Related papers: Molecular Auger Decay Rates from Complex-Variable …
Introducing an active space approximation is inevitable for the quantum computations of chemical systems. However, this approximation ignores the electron correlations related to non-active orbitals. Here, we propose a computational method…
The coupled cluster iteration scheme is analysed as a multivariate discrete-time map using nonlinear dynamics and synergetics. The nonlinearly coupled set of equations to determine the cluster amplitudes are driven by a fraction of the…
We have analyzed the cascade of secondary electrons in diamond and amorphous carbon generated by the thermalisation of a single Auger electron. The elastic electron mean free path was calculated as a function of impact energy in the…
In this article, a numerical analysis of the asymptotic behavior of the discrete energy associated to a dissipative coupled wave system is conducted. The numerical approximation of the system is constructed using the P1 finite element…
Alpha emission from a nucleus is a fundamental decay process in which the alpha particle formed inside the nucleus tunnels out through the potential barrier. We describe alpha decay of $^{212}$Po and $^{104}$Te by means of the configuration…
With an eye on plasma walls we investigate, within an effective model for the two active electrons involved in the process, secondary electron emission due to Auger de-excitation of metastable nitrogen $N_2(^3\sigma^+_u)$ molecules at…
Exponential decay laws describe systems ranging from unstable nuclei to fluorescent molecules, in which the probability of jumping to a lower-energy state in any given time interval is static and history-independent. These decays, involving…
${\textbf{Background:}}$ Atomic nuclei often exhibit collective rotational-like behavior in highly excited states, well above the particle emission threshold. What determines the existence of collective motion in the continuum region, is…
A general shell model formalism for the nonmesonic weak decay of the hypernuclei has been developed.It involves a partial wave expansion of the emitted nucleon waves,preserves naturally the antisymmetrization between the escaping particles…
Investigation of decay and scattering processes of particles in a vortex state offers a novel and promising approach for probing particle structure. Our study reveals distinct properties of vortex neutron decay, which deviate from those of…
We describe a new mechanism of decoherence in excited atoms as a result of thermal particles scattering by the atomic nucleus. It is based on the idea that a single scattering will produce a sudden displacement of the nucleus, which will be…
This report presents a new approach for treating the coupling of electrons and nuclei in quantum mechanical calculations for molecules and condensed matter. It includes the standard "Born-Oppenheimer approximation" as a special case but…
Electron acoustic waves (EAWs) are nonlinear plasma modes characterized by electron trapping, which suppresses the usual Landau damping. Despite being predicted in the 1990s, their excitation and decay mechanisms remain a subject of active…
In a recent letter [Phys. Rev. Lett. 110, 177406 (2013)], presenting a spectroscopic study of the electrons emitted from the GaN p-cap of a forward-biased InGaN/GaN light-emitting diode (LED), the authors observed at least two distinct…
Irradiation of a molecular system by an intense laser field can trigger dynamics of both electronic and nuclear subsystems. The lighter electrons usually move on much faster, attosecond time scale but the slow nuclear rearrangement damps…
Linear and nonlinear ion-acoustic waves are studied in a fluid model for non-relativistic, unmagnetized quantum plasma with electrons with an arbitrary degeneracy degree. The equation of state for electrons follows from a local Fermi-Dirac…
The rate at which excited charge carriers relax to their equilibrium state affects many aspects of the performance of nanoscale devices, including switching speed, carrier mobility and luminescent efficiency. Better understanding of the…
We theoretically study the longitudinal relaxation of a nitrogen-vacancy (NV) center surrounded by a 13C nuclear spin bath in diamond. By incorporating electron spin in the cluster, we generalize the cluster-correlation expansion (CCE) to…
The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…
We present a new method for ultrafast spectroscopy of molecular photoexcited dynamics. The technique uses a pair of femtosecond pulses: a photoexcitation pulse initiating excited state dynamics followed by a soft x-ray (SXR) probe pulse…