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Nanofluidics is an emerging field offering innovative solutions for energy harvesting and desalination. The efficiency of these applications depends strongly on liquid-solid slip, arising from a favorable ratio between viscosity and…

Soft Condensed Matter · Physics 2022-08-16 Cecilia Herrero , Gabriele Tocci , Samy Merabia , Laurent Joly

We studied the phase behavior of charged and sterically stabilized colloids using confocal microscopy in a less polar solvent (dielectric constant 5.4). Upon increasing the colloid volume fraction we found a transition from a fluid to a…

In this paper we present a new thermodynamically consistent phase transition model describing the evolution of a liquid substance, e.g., water, in a rigid container $\Omega$ when we freeze the container. Since the density $\varrho_{2}$ of…

Analysis of PDEs · Mathematics 2014-01-10 Michel Fremond , Elisabetta Rocca

We present a multi-scale formalism that accounts for the formation of nano-scale bubbles/cavities owing to a burst of water molecules after the passage of high energy charged particles that leads to the formation of hot non-ionizing…

We have employed the highly accurate complex absorbing potential based ionization potential equation-of-motion coupled cluster singles and doubles (CAP-IP-EOM-CCSD) method to study the various intermolecular decay processes in ionized…

Chemical Physics · Physics 2022-08-05 Ravi Kumar , Aryya Ghosh , Nayana Vaval

We present a detailed analysis of the molecular kinetics of CHCl$_3$ in a range of temperatures covering the solid and liquid phases. Using nuclear quadrupolar resonance we determine the relaxation times for the molecular rotations in solid…

Chemical Physics · Physics 2013-10-24 Nirvana B. Caballero , Mariano Zuriaga , Marcelo A. Carignano , Pablo Serra

The influence has been studied of the ionization laser polarization on the effective temperature of an ultracold electron source, which is based on near-threshold photoionization. This source is capable of producing both high-intensity and…

Atomic Physics · Physics 2013-12-24 W. J. Engelen , D. J. Bakker , O. J. Luiten , E. J. D. Vredenbregt

The Bernal-Fowler ice rules stipulate that each water molecule in an ice crystal should form four hydrogen bonds. However, in extreme or constrained conditions, the arrangement of water molecules deviates from conventional ice rules,…

Statistical Mechanics · Physics 2024-07-12 Pavan Ravindra , Xavier R. Advincula , Christoph Schran , Angelos Michaelides , Venkat Kapil

Experiments show that isochoric (constant-volume) conditions enhance supercooling stability relative to isobaric (constant-pressure) conditions. Here, combining Helmholtz equilibrium thermodynamics with a first-order perturbation…

Soft Condensed Matter · Physics 2026-04-30 Boris Rubinsky

Water exhibits rich polymorphism, where more than 20 crystalline phases have been experimentally reported. Five of them are metastable and form at low temperatures by either heating amorphous ice or degassing clathrate hydrates. However,…

It is proposed that the rapid observed homogeneous nucleation of ice dust in a cold, weakly-ionized plasma depends on the formation of hydroxide (OH$^-$) by fast electrons impacting water molecules. These OH$^{-}$ ions attract neutral water…

Plasma Physics · Physics 2022-08-31 Paul M. Bellan

Thermodiffusion in aqueous electrolyte solutions exhibits complex dependencies on temperature, concentration, and salt composition, yet its microscopic origins remain incompletely understood. Here, we employ non-equilibrium molecular…

Soft Condensed Matter · Physics 2026-04-21 Guansen Zhao , Fernando Bresme

Freezing of simple liquid metals and the relative stabilities of competing crystalline solids are investigated using thermodynamic perturbation theory, the interactions between ions being modeled by effective pair potentials derived from…

Materials Science · Physics 2009-10-31 A. R. Denton , G. Kahl , J. Hafner

Based on the earlier obtained equations of state for the ternary systems H2O-CO2-CaCl2 and H2O-CO2-NaCl, an equation of state for the four-component fluid system H2O-CO2-NaCl-CaCl2 is derived in terms of the Gibbs excess free energy. A…

Chemical Physics · Physics 2022-09-22 Mikhail V. Ivanov

First-principles calculations based on density functional theory and the pseudopotential method have been used to investigate the energetics of H$_2$O adsorption on the (110) surface of TiO$_2$ and SnO$_2$. Full relaxation of all atomic…

mtrl-th · Physics 2009-10-28 J. Goniakowski , M. J. Gillan

In the coldest (10--20 K) regions of the interstellar medium, the icy surfaces of interstellar grains serve as solid-state supports for chemical reactions. Among their plausible roles, that of third body is advocated, in which the reaction…

Astrophysics of Galaxies · Physics 2023-03-01 Stefano Ferrero , Stefano Pantaleone , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

We investigated interaction between hydrogen molecules and bare as well as functionalized single-wall carbon nanotubes (SWNT) using first-principles plane wave method. We found that the binding energy of the H$_{2}$ physisorbed on the bare…

Materials Science · Physics 2009-11-11 S. Dag , Y. Ozturk , S. Ciraci , T. Yildirim

An electrical method is used to study the early stages of coalescence of two low-viscosity drops. A drop of aqueous NaCl solution is suspended in air above a second drop of the same solution which is grown until the drops touch. At that…

Soft Condensed Matter · Physics 2009-11-13 Sarah C. Case

Glycerol acts as a natural cryoprotectant by depressing the temperature of ice nucleation and slowing down the dynamics of water mixtures. In this work we characterize dynamics -- diffusion, viscosity, and hydrogen-bond dynamics -- as well…

Isothermal-isobaric molecular dynamics simulations are used to examine the microscopic structure and other properties of a model solution consisting of NaCl salt dissolved in water-methanol mixture. The SPC/E water model and the united atom…

Soft Condensed Matter · Physics 2018-06-27 M. Cruz Sanchez , J. Gujt , S. Sokolowski , O. Pizio