Related papers: Quantum nonlinear spectroscopy of single nuclear s…
This thesis focuses on the experimental creation and detection of a variety of quantum correlations using nuclear magnetic resonance hardware. Quantum entanglement, being most common and counter-intuitive, is one of the main type considered…
Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…
Two-dimensional Nuclear Magnetic Resonance (NMR) is essential in molecular structure determination. The Nitrogen-Vacancy (NV) center in diamond has been proposed and developed as an outstanding quantum sensor to realize NMR in nanoscale. In…
Quantum search is a quantum mechanical technique for searching N possibilities in only sqrt(N) steps. This paper gives a fresh perspective on the algorithm in terms of a resonance phenomenon which is implemented through classical coupled…
The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…
This paper surveys our recent research on quantum information processing by nuclear magnetic resonance (NMR) spectroscopy. We begin with a geometric introduction to the NMR of an ensemble of indistinguishable spins, and then show how this…
We propose the use of non-equally spaced decoupling pulses for high-resolution selective addressing of nuclear spins by a quantum sensor. The analytical model of the basic operating principle is supplemented by detailed numerical studies…
We realize a two-qubit sensor designed for achieving high spectral resolution in quantum sensing experiments. Our sensor consists of an active "sensing qubit" and a long-lived "memory qubit", implemented by the electronic and the…
One of the key challenges in spectroscopy is inhomogeneous broadening that masks the homogeneous spectral lineshape and the underlying coherent dynamics. A variety of techniques including four-wave mixing and spectral hole-burning are used…
The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…
In recent years, electro-optic sampling, which is based on Pockel's effect between an electromagnetic mode and a copropagating, phase-matched ultrashort probe, has been largely used for the investigation of broadband quantum states of…
Atomic scale qubits, as may be realized in nitrogen vacancy (NV) centers in diamond, offer the opportunity to study magnetic field noise with nanometer scale spatial resolution. Using these spin qubits, one can learn a great deal about the…
Developing superior quantum sensing strategies ranging from ultra-high precision measurement to complex structural analysis is at the heart of quantum technologies. While strategies using quantum resources, such as entanglement among…
We present a general method to detect nonclassical radiation fields with systems of on-off detectors. We especially study higher order correlations for the identification of nonclassical radiation. This allows us to directly characterize…
Precision spectroscopy has long played a central role in testing the foundations of physics, from the early insights that led to the development of quantum mechanics to the validation of quantum electrodynamics and the determination of…
The field of quantum sensing explores the use of quantum phenomena to measure a broad range of physical quantities, of both static and time-dependent types. An important figure of merit for sensing time dependent signals is the spectral…
A qubit can be used as a sensitive spectrum analyzer of its environment. Here we show how the problem of spectral analysis of noise induced by a strongly coupled environment can be solved for discrete spectra. Our analytical model shows…
A bipartite quantum system in a mixed state can exhibit nonclassical correlations, which can go beyond quantum entanglement. While quantum discord is the standard measure of quantifying such general quantum correlations, the nonclassicality…
Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…
"Quantum sensing" describes the use of a quantum system, quantum properties or quantum phenomena to perform a measurement of a physical quantity. Historical examples of quantum sensors include magnetometers based on superconducting quantum…