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Unitary Coupled Cluster (UCC) approaches are an appealing route to utilising quantum hardware to perform quantum chemistry calculations, as quantum computers can in principle perform UCC calculations in a polynomially scaling fashion, as…

Quantum Physics · Physics 2022-06-15 Maria-Andreea Filip , Nathan Fitzpatrick , David Muñoz Ramo , Alex J. W. Thom

X-ray photoelectron spectroscopy (XPS) and KLL Auger spectra of aqueous KCl solution were measured for the K$^+$ and Cl$^-$ edges. While the XPS spectra of potassium and chloride have similar structures, both exhibiting only weak satellite…

One of the most significant hurdles to be overcome on the path to practical quantum information processors is dealing with quantum errors. Dynamical decoupling is a particularly promising approach that complements conventional quantum error…

Accurately describing strong electron correlation in complex systems remains a prominent challenge in computational chemistry as near-term quantum algorithms treating total correlation often require prohibitively deep circuits. Here we…

Computational Engineering, Finance, and Science · Computer Science 2026-04-21 Zhanou Liu , Yuhao Chen , Yingjin Ma , Xiao He , Yuxin Deng

Fully microscopic many-body models based on inputs from first principle density functional theory are used to calculate the carrier losses due to radiative- and Auger-recombinations in bulk tellurium. It is shown that Auger processes…

Materials Science · Physics 2022-11-23 Jörg Hader , Sven C. Liebscher , Jerome V. Moloney , Stephan W. Koch

The generator coordinate method of a microscopic cluster model is developed to treat the resonance and scattering of nuclear clusters with complex scaling. We consistently derive the formulation of the complex scaling for the microscopic…

Nuclear Theory · Physics 2023-06-19 Takayuki Myo , Hiroki Takemoto

Collective states in cold nuclei are represented by a wave function that assigns coherent phases to the participating nucleons. The degree of coherence decreases with excitation energy above the yrast line because of coupling to the…

Nuclear Theory · Physics 2020-01-08 S. Frauendorf , C. M. Petrache , R. Schwengner , K. Wimmer

A tenet of time-resolved spectroscopy is -faster laser pulses for shorter timescales- . Here we suggest turning this paradigm around, and slow down the system dynamics via repeated measurements, to do spectroscopy on longer timescales. This…

In quantum dots (QDs) the Auger recombination is a non-radiative scattering process in which the optical transition energy of a charged exciton (trion) is transferred to an additional electron leaving the dot. Electron tunneling from a…

Mesoscale and Nanoscale Physics · Physics 2023-10-23 Marcel Zöllner , Hendrik Mannel , Fabio Rimek , Britta Maib , Nico Schwarz , Andreas D. Wieck , Arne Ludwig , Axel Lorke , Martin Geller

The direct comparison of two different continuum discretization methods towards the solution of a composite particle scattering off a nucleus is presented. The first approach -- the Continumm-Discretized Coupled Channel method -- is based…

Nuclear Theory · Physics 2008-11-26 O. A. Rubtsova , V. I. Kukulin , A. M. Moro

This is the second paper in a cycle investigating the exact solution of loop equations in decaying turbulence. We perform numerical simulations of the Euler ensemble, suggested in the previous work, as a solution to the loop equations. We…

Fluid Dynamics · Physics 2024-03-04 Alexander Migdal

We discuss the decay of a two-level system into an engineered reservoir of coupled harmonic oscillators in the single-excitation manifold and propose its optical simulation with an homogeneous chain of coupled waveguides where individual…

Due to the electron correlation, a fast removal of an electron from a molecule may create a coherent superposition of cationic states and in this way initiate pure electronic dynamics in which the hole-charge left by ionization migrates…

Chemical Physics · Physics 2023-04-03 J. Vester , V. Despré , A. I. Kuleff

The fast nonradiative decay of multiexcitonic states via Auger recombination is a fundamental process affecting a variety of applications based on semiconductor nanostructures. From a theoretical perspective, the description of Auger…

Mesoscale and Nanoscale Physics · Physics 2018-12-26 John P. Philbin , Eran Rabani

This is a sequel to an earlier article on the theory of angular correlation for double photoionization. Here we consider the two-step double photoionization of a rare gas atom under the influence of a polarized photon beam described by…

Atomic Physics · Physics 2009-11-07 Chiranjib Sur , Dipankar Chattarji

We propose an orbital optimized method for unitary coupled cluster theory (OO-UCC) within the variational quantum eigensolver (VQE) framework for quantum computers. OO-UCC variationally determines the coupled cluster amplitudes and also…

Strongly Correlated Electrons · Physics 2020-09-23 Wataru Mizukami , Kosuke Mitarai , Yuya O. Nakagawa , Takahiro Yamamoto , Tennin Yan , Yu-ya Ohnishi

Ultrahigh rate performance of active particles used in lithium-ion battery electrodes has been revealed by single-particle measurements, which indicates a huge potential for developing high-power batteries. However, the charging/discharging…

Chemical Physics · Physics 2022-07-25 Ruoyu Xiong , Mengyuan Zhou , Longhui Li , Jia Xu , Maoyuan Li , Bo Yan , Dequn Li , Yun Zhang , Huamin Zhou

The formation of clusters in nuclear matter is investigated, which occurs e.g. in low energy heavy ion collisions or core-collapse supernovae. In astrophysical applications, the excluded volume concept is commonly used for the description…

Nuclear Theory · Physics 2011-11-24 Matthias Hempel , Jürgen Schaffner-Bielich , Stefan Typel , Gerd Röpke

Classical nucleation theory (CNT), linking rare nucleation events to the free energy landscape of a growing nucleus, is central to understanding phase-change kinetics in passive fluids. Nucleation in non-equilibrium systems is much harder…

Soft Condensed Matter · Physics 2023-03-15 M. E. Cates , C. Nardini

Atomic nuclei are self-organized, many-body quantum systems bound by strong nuclear forces within femtometer-scale space. These complex systems manifest a variety of shapes, traditionally explored using non-invasive spectroscopic techniques…

Nuclear Experiment · Physics 2024-11-19 STAR Collaboration