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Properties of iron oxides at the extreme conditions are of essential importance in condensed matter physics and Geophysics. The recent discovery of a new type of iron oxide, Fe4O5, at high pressure and high temperature of Earth's deep…

Strongly Correlated Electrons · Physics 2021-09-14 Aiqin Yang , Qiaoying Qin , Xiangru Tao , Shengli Zhang , Yongtao Zhao , Peng Zhang

The archetypal $3d$ Mott insulator hematite, Fe$_2$O$_3$, is one of the basic oxide components playing an important role in mineralogy of Earth's lower mantle. Its high pressure-temperature behavior, such as the electronic properties,…

Strongly Correlated Electrons · Physics 2019-10-07 I. Leonov , G. Kh. Rozenberg , I. A. Abrikosov

Electronic structure and magnetic properties of Fe$_3$Se$_4$ are calculated using the density functional approach. Due to the metallic properties, magnetic moments of the iron atoms in two nonequivalent positions in the unit cell are…

Materials Science · Physics 2022-07-05 L. V. Begunovich , M. M. Korshunov , S. G. Ovchinnikov

The magnetic and electronic structures of Fe4O5 have been investigated at ambient and high pressures via a combination of representation analysis, density functional theory (DFT+U) calculations, and M\"ossbauer spectroscopy. A few spin…

Materials Science · Physics 2023-01-10 V. S. Zhandun , N. V. Kazak , I. Kupenko , D. M. Vasiukov , X. Li , E. Blackburn , S. G. Ovchinnikov

The electronic structures of four Laves phase iron compounds (e.g. YFe$_2$, ZrFe$_2$, LuFe$_2$ and HfFe$_2$) have been calculated by the state-of-the-art full potential electronic structure code. The magnetic moments collapse under…

Materials Science · Physics 2015-12-08 Wenxu Zhang , Wanli Zhang

We provide experimental and theoretical evidence for a novel type of pressure-induced insulator-metal transition characterized by site-selective delocalization of the electrons. M\"ossbauer spectroscopy, X-ray diffraction and electrical…

Strongly Correlated Electrons · Physics 2018-09-19 E. Greenberg , I. Leonov , S. Layek , Z. Konopkova , M. P. Pasternak , L. Dubrovinsky , R. Jeanloz , I. A. Abrikosov , G. Kh. Rozenberg

We present density functional theory calculations for low-$T_c$ metallic ferromagnet La$_5$Co$_2$Ge$_3$ at ambient and applied pressures. Our investigations reveal that the system is a quasi-one-dimensional ferromagnet with a peculiar…

Strongly Correlated Electrons · Physics 2026-01-13 Giuseppe Cuono , Carmine Autieri , Marcin M. Wysokiński

We compute the electronic structure, spin and charge state of Fe ions, and structural phase stability of paramagnetic CaFeO$_3$ under pressure using a fully self-consistent in charge density DFT+dynamical mean-field theory method. We show…

Strongly Correlated Electrons · Physics 2022-02-01 I. Leonov

We consider electronic correlation effects and their impact on magnetic properties of tetragonally distorted chemically ordered FeCo alloys (L1$_0$ structure) being a promising candidate for rare-earth-free permanent magnets. We employ a…

Strongly Correlated Electrons · Physics 2022-06-02 A. S. Belozerov , A. A. Katanin , V. I. Anisimov

Iron oxide is a key compound to understand the state of the deep Earth. It has been believed that previously known oxides such as FeO and Fe2O3 will be dominant at the mantle conditions. However, recent observation of FeO2 shed another…

Strongly Correlated Electrons · Physics 2017-03-01 Bo Gyu Jang , Duck Young Kim , Ji Hoon Shim

Iron-bearing oxides undergo a series of pressure-induced electronic, spin and structural transitions that can cause seismic anomalies and dynamic instabilities in Earth's mantle and outer core. We employ x-ray diffraction and x-ray emission…

Strongly Correlated Electrons · Physics 2023-07-10 E. Greenberg , R. Nazarov , A. Landa , J. Ying , R. Q. Hood , B. Hen , R. Jeanloz , V. B. Prakapenka , V. V. Struzhkin , G. Kh. Rozenberg , I. Leonov

The electronic and magnetic properties of recently discovered new important constituent of the Earth's lower mantle FeO2H were investigated by means of the density functional theory combined with the dynamical mean field theory (DFT+DMFT).…

Strongly Correlated Electrons · Physics 2018-11-07 Alexey O. Shorikov , Alexander I. Poteryaev , Vladimir I. Anisimov , Sergey V. Streltsov

The magnets are typically classified into Stoner and Heisenberg type, depending on the itinerant or localized nature of the constituent magnetic moments. In this work, we investigate theoretically the behaviour of the magnetic moments of…

We report a detail theoretical study of the electronic structure and phase stability of transition metal oxides MnO, FeO, CoO, and NiO in their paramagnetic cubic B1 structure by employing dynamical mean-field theory of correlated electrons…

Strongly Correlated Electrons · Physics 2016-10-26 I. Leonov , L. Pourovskii , A. Georges , I. A. Abrikosov

We investigate the effect of external pressure on the Fe magnetic moment in undoped LaOFeAs within the framework of density functional theory and show that this system is close to a magnetic instability: The Fe moment is found to drop by…

Superconductivity · Physics 2009-01-22 I. Opahle , H. C. Kandpal , Y. Zhang , C. Gros , R. Valenti

The effect of local environment on the formation of magnetic moments on Fe atoms in iron silicides are studied by combination of ab initio and model calculations. The suggested model includes all Fe d- and Si p-orbitals, intra-atomic…

Materials Science · Physics 2016-07-13 N. G. Zamkova , V. S. Zhandun , S. G. Ovchinnikov , I. S. Sandalov

We report the discovery of a new allotrope of iron by first principles calculations. This phase has $Pmn2_1$ symmetry, a six-atom unit cell (hence the name Fe$_6$), and the highest magnetization density (M$_s$) among all known crystalline…

We study the electronic and magnetic properties of monolayer Fe$_3$GeTe$_2$ within the DFT+DMFT approach in the paramagnetic phase. We argue that this compound is sufficiently far from the local magnetic moment limit, demonstrating…

Strongly Correlated Electrons · Physics 2026-03-13 A. A. Katanin , A. N. Rudenko , D. I. Badrtdinov , M. I. Katsnelson

We report on a density functional theory study demonstrating the coexistence of weak ferromagnetism and antiferroelectricity in boron-deficient MgB6. A boron vacancy produces an almost one dimensional extended molecular orbital, which is…

Materials Science · Physics 2012-03-09 Igor Popov , Nadjib Baadji , Stefano Sanvito
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