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Cavity polaritonics is capturing the imagination of the chemistry community because of the novel opportunities it creates to direct chemistry. Electron transfer (ET) reactions are among the simplest reactions, and they also underpin…

Quantum Physics · Physics 2022-08-12 Sutirtha N. Chowdhury , Peng Zhang , David N. Beratan

We consider a simple cubic array of metallic nanoparticles supporting extended collective plasmons that arise from the near-field dipolar interaction between localized surface plasmons in each nanoparticle. We develop a fully analytical…

Mesoscale and Nanoscale Physics · Physics 2015-01-12 Guillaume Weick , Eros Mariani

Surface plasmon polaritons (plasmons) are a combination of light and a collective oscillation of the free electron plasma at metal-dielectric interfaces. This interaction allows sub-wavelength confinement of light, beyond the diffraction…

Mesoscale and Nanoscale Physics · Physics 2013-09-27 Reinier W. Heeres , Leo P. Kouwenhoven , Valery Zwiller

There is an increasing scientific and technological interest on the design and implementation of nanoscale sources of quantum light. Here, we investigate the quantum statistics of the light scattered from a plasmonic nanocavity coupled to a…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 R. Sáez-Blázquez , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

We study dynamics of the interaction between two weak light beams mediated by a strongly coupled quantum dot-photonic crystal cavity system. First, we perform all optical switching of a weak continuous-wave signal with a pulsed control…

Quantum Physics · Physics 2012-03-06 Dirk Englund , Arka Majumdar , Michal Bajcsy , Andrei Faraon , Pierre Petroff , Jelena vuckovic

We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…

Quantum Physics · Physics 2024-02-28 Q. Zhang , M. Asjad , M. Reitz , C. Sommer , B. Gurlek , C. Genes

Quantized nano-objects offer a myriad of exciting possibilities for manipulating electrons and light that impact photonics, nanoelectronics, and quantum information. In this context, ultrashort laser pulses combined with nanotips and field…

Engineering strong interactions between optical photons is a great challenge for quantum science. Envisioned applications range from the realization of photonic gates for quantum information processing to synthesis of photonic quantum…

Mesoscale and Nanoscale Physics · Physics 2019-11-26 Patrick Knüppel , Sylvain Ravets , Martin Kroner , Stefan Fält , Werner Wegscheider , Atac Imamoglu

We experimentally demonstrate the coupling of far-field light to highly confined plasmonic gap modes via connected nanoantennas. The excitation of plasmonic gap modes is shown to depend on the polarization, position and wavelength of the…

Polariton chemistry has been hailed as a potential new route to direct molecular processes with electromagnetic fields. To make further strides, it is essential for the community to clarify which unusual polaritonic phenomena are true…

Chemical Physics · Physics 2025-11-19 Alexander M. McKillop , Marissa L. Weichman

The ability to engineer localized surface plasmon resonances at large scale usually relies on precise nanoscale patterning. Here, we demonstrate that mid-infrared plasmonic responses can instead emerge in unpatterned polysilicon films…

We theoretically investigate the quantum scattering of a single-photon pulse interacting with an ensemble of $\Lambda$-type three-level atoms coupled to a one-dimensional waveguide. With an effective non-Hermitian Hamiltonian, we study the…

Quantum Physics · Physics 2017-11-08 Guo-Zhu Song , Ewan Munro , Wei Nie , Fu-Guo Deng , Guo-Jian Yang , Leong-Chuan Kwek

We demonstrate the existence of new nonclassical correlations in the radiation of two atoms, which are coherently driven by a continuous laser source. The photon-photon-correlations of the fluorescence light show a spatial interferene…

Quantum Physics · Physics 2015-01-15 C. Skornia , J. von Zanthier , G. S. Agarwal , E. Werner , H. Walther

Interactions between light and matter play an instrumental role in many fields of science, giving rise to important applications in spectroscopy, sensing, quantum information processing, and lasers. In most of these applications, light is…

Optics · Physics 2023-03-22 Nicholas Rivera , Ido Kaminer

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou

Interactions between particles in quantum many-body systems play a crucial role in determining the electric, magnetic, optical, and thermal properties of the system. The recent progress in the laser-pulse technique has enabled the…

Strongly Correlated Electrons · Physics 2021-09-07 Nguyen Thanh Phuc , Pham Quang Trung

Polaritonic states, which arise from strong coupling between light and matter, show great promise in modifying chemical reactivity. However, reproducible enhancement of chemical reactions with polaritons is challenging due to a lack of…

Chemical Physics · Physics 2025-01-14 Shahzad Alam , Yicheng Liu , Russell J. Holmes , Renee R. Frontiera

When mid-infrared light interacts with nanoscale polar dielectric structures optical phonon propagation cannot be ignored, leading to a rich nonlocal phenomenology which we have only recently started to uncover. In properly crafted…

Mesoscale and Nanoscale Physics · Physics 2021-08-10 Christopher R. Gubbin , Simone De Liberato

Out of equilibrium, the action-reaction symmetry of the interactions is often broken, leading to the emergence of various collective phenomena with no equilibrium counterparts. Although ubiquitous in classical active systems, implementing…

Strongly Correlated Electrons · Physics 2025-09-22 Ryo Hanai , Daiki Ootsuki , Rina Tazai

Quantum path interferences occur whenever multiple equivalent and coherent transitions result in a common final state. Such interferences strongly modify the probability of a particle to be found in that final state, a key concept of…

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