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We present the observation of an isostructural Mott insulator-metal transition in van-der-Waals honeycomb antiferromagnet V$_{0.9}$PS$_3$ through high-pressure x-ray diffraction and transport measurements. The MPX$_3$ family of magnetic…

Strongly Correlated Electrons · Physics 2019-03-27 M. J. Coak , S. Son , D. Daisenberger , H. Hamidov , C. R. S. Haines , P. L. Alireza , A. R. Wildes , C. Liu , S. S. Saxena , J. -G. Park

Metal-to-insulator transitions (MIT) can be driven by a number of different mechanisms, each resulting in a different type of insulator -- Change in chemical potential can induce a transition from a metal to a band insulator; strong…

Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work…

Strongly Correlated Electrons · Physics 2019-01-02 C. R. S. Haines , M. J. Coak , G. I. Lampronti , C. Liu , H. Hamidov , A. R. Wildes , D. Daisenberger , P. Nahai-Williamson , S. S. Saxena

The metal-insulator transition in VO2 was investigated using the three-band Hubbard model, in which the degeneracy of the 3d orbitals, the on-site Coulomb and exchange interactions, and the effects of lattice distortion were considered. A…

Condensed Matter · Physics 2009-11-10 Arata Tanaka

Technology moves towards ever faster switching between different electronic and magnetic states of matter. Manipulating properties at terahertz rates requires accessing the intrinsic timescales of electrons (femtoseconds) and associated…

We observe an insulator-to-metal (I-M) transition in crystalline silicon doped with sulfur to non- equilibrium concentrations using ion implantation followed by pulsed laser melting and rapid resolidification. This I-M transition is due to…

Materials Science · Physics 2015-05-27 Mark T. Winkler , Daniel Recht , Meng-Ju Sher , Aurore J. Said , Eric Mazur , Michael J. Aziz

Transition metal dichalcogenide superlattices provide an exciting new platform for exploring and understanding a variety of phases of matter. The moir\'e continuum Hamiltonian, of two-dimensional jellium in a modulating potential, provides…

Strongly Correlated Electrons · Physics 2024-02-16 Yubo Yang , Miguel Morales , Shiwei Zhang

Recently, the pressure has been used as external stimuli to induce structural and magnetic phase transitions in many layered quantum materials whose layers are linked by van der Waals forces. Such materials with weakly held layers allow…

Dynamic control of conductivity and optical properties via atomic structure changes is of tremendous technological importance in information storage. Energy consumption considerations provide a driving force toward employing thin materials…

Materials Science · Physics 2016-02-16 Yao Li , Karel-Alexander N. Duerloo , Kerry Wauson , Evan J. Reed

To elucidate the pressure evolution of the electronic structure in an antiferromagnetic dimer-Mott (DM) insulator ${\beta}^{\prime}$-(BEDT-TTF)$_2$ICl$_2$, which exhibits superconductivity at 14.2 K under 8 GPa, we measured the polarized…

Strongly Correlated Electrons · Physics 2015-09-01 K. Hashimoto , R. Kobayashi , H. Okamura , H. Taniguchi , Y. Ikemoto , T. Moriwaki , S. Iguchi , M. Naka , S. Ishihara , T. Sasaki

The results of magnetic and spectral properties calculation for paramagnetic phase of ferropericlase (Fe$_{1/4}$Mg$_{3/4}$)O at ambient and high pressures are reported. Calculations were performed by combined Local Density Approximation +…

Materials Science · Physics 2014-11-21 N. A. Skorikov , A. O. Shorikov , S. L. Skornyakov , M. A. Korotin

Pump-probe experiments with femtosecond time resolution allow to disentangle the electronic dynamics from the lattice response and thus provide valuable insights into the non-equilibrium behavior of correlated materials. In Cr-doped…

Strongly Correlated Electrons · Physics 2024-07-15 Jiyu Chen , Francesco Petocchi , Viktor Christiansson , Philipp Werner

Observations are reported of a metal-insulator transition in a 2D hole gas in asymmetrically doped strained SiGe quantum wells. The metallic phase, which appears at low temperatures in these high mobility samples, is characterised by a…

Strongly Correlated Electrons · Physics 2009-10-30 P. T. Coleridge , R. L. Williams , Y. Feng , P. Zawadzki

We systematically study the effect of high pressure on the structure, electronic structure and transport properties of 2H-MoS$_2$, based on first-principles density functional calculations and the Boltzmann transport theory. Our calculation…

Materials Science · Physics 2013-09-18 Huaihong Guo , Teng Yang , Peng Tao , Yong Wang , Zhidong Zhang

We investigate the metal-insulator Mott transition in a generalized version of the periodic Anderson model, in which a band of itinerant electrons is hybridrized with a narrow and strongly correlated band. Using dynamical mean-field theory,…

Strongly Correlated Electrons · Physics 2017-07-18 Adriano Amaricci , Luca de' Medici , Massimo Capone

The ground state of the Hubbard model is studied within the single-site approximation (SSA) and beyond the SSA. Within the SSA, the ground state is a typical Mott insulator at the critical point n=1 and U/W=+infty, with n being the electron…

Strongly Correlated Electrons · Physics 2007-05-23 Fusayoshi J. Ohkawa

In this article, a brief introduction is first given on infrared studies of materials at high pressures using a diamond anvil cell. Then, our recent results of high-pressure infrared studies are described for Mg$_2$Si, InAs, and InSb. For…

The Mott metal-insulator transition-a drastic manifestations of Coulomb interactions among electrons-is the first-order transition of clear discontinuity, as shown by various experiments and the celebrated dynamical mean-field theory.…

Strongly Correlated Electrons · Physics 2018-03-01 Tetsuya Furukawa , Kazuhiko Kobashi , Yosuke Kurosaki , Kazuya Miyagawa , Kazushi Kanoda

We present results of combined density functional theory plus dynamical mean-field theory (DFT+DMFT) calculations, which show that the Mott insulator LaTiO3 undergoes an insulator-to-metal transition under compressive epitaxial strain of…

Strongly Correlated Electrons · Physics 2014-04-17 Krzysztof Dymkowski , Claude Ederer

In ReS$_2$ a layer-independent direct band-gap of 1.5 eV implies a potential for its use in optoelectronic applications. ReS$_2$ crystallizes in the 1T$^{\prime}$-structure which leads to anisotropic physical properties and whose…