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Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

We present a semiclassical two-step model for strong-field ionization that accounts for path interferences of tunnel-ionized electrons in the ionic potential beyond perturbation theory. Within the framework of a classical trajectory…

Within a semiclassical description of above-threshold ionization (ATI) we identify the interplay between intracycle and intercycle interferences. The former is imprinted as a modulation envelope on the discrete multiphoton peaks formed by…

Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…

Atomic Physics · Physics 2007-12-11 P. Johnsson , J. Mauritsson , T. Remetter , A. LHuillier , K. J. Schafer

We investigate the feasibility of using high-harmonic generation (HHG) as a complementary probe of tunneling delay in strong-field ionization. By combining time--frequency analysis of HHG spectra obtained from full time-dependent…

Atomic Physics · Physics 2026-01-15 Amol R. Holkundkar

Over the last three decades numerous numerical methods for solving the time-dependent Schr\"{o}dinger equation within the single-active electron approximation have been developed for studying ionization of atomic targets exposed to an…

Atomic Physics · Physics 2020-08-12 B. Fetić , W. Becker , D. B. Milošević

We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and neutral particles with permanent dipole moments. Interference is studied when electrons or atomic…

Quantum Physics · Physics 2009-11-11 Fernando C. Lombardo , Paula I. Villar

We observe the phase space trajectory of an entangled wave packet of a trapped ion with high precision. The application of a spin dependent light force on a superposition of spin states allows for coherent splitting of the matter wave…

Quantum Physics · Physics 2014-05-22 Ulrich Poschinger , Andreas Walther , Kilian Singer , Ferdinand Schmidt-Kaler

This paper has been prepared by the Symphony collaboration (University of Warsaw, Uniwersytet Jagiello\'nski, DESY/CNR and ICFO) on the occasion of the 25th anniversary of the "simple man's models" which underlie most of the phenomena that…

The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent…

Quantum Physics · Physics 2017-09-13 Guennaddi K. Paramonov , Andre D. Bandrauk , Oliver Kühn

Attosecond streaking, as a measurement technique, was originally conceived as a means to characterize attosecond light pulses, which is a good approximation if the relevant transition matrix elements are approximately constant within the…

Atomic Physics · Physics 2015-05-19 Vladislav S. Yakovlev , Justin Gagnon , Nicholas Karpowicz , Ferenc Krausz

Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…

Optics · Physics 2023-02-22 H. Y. Kim , M. Garg , S. Mandal , L. Seiffert , T. Fennel , E. Goulielmakis

We present ionization probability and line shape calculations for the two-step 3-photon ionization process, $1S \stackrel{2\hbar \omega}{\longrightarrow}2S \stackrel{\hbar \omega}{\longrightarrow}\epsilon P $, of the ground state of…

Atomic Physics · Physics 2016-08-15 V Yakhontov , R. Santra , K. Jungmann

Quantum calculations of tunneling in strong-field ionization (SFI) predict intricate momentum distributions due to sub-laser-cycle attosecond electron dynamics. These are obscured in most experiments by the dominance of inter-cycle…

Atomic Physics · Physics 2021-06-03 Nicholas Werby , Adi Natan , Ruaridh Forbes , Philip Bucksbaum

Shape resonances in physics and chemistry arise from the spatial confinement of a particle by a potential barrier. In molecular photoionization, these barriers prevent the electron from escaping instantaneously, so that nuclei may move and…

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with…

Atomic Physics · Physics 2014-03-28 Wei-Chun Chu , Toru Morishita , C. D. Lin