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The correlations of fluctuations are key to studying fundamental quantum physics and quantum many-body dynamics. They are also useful information for understanding and combating decoherence in quantum technology. Nonlinear spectroscopy and…

Quantum Physics · Physics 2023-09-04 Brian Chung Hang Cheung , Ren-Bao Liu

Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection…

Quantum spectroscopy with single two level systems has considerably improved our ability to detect weak signals. Recently it was realized that for classical signals, precision and resolution of quantum spectroscopy is limited mainly by…

Quantum Physics · Physics 2018-08-01 Tuvia Gefen , Maxim Khodas , Liam P. McGuinness , Fedor Jelezko , Alex Retzker

Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 S. Alex Breitweiser , Mathieu Ouellet , Tzu-Yung Huang , Tim H. Taminiau , Lee C. Bassett

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of…

Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…

Quantum Physics · Physics 2017-02-01 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

Recent advances in engineering and control of nanoscale quantum sensors have opened new paradigms in precision metrology. Unfortunately, hardware restrictions often limit the sensor performance. In nanoscale magnetic resonance probes, for…

Quantum Physics · Physics 2017-07-05 A. Ajoy , Y. X. Liu , K. Saha , L. Marseglia , J. -C. Jaskula , U. Bissbort , P. Cappellaro

Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…

Sensing, localising and identifying individual nuclear spins or frequency components of a signal in the presence of a noisy environments requires the development of robust and selective methods of dynamical decoupling. An important…

Quantum correlations are key information about the structures and dynamics of quantum many-body systems. There are many types of high-order quantum correlations with different time orderings, but only a few of them are accessible to the…

Quantum Physics · Physics 2022-06-14 Ze Wu , Ping Wang , Tianyun Wang , Yuchen Li , Ran Liu , Yuquan Chen , Xinhua Peng , Ren-Bao Liu , Jiangfeng Du

Quantum sensing takes advantage of well controlled quantum systems for performing measurements with high sensitivity and precision. We have implemented a concept for quantum sensing with arbitrary frequency resolution, independent of the…

Quantum Physics · Physics 2017-06-07 J. M. Boss , K. S. Cujia , J. Zopes , C. L. Degen

Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Ulf Bissbort , Mikhail D. Lukin , Ronald L. Walsworth , Paola Cappellaro

Quantum entanglement has long been recognized as an important resource for quantum sensing. In this work, we demonstrate the use of multiple-quantum solid-state NMR for quantum sensing by creating, manipulating, and detecting large clusters…

Quantum Physics · Physics 2025-12-02 Conan Alexander , T S Mahesh

The analysis of a continuous measurement record $z(t)$ poses a fundamental challenge in quantum measurement theory. Different approaches have been used in the past as records can, e.g., exhibit predominantly Gaussian noise, telegraph noise,…

Quantum Physics · Physics 2024-06-12 Markus Sifft , Daniel Hägele

The spin of an electron in a semiconductor quantum dot represents a natural nanoscale solid state qubit. Coupling to nuclear spins leads to decoherence that limits the number of allowed quantum logic operations for this qubit. Traditional…

Mesoscale and Nanoscale Physics · Physics 2016-07-13 Alexander Bechtold , Fuxiang Li , Kai Müller , Tobias Simmet , Per-Lennart Ardelt , Jonathan J. Finley , Nikolai A. Sinitsyn

Nuclear magnetic resonance (NMR) has enormous applications. Two-dimensional NMR is an essential technique to characterize correlations between nuclei and, hence, molecule structures. Towards the ultimate goal of single-molecule NMR,…

Quantum Physics · Physics 2016-11-30 Wen-Long Ma , Ren-Bao Liu

Ultimate limits for sensing of fields and forces are set by the quantum noise of a sensor. Entanglement allows for suppression of such noise and for achieving sensitivity beyond standard quantum limits. Applicability of quantum optical…

Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications,…

Quantum Physics · Physics 2022-05-12 Ziwei Qiu , Uri Vool , Assaf Hamo , Amir Yacoby

System noise identification is crucial to the engineering of robust quantum systems. Although existing quantum noise spectroscopy (QNS) protocols measure an aggregate amount of noise affecting a quantum system, they generally cannot…

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