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Realizing nonlinear coupling across space can enable new scientific and technological advances, including ultrafast operation and propagation of information in IR photonic circuitry, remote triggering or catalyzing of chemical reactions,…

Optics · Physics 2019-12-13 Jiaxi Wang , Bo Xiang , Wei Xiong

Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group…

Chemical Physics · Physics 2023-10-18 Zeyu Zhou , Hsing-Ta Chen , Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

Investigating the interaction of electron beams with materials and light has been a field of research since more than a century. The field was advanced theoretically by the raise of quantum mechanics and technically by the introduction of…

Optics · Physics 2017-10-11 Nahid Talebi

Polaritonic chemistry has ushered in new avenues for controlling molecular dynamics. However, two key questions remain: (i) Can classical light sources elicit the same effects as certain quantum light sources on molecular systems? (ii) Can…

Quantum Physics · Physics 2023-12-13 Leonardo F. Calderón , Humberto Triviño , Leonardo A. Pachón

Recently, the concept of strong light-matter coupling has been demonstrated in semiconductor structures, and it is poised to revolutionize the design and implementation of components, including solid state lasers and detectors. We…

Cavity quantum electrodynamics provides an ideal platform to engineer and control light-matter interactions with polariton quasiparticles. In this work, we investigate collective phenomena in a system of many particles in a harmonic trap…

Quantum Physics · Physics 2023-06-21 V. Rokaj , S. I. Mistakidis , H. R. Sadeghpour

We introduce and theoretically analyze a scheme to prepare and detect non-Gaussian quantum states of an optically levitated particle via the interaction with a light pulse that generates cubic and inverted potentials. We show that this…

We observe energy-dependent angle-resolved diffraction patterns in protons from strong-field dissociation of the molecular hydrogen ion H$_2^+$. The interference is a characteristic of dissociation around a laser-induced conical…

Atomic and Molecular Clusters · Physics 2016-04-11 Adi Natan , Matthew R Ware , Vaibhav S. Prabhudesai , Uri Lev , Barry D. Bruner , Oded Heber , Philip H Bucksbaum

Conical intersections (CI) between molecular potential energy surfaces with non-vanishing non-adiabatic couplings generally occur in any molecule consisting of at least three atoms. They play a fundamental role in describing the molecular…

Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…

Chemical Physics · Physics 2024-04-11 Nikolay V. Golubev , Jiří Vaníček

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…

Exciton-polaritons generated by light-induced potentials can spontaneously condense into macroscopic quantum states that display nontrivial spatial and temporal density modulation. While these patterns and their dynamics can be reproduced…

Mesoscale and Nanoscale Physics · Physics 2013-11-20 Li Ge , Ani Nersisyan , Baris Oztop , Hakan E. Tureci

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this…

The direct interaction of nuclei with super-intense laser fields is studied. We show that present and upcoming high-frequency laser facilities, especially together with a moderate acceleration of the target nuclei, do allow for resonant…

Nuclear Theory · Physics 2009-11-11 Thomas J. Buervenich , Joerg Evers , Christoph H. Keitel

Nonadiabatic effects are ubiquitous in physics, chemistry and biology. They are strongly amplified by conical intersections (CIs) which are degeneracies between electronic states of triatomic or larger molecules. A few years ago it has been…

Atomic and Molecular Clusters · Physics 2014-11-25 Gábor J. Halász , Ágnes Vibók , Lorenz S. Cederbaum

We find and analyze the exact time-dependent potential energy surface driving the proton motion for a model of cavity-induced suppression of proton-coupled electron-transfer. We show how, in contrast to the polaritonic surfaces, its…

Chemical Physics · Physics 2019-08-28 Lionel Lacombe , Norah M. Hoffmann , Neepa T. Maitra

Nanoscale quantum dots in microwave cavities can be used as a laboratory for exploring electron-electron interactions and their spin in the presence of quantized light and a magnetic field. We show how a simple theoretical model of this…

Mesoscale and Nanoscale Physics · Physics 2023-11-16 S. S. Beltrán-Romero , F. J. Rodríguez , L. Quiroga , N. F. Johnson

We review the design, theory, and applications of two dimensional periodic lattices hosting conical intersections in their energy-momentum spectrum. The best known example is the Dirac cone, where propagation is governed by an effective…

Optics · Physics 2016-06-01 Daniel Leykam , Anton S. Desyatnikov

Recent experiments have demonstrated strong light-matter coupling between electromagnetic nanoresonators and pristine sheets of two-dimensional semiconductors, and it has been speculated whether these systems can enter the quantum regime…

Quantum Physics · Physics 2022-02-23 E. V. Denning , M. Wubs , N. Stenger , J. Mork , P. T. Kristensen

Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced…

Quantum Physics · Physics 2021-12-22 Artur Skljarow , Harald Kübler , Charles S. Adams , Tilman Pfau , Robert Löw , Hadiseh Alaeian