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Silicon (Si) anodes attract a lot of research attention for their potential to enable high energy density lithium-ion batteries (LIBs). Many studies focus on nanostructured Si anodes to counteract deterioration. In this work, we model LIBs…

Chemical Physics · Physics 2024-04-23 Franziska Kilchert , Max Schammer , Arnulf Latz , Birger Horstmann

Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

Numerical Analysis · Mathematics 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

This paper presents a novel diffuse-interface electrochemical model that simultaneously simulates the evolution of the metallic negative electrode and interfacial voids during the stripping and plating processes in solid-state batteries.…

Materials Science · Physics 2024-12-24 Sourav Chatterjee , Michael Tonks , William Gardner , Marina Sessim

In mathematical models of lithium-ion batteries, the highly heterogeneous porous electrodes are frequently approximated as comprising spherical particles of uniform size, leading to the commonly-used single-particle model (SPM) when…

Applied Physics · Physics 2020-06-24 Toby L. Kirk , Jack Evans , Colin P. Please , S. Jonathan Chapman

In this work, a stochastic, physics-based model for Lithium-ion batteries (LIBs) is presented in order to study the effects of parametric model uncertainties on the cell capacity, voltage, and concentrations. To this end, the proposed…

Computational Physics · Physics 2015-09-17 Mohammad Hadigol , Kurt Maute , Alireza Doostan

Core-shell electrode particles are a promising morphology control strategy for high-performance lithium-ion batteries. However, experimental observations reveal that these structures remain prone to mechanical failure, with shell fractures…

Computational Engineering, Finance, and Science · Computer Science 2025-11-14 Y. Tu , B. Wu , E. Martínez-Pañeda

Renewable energy is critical for combating climate change, whose first step is the storage of electricity generated from renewable energy sources. Li-ion batteries are a popular kind of storage units. Their continuous usage through…

Methodology · Statistics 2024-11-05 Youngjin Cho , Quyen Do , Pang Du , Yili Hong

Redox flow batteries (RFBs) have gained popularity as large-scale energy storage systems for wind and solar powered grids. Modern RFB systems are based on highly corrosive and/or flammable electrolytes. Organic redox active species for RFBs…

Materials Science · Physics 2021-06-22 Rohan Borah , Fraser R Hughson , Thomas Nann

Redox Flow Batteries are a promising option for large-scale stationary energy storage. The vanadium redox flow battery is the most widely commercialized system thanks to its chemical stability and performance. This work aims to optimize the…

Optimization and Control · Mathematics 2023-01-04 Diana Cremoncini , Guido Francesco Frate , Aldo Bischi , Lorenzo Ferrari

It is of great importance to develop inorganic solid electrolytes with high ionic conductivity, thus enabling solid state Li-ion batteries to address the notorious safety issue about the current technology due to use of highly flammable…

Chemical Physics · Physics 2017-07-17 Zhuo Wang , Min Jie Xuan , Hong Jie Xu , Guosheng Shao

Next-generation high-energy-density batteries require ideally stable metal anodes, for which smooth metal deposits during battery recharging are considered a sign of interfacial stability that can ensure high efficiency and long cycle life.…

Materials Science · Physics 2022-01-11 Bingyuan Ma , Peng Bai

Here we report fabrication of flexible and stretchable battery composed of strain free LiFePO4 cathode, Li4Ti5O10 anode and a solid poly ethylene oxide (PEO) electrolyte as a separator layer. The battery is developed in a view of smart…

Materials Science · Physics 2015-03-13 Yang Liu , Maksim Skorobogatiy

The first and most important purpose of the current research work is to investigate the effects that different battery types have on the optimal configuration of photovoltaic (PV) and battery systems, from both economic and resilience…

Signal Processing · Electrical Eng. & Systems 2019-02-01 Stamatis Tsianikas , Jian Zhou , Nooshin Yousefi , David W. Coit

The increasing relevance of energy storage technologies demands high-capacity cathode materials for Li-ion batteries. Recently, Li-rich defect anti-fluorite Li$_5$FeO$_4$ has emerged as a high-capacity cathode material exhibiting…

Materials Science · Physics 2022-06-24 Anu Maria Augustine , Vishnu Sudarsanan , P. Ravindran

All solid state Li-ion batteries employing metallic lithium as an anode offer higher energy densities while also being safer than conventional liquid electrolyte based Li-ion batteries. However, the growth of tiny filaments of lithium…

Applied Physics · Physics 2020-01-20 Vikalp Raj , Varun R Kankanallu , Bibhatsu Kuiri , Naga Phani B Aetukuri

An appropriate description of the lithiation/delithiation dynamics in bi-phasic primary cathode particles of Li-ion batteries requires an accurate treatment of the conditions holding at the interface between the particle and the surrounding…

Materials Science · Physics 2024-11-01 Ahmed Yousfi , Arnaud Demortière , Guillaume Boussinot

The complex electrochemical behavior of lithium-ion batteries results in non-linear dynamics and appropriate modeling of this non-linear dynamical system is of interest for better management and control. In this work, we proposed a family…

Systems and Control · Electrical Eng. & Systems 2026-02-25 Khalid Mahmud Labib , Shabbir Ahmed

An important objective of designing lithium-ion rechargeable battery cells is to maximize their rate performance without compromising the energy density, which is mainly achieved through computationally expensive numerical simulations at…

Materials Science · Physics 2020-05-05 Fan Wang , Ming Tang

Lithium-ion batteries (LIBs) have found wide applications in a variety of fields such as electrified transportation, stationary storage and portable electronics devices. A battery management system (BMS) is critical to ensure the…

Systems and Control · Electrical Eng. & Systems 2024-02-02 Yiming Xu , Xiaohua Ge , Ruohan Guo , Weixiang Shen

A safe lithium-sulfur (Li-S) battery employs a composite polymer electrolyte based on a poly(ethylene glycol) dimethyl ether (PEGDME) solid at room temperature. The electrolyte membrane enables a stable and reversible Li-S electrochemical…

Applied Physics · Physics 2021-10-27 Vittorio Marangon , Daniele Di Lecce , Luca Minnetti , Jusef Hassoun