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Combining the ability to prepare high-quality, intrinsic Bi$_2$Te$_3$ topological insulator thin films of low carrier density with in-situ protective capping, we demonstrate a pronounced, gate-tunable change in transport properties of…

Mesoscale and Nanoscale Physics · Physics 2016-07-04 Prosper Ngabonziza , Martin P. Stehno , Hiroaki Myoren , Viola A. Neumann , Gertjan Koster , Alexander Brinkman

We demonstrate the capability of growing high quality ultrathin films of the topological insulators Bi2Se3 and Bi2Te3 using molecular beam epitaxy. Unlike previous growth techniques, which often pin the Fermi energy in the conduction band…

Materials Science · Physics 2014-01-15 J. J. Lee , F. T. Schmitt , R. G. Moore , I. M. Vishik , Y. Ma , Z. X. Shen

Combined in-situ x-ray photoemission spectroscopy, scanning tunnelling spectroscopy and angle resolved photoemission spectroscopy of molecular beam epitaxy grown Bi2Te3 on lattice mismatched substrates reveal high quality stoichiometric…

Alloys of Bi$_2$Te$_3$ and Sb$_2$Te$_3$ ((Bi$_{1-x}$Sb$_x$)$_2$Te$_3$) have played an essential role in the exploration of topological surface states, allowing us to study phenomena that would otherwise be obscured by bulk contributions to…

Materials Science · Physics 2018-04-04 Kane L Scipioni , Zhenyu Wang , Yulia Maximenko , Ferhat Katmis , Charlie Steiner , Vidya Madhavan

Electrical field control of the carrier density of topological insulators (TI) has greatly expanded the possible practical use of these materials. However, the combination of low temperature local probe studies and a gate tunable TI device…

Mesoscale and Nanoscale Physics · Physics 2013-04-15 Tong Zhang , Niv Levy , Jeonghoon Ha , Young Kuk , Joseph A. Stroscio

We demonstrate the ability to reduce the carrier concentration of thin films of the topological insulator (TI) Bi2Se3 by utilizing a novel approach, namely non-volatile electrostatic gating via corona charging of electret polymers.…

Mesoscale and Nanoscale Physics · Physics 2018-04-11 R. M. Ireland , Liang Wu , M. Salehi , S. Oh , N. P. Armitage , H. E. Katz

Although over the past number of years there have been many advances in the materials aspects of topological insulators (TI), one of the ongoing challenges with these materials is the protection of them against aging. In particular, the…

Materials Science · Physics 2015-10-08 Maryam Salehi , Matthew Brahlek , Nikesh Koirala , Jisoo Moon , Liang Wu , N. P. Armitage , Seongshik Oh

SrMoO$_3$ is a promising material for its excellent electrical conductivity, but growing high-quality thin films remains a challenge. Here we synthesized epitaxial films of SrMoO$_3$ using the molecular beam epitaxy (MBE) technique under a…

Here, we study the effects of a GaAs buffer layer on the structural, magnetic, and transport properties of Cr$_y$(Bi$_x$Sb$_{1-x}$)$_{2-y}$Te$_3$ magnetic topological insulator thin films and compare them with those of…

Mesoscale and Nanoscale Physics · Physics 2025-02-03 Yusuke Nakazawa , Takafumi Akiho , Kiyoshi Kanisawa , Hiroshi Irie , Norio Kumada , Koji Muraki

Topological insulators (TIs) are exotic materials which have topologically protected states on the surface due to the strong spin-orbit coupling. However, a lack of ordered growth of TI thin films on amorphous dielectrics and/or insulators…

As a 3D topological insulator, bismuth selenide (Bi2Se3) has potential applications for electrically and optically controllable magnetic and optoelectronic devices. How the carriers interact with lattice is important to understand the…

Bismuth selenide (Bi2Se3) is a good topological insulator (TI) with its surface band Dirac point inside the bulk bandgap. However, Bi2Se3 films grown by molecular beam epitaxy (MBE) often require tuning of Fermi level near the Dirac point…

Mesoscale and Nanoscale Physics · Physics 2025-09-11 Shu-Wei Wang , Hang Chi , Jui-Che Chung

High quality chromium (Cr) doped three-dimensional topological insulator (TI) Sb2Te3 films are grown via molecular beam epitaxy on heat-treated insulating SrTiO3(111) substrates. We report that the Dirac surface states are insensitive to Cr…

Mesoscale and Nanoscale Physics · Physics 2016-02-03 Cui-Zu Chang , Min-Hao Liu , Zuo-Cheng Zhang , Yayu Wang , Ke He , Qi-Kun Xue

The integration of quantum materials like topological insulators (TIs) with magnetic insulators (MIs) has important technological implications for spintronics and quantum computing. Here we report excellent crystallinity of c-axis oriented…

Materials Science · Physics 2019-02-12 C. C. Chen , K. H. M. Chen , Y. T. Fanchiang , C. C. Tseng , S. R. Yang , C. N. Wu , M. X. Guo , C. K. Cheng , C. T. Wu , M. Hong , J. Kwo

Quality of epitaxial films strongly depends on their structural and chemical match with the substrates: the more closely they match, the better the film quality is. Topological insulators (TI) such as Bi2Se3 thin films are of no exception.…

Materials Science · Physics 2020-06-25 Xiong Yao , Jisoo Moon , Sang-Wook Cheong , Seongshik Oh

The tunability of the chemical potential for a wide range encompassing the Dirac point is important for many future devices based on topological insulators. Here we report a method to fabricate highly efficient top gates on epitaxially…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Fan Yang , A. A. Taskin , Satoshi Sasaki , Kouji Segawa , Yasuhide Ohno , Kazuhiko Matsumoto , Yoichi Ando

An important challenge in the field of topological materials is to carefully disentangle the electronic transport contribution of the topological surface states from that of the bulk. For Bi$_2$Te$_3$ topological insulator samples, bulk…

Materials Science · Physics 2018-05-02 Prosper Ngabonziza , Yi Wang , Alexander Brinkman

Metal chalcogenides are promising layered topological materials, yet their electronic performance is often limited by parasitic bulk conduction arising from defects that introduce excess carriers and shift the Fermi level out of the…

(Bi$_{1-x}$Sb$_x$)$_2$Te$_3$ alloys are non-degenerate topological insulators (TIs) whose Dirac point (DP) can be tuned within the bulk bandgap by varying the composition, effectively reducing bulk conduction while allowing surface carrier…

Atomically sharp epitaxial growth of Bi2Se3 films is achieved on Si (111) substrate with MBE (Molecular Beam Epitaxy). Two-step growth process is found to be a key to achieve interfacial-layer-free epitaxial Bi2Se3 films on Si substrates.…

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