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Comptonization is the process in which photon spectrum changes due to multiple Compton scatterings in the electronic plasma. It plays an important role in the spectral formation of astrophysical X-ray and gamma-ray sources. There are…

Computational Physics · Physics 2009-10-30 Xin-Min Hua

The characterization of the electronic structure and chemical states of gases, solids, and liquids can be effectively performed using ambient pressure X-ray photoelectron spectroscopy (AP-XPS). However, the acquisition of electronic and…

Chemical Physics · Physics 2025-03-17 Yang Gu , Zhehao Qiu , Shui Lin , Yong Han , Hui Zhang , Zhi Liu , Jun Cai

Phase-shaped electron energy-loss spectroscopy (PSEELS) measures the scattering probability of structured free electron beams by a target. Over the last decade, it was shown that this scheme can be employed to emulate polarized optical…

Optics · Physics 2024-11-19 Simon Garrigou , Hugo Lourenço-Martins

We have developed a simulation-based method of spectral analysis for pile-up affected data of X-ray CCDs without any loss of photon statistics. As effects of the photon pile-up appear as complicated nonlinear detector responses, we employ a…

Instrumentation and Methods for Astrophysics · Physics 2022-03-14 Tsubasa Tamba , Hirokazu Odaka , Aya Bamba , Hiroshi Murakami , Koji Mori , Kiyoshi Hayashida , Yukikatsu Terada , Tsunefumi Mizuno , Masayoshi Nobukawa

Polarization dependence has historically seen extensive use in x-ray spectroscopy to determine magnetic and local geometric properties, but more broadly as a way to gain extra sensitivity to electronic structure at the level of individual…

The lateral resolution of an X-ray photoelectron spectroscopy instrument, which is equipped with a focused X-ray beam, is limited by the nominal X-ray beam diameter and the long tail intensity distri-bution of the X-ray beam. The long tail…

Instrumentation and Detectors · Physics 2020-12-21 Uwe Scheithauer

Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…

Instrumentation and Detectors · Physics 2020-05-06 Yanwen Sun , Mike Dunne , Paul Fuoss , Taito Osaka , Aymeric Robert , Mark Sutton , Makina Yabashi , Diling Zhu

We have studied the Stark effect in the soft x-ray region for various small molecules by calculating the field-dependent x-ray absorption spectra. This effect is explained in terms of the response of molecular orbitals (core and valence),…

Chemical Physics · Physics 2025-03-26 Avdhoot Datar , Catherine Wright , Devin A. Matthews

In this work we present a modification to conventional X-rays fluorescence using electrons as excitation source, and compare it with the traditional X-ray excitation for the study of pigments. For this purpose we have constructed a…

Instrumentation and Detectors · Physics 2016-08-24 F. Valle Brozas , A. Crego , L. Roso , A. Peralta Conde

Advances in the ability to manipulate free electron phase profiles within the electron microscope have spurred development of quantum-mechanical descriptions of electron energy loss (EEL) processes involving transitions between phase-shaped…

Mesoscale and Nanoscale Physics · Physics 2024-02-09 Marc R. Bourgeois , Austin G. Nixon , Matthieu Chalifour , David J. Masiello

In this work, we report on modelling results obtained with our recently developed simulation tool enabling nanoscopic description of electronic processes in X-ray irradiated ferromagnetic materials. With this tool, we have studied the…

We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…

Materials Science · Physics 2021-05-05 Dino Novko , Vito Despoja , Marcel Reutzel , Andi Li , Hrvoje Petek , Branko Gumhalter

X-ray near-field speckle-based phase-sensing approaches provide efficient means to characterise optical elements. Here, we present a theoretical review of several of these speckle methods in the frame of optical characterisation and provide…

Synchrotron based photoemission electron microscopy with energy filter combines real space imaging with microprobe diffraction ($\mu$-ARPES), giving access to the local electronic structure of laterally inhomogeneous materials. We present…

Mesoscale and Nanoscale Physics · Physics 2013-01-01 Tevfik Onur Menteş , Andrea Locatelli

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

Digital array orthogonal transformations that can be presented as a decomposition over basis items or basis images are considered. The orthogonal transform provides digital data scattering, a process of pixel energy redistributing, that is…

Multimedia · Computer Science 2019-01-24 V. N. Gorbachev , L. A. Denisov , E. M. Kaynarova , I. K. Metelev , E. S. Yakovleva

X-ray binaries hosting a compact object have been among the main targets of the Imaging X-ray Polarimetry Explorer (IXPE) since its launch, due to their high brightness in the 2-8 keV energy band. The spectropolarimetric analysis performed…

High Energy Astrophysical Phenomena · Physics 2024-01-30 R. Farinelli , A. Waghmare , L. Ducci , A. Santangelo

The application of PhotoEmission Electron Microscopy (PEEM) and Low Energy Electron Microscopy (LEEM) techniques to the study of the electronic and chemical structure of ferroelectric materials is reviewed. Electron optics in both…

X-ray absorption spectroscopy yields direct access to the electronic and geometric structure of hybrid inorganic-organic interfaces formed upon adsorption of complex molecules at metal surfaces. The unambiguous interpretation of…

Chemical Physics · Physics 2017-06-19 Katharina Diller , Reinhard J. Maurer , Moritz Müller , Karsten Reuter

Imaging structures at the molecular level is a fast developing interdisciplinary research field that spans across the boundaries of physics and chemistry. High spatial resolution images of molecules can be obtained with photons or ultrafast…

Atomic Physics · Physics 2016-09-01 R. Puthumpally-Joseph , J. Viau-Trudel , M. Peters , T. T. Nguyen-Dang , O. Atabek , E. Charron