic level we study the normal-state correlated electronic structure of the high-pressure superconductor La3_3Ni2_2O7_7 and compare the features of the conventional bilayer (2222) Ruddelsden-Popper crystal structure with those of a newly-identified monolayer-trilayer (1313) alternation. Both structural cases display Ni-dz2d_{z^2} flat-band character at low-energy, which drives an electronic instability with a wave vector qI=(0.25,0.25,qz){\bf q_{\rm I}}=(0.25,0.25,q_z) at ambient pressure, in line with recent experimental findings. The 1313 electronic structure exhibits significant layer selectivity, rendering especially the monolayer part to be Mott-critical. At high pressure, this layer selectivity weakens and the 1313 fermiology displays arcs reminiscent to those of high-TcT_c cuprates. In contrast to dominant inter-site self-energy effects in the latter systems, here the Fermi arcs are the result of the multiorbital and multilayer interplay within a correlated flat-band scenario.

Keywords

Cite

@article{arxiv.2403.12831,
  title  = {Electronic instability, layer selectivity and Fermi arcs in La$_3$Ni$_2$O$_7$},
  author = {Frank Lechermann and Steffen Bötzel and Ilya M. Eremin},
  journal= {arXiv preprint arXiv:2403.12831},
  year   = {2024}
}

Comments

7 pages, 4 figures

R2 v1 2026-06-28T15:25:54.598Z