Related papers: Quantum Dynamics with Electronic Friction
The present paper is based upon equations obtained in an earlier paper by the author devoted to a new formulation of quantum electrodynamics. The equations describe the structure of the electron as well as its motion in external fields,…
The exact nuclear time-dependent potential energy surface arises from the exact decomposition of electronic and nuclear motion, recently presented in [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys. Rev. Lett. 105, 123002 (2010)]. Such…
Friction is usually a very complicated process. It appears in its most elementary form when two flat surfaces separated by vacuum gap are sliding relative to each other at zero Kelvin and the friction is generated by the relative movement…
Electronic coherences are key to understanding and controlling photo-induced molecular transformations. We identify a crucial quantum-mechanical feature of electron-nuclear correlation, the projected nuclear quantum momenta, essential to…
The Exact Factorization (XF) of molecular wavefunctions can be viewed as an 'electronic wavepacket' framework for quantum dynamics. It is an appealing alternative to the conventional non-adiabatic dynamics, unfolding in the space of coupled…
A quantum analog of friction (understood as a completely positive, Markovian, translation-invariant and phenomenological model of dissipation) is known to be in odds with the detailed balance in the thermodynamic limit. We show that this is…
The processes of radiation damping and decoherence in Quantum Electrodynamics are studied from an open system's point of view. Employing functional techniques of field theory, the degrees of freedom of the radiation field are eliminated to…
A first-principles treatment of the vibrational dynamics of molecular chemisorbates on metal surfaces is presented. It is shown that the mean field quantum evolution of the vibrational position operator is determined by a quantum Langevin…
In quantum electrodynamics, the quantitatively most successful theory in the history of science, intercharge forces obeying the inverse square law are due to the exchange of space-like virtual photons. The fundamental quantum process…
Molecular motion at metallic surfaces is affected by nonadiabatic effects and electron-phonon coupling. The ensuing energy dissipation and dynamical steering effects are not captured by classical molecular dynamics simulations, but can be…
This work builds on the following result of a previous article (quant-ph/0509044): the matter field can be naturally eliminated from the equations of the scalar electrodynamics (the Klein-Gordon-Maxwell electrodynamics) in the unitary…
Friction at water-carbon interfaces remains a major puzzle with theories and simulations unable to explain experimental trends in nanoscale waterflow. A recent theoretical framework -- quantum friction (QF)-- proposes to resolve these…
We derive a quantum master equation from first principles to describe friction in one dimensional, collisional Brownian motion. We are the first to avoid an ill-defined square of the Dirac delta function by using localized wave packets…
We derive a quantum kinetic theory for QED based on Kadanoff-Baym equations for Wigner functions. By assuming parity invariance and considering a complete set of self-energy diagrams, we find the resulting kinetic theory expanded to lowest…
The interaction between freely propagating electrons and light waves is typically described using an approximation in which we assume that the electron velocity remains approximately the same during the interaction. In this article we…
Electron gases in metals are described as quantum charged Newtonian viscous fluids experiencing Ohmic Darcy friction on the solid lattice ions as well. The dispersion relation of the electron acoustic waves is derived, which shows the…
The Brownian motion of a light quantum particle in a heavy classical gas is theoretically described and a new expression for the friction coefficient is obtained for arbitrary temperature. At zero temperature it equals to the de Broglie…
A relativistic quantum mechanical model to describe the quantum FEL dynamics has been developed. Neglecting the spin of electrons in the impacting beam, this model is based on the Klein-Gordon equation coupled to the Poisson equation for…
In the electron dynamics in quantum matter, the Berry curvature of the electronic wave function provides the artificial magnetic field (AMF) in momentum space, which leads to non-trivial contributions to transport coefficients. It is known…
We present an approach for carrying out non-adiabatic molecular dynamics simulations of systems in which non-adiabatic transitions arise from the coupling between the classical atomic motions and a quasi-continuum of electronic quantum…