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Correlated Dirac semimetal phases emerge in lightly doped (Tb- or La-doped) Mott insulator Sr$_2$IrO$_4$, where a d-wave symmetry-breaking order underlying a pseudogap plays a crucial role in determining the nature of Dirac degeneracy,…

Strongly Correlated Electrons · Physics 2021-01-18 Sun-Woo Kim , Myungjun Kang , Sangmo Cheon

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

We present measurements of the optical spectra on single crystals of spinel-type compound \cis. This material undergoes a sharp metal-insulator transition at 230 K. Upon entering the insulating state, the optical conductivity shows an…

Strongly Correlated Electrons · Physics 2009-11-10 N. L. Wang , G. H. Cao , P. Zheng , G. Li , Z. Fang , T. Xiang , H. Kitazawa , T. Matsumoto

We investigate the electronic structure and magnetic properties of a $J_\text{eff} = 1/2$ iridate Ca$_4$IrO$_6$ and the implications of doping electrons and holes using ab initio density functional theory. Our calculations considering…

Strongly Correlated Electrons · Physics 2022-09-02 Avishek Singh , Jayita Chakraborty , Nirmal Ganguli

Iridium-based 5d transition-metal oxides are attractive candidates for the study of correlated electronic states due to the interplay of enhanced crystal-field, Coulomb and spin-orbit interaction energies. At ambient pressure, these…

Strongly Correlated Electrons · Physics 2014-06-05 D. A. Zocco , J. J. Hamlin , B. D. White , B. J. Kim , J. R. Jeffries , S. T. Weir , Y. K. Vohra , J. W. Allen , M. B. Maple

A detailed study of the effect caused by the partial substitution of Ru by Ir on the magnetic and superconducting properties of the ruthenocuprate Ru(1-x)Ir(x)Sr2GdCu2o8; 0 <= x <= 0.10; is presented. The combined experimental results of…

Superconductivity · Physics 2007-05-23 A. R. Jurelo , S. Andrade , R. F. Jardim , F. C. Fonseca , M. S. Torikachvili , A. H. Lacerda , L. Ben-Dor

We present a single crystal Cu NMR study of the cuprate superconductor La$_{2-x}$Sr$_{x}$CuO$_4$ with hole doping levels between $x=2$\% and $8$\%. Measurements with short spin echo times enable us to systematically study the local…

We have investigated the temperature evolution of magnetism and its interrelation with structural parameters in perovskite-based layered compound Sr$_2$IrO$_4$, which is believed to be a $J_{eff}$ = 1/2 Mott insulator. The structural…

Strongly Correlated Electrons · Physics 2014-12-15 Imtiaz Noor Bhatti , R. Rawat , A. Banerjee , A. K. Pramanik

The ab-plane optical conductivity of eleven single crystals, belonging to the families Sr2-xCuO2Cl2, Y1-xCaxBa2Cu3O6, Bi2Sr2-xLaxCuO6, and Bi2Sr2CaCu2O8 has been measured with hole concentrations p between 0 and 0.18, and for 6 K < T < 500…

Superconductivity · Physics 2015-03-17 D. Nicoletti , P. Di Pietro , O. Limaj , P. Calvani , U. Schade , S. Ono , Yoichi Ando , S. Lupi

Layered ruthenates are prototype materials with strong structure-property correlations. We report the structural and physical properties of double-layered perovskite Sr3(Ru1-xMnx)2O7 single crystals with 0<=x<=0.7. Single crystal x-ray…

Strongly Correlated Electrons · Physics 2012-05-01 Biao Hu , Gregory T. McCandless , V. O. Garlea , S. Stadler , Yimin Xiong , Julia Y. Chan , E. W. Plummer , R. Jin

We use single-crystal neutron diffraction to determine the crystal structure symmetry and the magnetic evolution in the rhodium doped iridates $\rm Sr_2Ir_{1-x}Rh_{x}O_4$ ($0\leq x \leq 0.16$). Throughout this doping range, the crystal…

The effects of Ir doping on the thermoelectric properties of Pt1-xIrxSb2 (x = 0, 0.01, 0.03, and 0.1) with pyrite structure were studied. Measurements of electrical resistivity rho, Seebeck coefficient S, and thermal conductivity kappa were…

Strongly Correlated Electrons · Physics 2012-06-21 Y. Nishikubo , S. Nakano , K. Kudo , M. Nohara

A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr$_2$IrO$_4$ a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and…

Strongly Correlated Electrons · Physics 2016-01-11 L. Zhao , D. H. Torchinsky , H. Chu , V. Ivanov , R. Lifshitz , R. Flint , T. Qi , G. Cao , D. Hsieh

SrPt$_2$As$_2$ single crystals with CaBe$_2$Ge$_2$-type structure were synthesized by self-melting technique. X-ray diffraction, transmission electron microscopy, electrical resistivity, specific heat and optical spectroscopy measurements…

Superconductivity · Physics 2013-05-30 A. F. Fang , T. Dong , H. P. Wang , Z. G. Chen , B. Cheng , Y. G. Shi , P. Zheng , G. Xu , L. Wang , J. Q. Li , N. L. Wang

We propose the parent compound of the newly discovered superconducting nickelate Nd$_{1-x}$Sr$_{x}$NiO$_{2}$ as a self-doped Mott insulator, in which the low-density Nd-$5d$ conduction electrons couple to localized Ni-3$% d_{x^{2}-y^{2}}$…

Superconductivity · Physics 2020-01-15 Guang-Ming Zhang , Yi-Feng Yang , Fu-Chun Zhang

Centimeter-sized single crystals of Sr$_{1.5}$La$_{0.5}$RhO$_{4}$ were grown by the floating zone method at oxygen pressures of 20~bar. The quality of our single crystals was confirmed by X-ray Laue, powder and single crystal X-ray…

Strongly Correlated Electrons · Physics 2017-09-06 Z. W. Li , H. Guo , Z. Hu , T. S. Chan , K. Nemkovski , A. C. Komarek

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

Strongly Correlated Electrons · Physics 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

A systematic LSDA+U study of doping effects on the electronic and structural properties of single layer CoO2 is presented. Undoped CoO2 is a charge transfer insulator within LSDA+U and a metal with a high density of states (DOS) at the…

Superconductivity · Physics 2007-05-23 Peihong Zhang , Weidong Luo , Vincent H. Crespi , Marvin L. Cohen , Steven G. Louie

We investigated the electronic structures of the two-dimensional layered perovskite Sr$_{2}$\textit{M}O$_{4}$ (\textit{M}=4\textit{d} Ru, 4\textit{d} Rh, and 5\textit{d} Ir) using optical spectroscopy and polarization-dependent O…

Strongly Correlated Electrons · Physics 2009-11-11 S. J. Moon , M. W. Kim , K. W. Kim , Y. S. Lee , J. -Y. Kim , J. -H. Park , B. J. Kim , S. -J. Oh , S. Nakatsuji , Y. Maeno , I. Nagai , S. I. Ikeda , G. Cao , T. W. Noh

We study the effect of isoelectronic doping and external pressure in tuning the ground state of the honeycomb iridate Na$_2$IrO$_3$ by combining optical spectroscopy with synchrotron x-ray diffraction measurements on single crystals. The…

Strongly Correlated Electrons · Physics 2018-01-31 V. Hermann , J. Ebad-Allah , F. Freund , I. M. Pietsch , A. Jesche , A. A. Tsirlin , J. Deisenhofer , M. Hanfland , P. Gegenwart , C. A. Kuntscher