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Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

We study single-photon ionization of aligned H$_2^+$ in low-intensity near-circular laser fields with lower photon energy numerically and analytically. The photoelectron momentum distribution (PMD) within the laser polarization plane,…

Atomic Physics · Physics 2025-05-13 Z. Y. Chen , S. Q. Shen , M. Q. Liu , J. Y. Che , Y. J. Chen

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

Atomic and Molecular Clusters · Physics 2015-05-20 C. -H. Zhang , U. Thumm

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

Atomic Physics · Physics 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

A versatile semiclassical approximation for intense laser-atom processes is presented. This uniform approximation is no more complicated than the frequently-used multi-dimensional saddle-point approximation and far superior, since it…

Atomic Physics · Physics 2016-09-08 C. Figueira de Morisson Faria , H. Schomerus , W. Becker

Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…

Ionization of an atom or molecule presents surprising richness beyond our current understanding: strong-field ionization with low-frequency fields recently revealed unexpected kinetic energy structures (1, 2). A solid grasp on electron…

The calculation of partial two-photon ionization cross sections in the above-threshold energy region is discussed in the framework of exterior complex scaling. It is shown that with a minor modification of the usual procedure, which is…

Atomic Physics · Physics 2018-08-17 Andrej Mihelič

We use a quantum trajectory-based semi-classical method to account for Coulomb interaction between the photoelectron and the parent ion in the classically forbidden, sub-barrier region during strong-field tunneling ionization processes. We…

Atomic Physics · Physics 2017-11-21 Tian-Min Yan , D. Bauer

The exact delay-zero calibration in an attosecond pump-probe experiment is important for the correct interpretation of experimental data. In attosecond transient absorption spectroscopy the determination of the delay-zero exclusively from…

We study ionization of atoms in strong elliptically-polarized laser fields. We focus on the physical origin of the offset angle in the photoelectron momentum distribution and its possible relation to a specific time. By developing a model…

Atomic Physics · Physics 2022-12-12 Y. G. Peng , J. Y. Che , C. Chen , G. G. Xin , Y. J. Chen

We present a study of multiphoton dissociative ionization from molecules. By solving the time-dependent Schr\"{o}dinger equation for H$_2^+$ and projecting the solution onto double continuum scattering states, we observe the correlated…

Atomic Physics · Physics 2012-07-03 C B Madsen , F Anis , L B Madsen , B D Esry

This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…

Optics · Physics 2026-01-14 Oren Cohen

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800~nm) 27~fs laser pulse. For intensities ranging from the tunneling to the over-the-barrier regime, we identify…

Atomic Physics · Physics 2011-01-27 A. Emmanouilidou , D. S. Tchitchekova

Tunneling and over-barrier ionization are the primary processes of strong-field ionization of atoms and molecules. While the dynamics of tunneling ionization have been extensively studied, exploration of over-barrier ionization dynamics has…

Atomic Physics · Physics 2025-09-03 Yongzhe Ma , Qingcao Liu , Hongcheng Ni , Jian Wu

A unitary model describing the electronic transitions in an atom subject to a strong high frequency laser pulse is proposed. The model fully accounts for the initial state coupling with the continuum spectrum. Continuum-continuum as well as…

Atomic Physics · Physics 2016-05-10 M. G. Bustamante , V. D. Rodríguez

The time-dependent electromagnetic field can results both pair waves and pair particles. It can be for mathematical relations between two functions with identical argument and difference of phases equal to $\pi$. Two examples both the…

Atomic Physics · Physics 2007-05-23 Evgueni V. Kovarski

Determination and interpretation of Wigner-like photoionisation delays is one of the most active fields of attosecond science. Previous results have suggested that large photoionisation delays are associated with structured continua, but a…

Atomic Physics · Physics 2024-10-14 Jia-Bao Ji , Anatoli S. Kheifets , Meng Han , Kiyoshi Ueda , Hans Jakob Wörner

Study on ionization process of molecules in an intense infrared laser field is of paramount interest in strong-field physics and constitutes the foundation of imaging of molecular valence orbitals and attosecond science. We show measurement…

How quanta of energy and charge are transported on both atomic spatial and ultrafast time scales is at the heart of modern technology. Recent progress in ultrafast spectroscopy has allowed us to directly study the dynamical response of an…

Other Condensed Matter · Physics 2015-04-28 R. Locher , L. Castiglioni , M. Lucchini , M. Greif , L. Gallmann , J. Osterwalder , M. Hengsberger , U. Keller