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Related papers: Evolution of electronic structure of Ru-doped sing…

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We report structural, magnetic, transport and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 < x< 0.65). Ca2RuO4 is a structurally-driven Mott insulator with a metal-insulator transition at TMI = 357 K, which is well separated from…

Strongly Correlated Electrons · Physics 2016-04-26 S. J. Yuan , J. Terzic , J. C. Wang , S. Aswartham , W. H. Song , F. Ye , G. Cao

We investigated the temperature-dependent evolution of the electronic structure of the Jeff,1/2 Mott insulator Sr2IrO4 using optical spectroscopy. The optical conductivity spectra $\sigma(\omega)$ of this compound has recently been found to…

Strongly Correlated Electrons · Physics 2009-10-23 S. J. Moon , Hosub Jin , W. S. Choi , J. S. Lee , S. S. A. Seo , J. Yu , G. Cao , T. W. Noh , Y. S. Lee

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

Strongly Correlated Electrons · Physics 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

One way to induce insulator to metal transitions in the spin-orbit Mott insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by…

Strongly Correlated Electrons · Physics 2021-09-08 Véronique Brouet , Paul Foulquier , Alex Louat , François Bertran , Patrick Le Fèvre , Julien E. Rault , Dorothée Colson

Here, we report an investigation of structural, magnetic and electronic properties in Y-doped layered iridate (Sr$_{1-x}$Y$_x$)$_2$IrO$_4$ ($x$ $\leq$ 0.1). The parent Sr$_2$IrO$_4$ is a well-studied spin-orbit coupling (SOC) induced…

Strongly Correlated Electrons · Physics 2021-03-17 Imtiaz Noor Bhatti , A. K. Pramanik

Sr2IrO4 is a magnetic insulator assisted by strong spin-orbit coupling (SOC) whereas the Sr2RuO4 is a p-wave superconductor. The contrasting ground states have been shown to result from the critical role of the strong SOC in the iridate.…

Strongly Correlated Electrons · Physics 2016-04-26 S. J. Yuan , S. Aswartham , J. Terzic , H. Zheng , H. D. Zhao , P. Schlottmann , G. Cao

Stoichiometric Sr2IrO4 is a ferromagnetic Jeff = 1/2 Mott insulator driven by strong spin-orbit coupling. Introduction of very dilute oxygen vacancies into single-crystal Sr2IrO4-delta with delta < 0.04 leads to significant changes in…

Strongly Correlated Electrons · Physics 2010-08-30 O. B. Korneta , Tongfei Qi , S. Chikara , S. Parkin L. E. De Long , P. Schlottmann , G. Cao

VO2, of interest for decades due to both its phenomenology and its potential applications, has a monoclinic distortion of the rutile crystal structure at ambient temperature that is coupled to its metal-insulator transition (MIT). In…

Materials Science · Physics 2022-07-14 Xin Gui , Robert J. Cava

Neutron single crystal diffraction and rotational anisotropy optical second harmonic generation data are presented resolving the nature of the structural distortion realized in electron-doped (Sr$_{1-x}$La$_x$)$_3$Ir$_2$O$_7$ with $x=0.035$…

Strongly Correlated Electrons · Physics 2017-06-28 Tom Hogan , Xiaoping Wang , H. Chu , David Hsieh , Stephen D. Wilson

Sr3Ir2O7 exhibits a novel Jeff=1/2 insulating state that features a splitting between Jeff=1/2 and 3/2 bands due to spin-orbit interaction. We report a metal-insulator transition in Sr3Ir2O7 via either dilute electron doping (La3+ for Sr2+)…

Strongly Correlated Electrons · Physics 2015-06-15 L. Li , P. P. Kong , T. F. Qi , C. Q. Jin , S. J. Yuan , L. E. DeLong , P. Schlottmann , G. Cao

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

Strongly Correlated Electrons · Physics 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic…

Strongly Correlated Electrons · Physics 2017-04-25 H. Chu , L. Zhao , A. de la Torre , T. Hogan , S. D. Wilson , D. Hsieh

Sr2IrO4 was predicted to be a high temperature superconductor upon electron doping since it highly resembles the cuprates in crystal structure, electronic structure and magnetic coupling constants. Here we report a scanning tunneling…

Superconductivity · Physics 2015-11-11 Y. J. Yan , M. Q. Ren , H. C. Xu , B. P. Xie , R. Tao , H. Y. Choi , N. Lee , Y. J. Choi , T. Zhang , D. L. Feng

The physics of doped Mott insulators remains controversial after decades of active research, hindered by the interplay among possible competing orders and fluctuations. It is thus highly desired to distinguish the intrinsic characters of…

Despite many efforts to rationalize the strongly correlated electronic ground states in doped Mott insulators, the nature of the doping induced insulator to metal transition is still a subject under intensive investigation. Here we probe…

The simultaneous presence of sizable spin-orbit interactions and electron correlations in iridium oxides has led to predictions of novel ground states including Dirac semimetals, Kitaev spin liquids, and superconductivity. Electron and hole…

Strongly Correlated Electrons · Physics 2017-02-22 S. Chikara , G. Fabbris , J. Terzic , G. Cao , D. Khomskii , D. Haskel

The spectral properties of a one-dimensional (1D) single-chain Mott insulator Sr$_2$CuO$_{3}$ have been studied in angle-resolved photoemission and optical spectroscopy, at half filling and with small concentrations of extra charge doped…

Strongly Correlated Electrons · Physics 2008-03-04 T. Valla , T. E. Kidd , P. D. Johnson , K. W. Kim , C. C. Homes , G. D. Gu

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

In this work, the high entropy oxide A2CuO4 Ruddlesden-Popper (La0.2Pr0.2Nd0.2Sm0.2Eu0.2)2CuO4 is explored by charge doping with Ce+4 and Sr+2 at concentrations known to induce superconductivity in the simple parent compounds, Nd2CuO4 and…

Solid state synthesis and physical mechanisms of electrical conductivity variation in polycrystalline, strontium doped indium oxide In2O3:(SrO)x were investigated for materials with different doping levels at different temperatures…

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