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We provide a comprehensive theory of magnetic phases in two-dimensional triangulene crystals, using both Hubbard model and density functional theory (DFT) calculations. We consider centrosymmetric and non-centrosymmetric triangulene…

Mesoscale and Nanoscale Physics · Physics 2024-11-01 G. Catarina , J. C. G. Henriques , A. Molina-Sánchez , A. T. Costa , J. Fernández-Rossier

Owing to the presence of strong static correlation effects, accurate prediction of the electronic properties (e.g., the singlet-triplet energy gaps, vertical ionization potentials, vertical electron affinities, fundamental gaps, symmetrized…

Chemical Physics · Physics 2016-11-18 Chun-Shian Wu , Pei-Yin Lee , Jeng-Da Chai

We investigate magnetic properties of CrTe$_2$ within the density functional theory (DFT) approach in ferromagnetic phase and combination of DFT and dynamical mean field theory (DFT+DMFT) approach in paramagnetic phase. We show that few…

Strongly Correlated Electrons · Physics 2026-03-03 A. A. Katanin , E. M. Agapov

Using density functional theory with added on-site interactions (DFT+U), we study the electronic structure of bulk, monolayer, and bilayer of the layered transition-metal dichalcogenide $1T-TaS_2$. We show that a two-dimensional…

Materials Science · Physics 2015-06-18 Pierre Darancet , Andrew J. Millis , Chris A. Marianetti

We employ density functional theory to study in detail the crystallization of super-paramagnetic particles in two dimensions under the influence of an external magnetic field that lies perpendicular to the confining plane. The field induces…

Soft Condensed Matter · Physics 2009-11-13 Sven van Teeffelen , Hartmut Löwen , Christos N. Likos

We consider a system of particles interacting via a purely repulsive, soft-core potential recently introduced to model effective pair interactions between dendrimers, which is expected to lead to the formation of crystals with multiple…

Soft Condensed Matter · Physics 2015-05-11 Davide Pini

Magnetic order in most materials occurs when magnetic ions with finite moments in a crystalline lattice arrange in a particular pattern below the ordering temperature determined by exchange interactions between the ions. However, when the…

We study the magnetic phases of two coupled two-dimensional electron gases in order to determine under what circumstances these phases may occur in real semiconductor quantum wells and what the experimental properties of the broken-symmetry…

Condensed Matter · Physics 2007-05-23 P. I. Tamborenea , R. J. Radtke , S. Das Sarma

Periodic and cluster density-functional theory (DFT) calculations, including DFT+U and hybrid functionals, are applied to study magnetostructural correlations in spin-1/2 frustrated chain compounds CuX2: CuCl2, CuBr2, and a fictitious chain…

Strongly Correlated Electrons · Physics 2013-07-02 S. Lebernegg , M. Schmitt , A. A. Tsirlin , O. Janson , H. Rosner

The correlation between structural distortion and emergence of magnetism in graphene containing a single vacancy was investigated using first-principles calculations based on density functional theory (DFT). Our results have shown that a…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Wendel S. Paz , Wanderlã L. Scopel , Jair C. C. Freitas

For more than a century, electricity and magnetism have been believed to always exhibit inextricable link due to the symmetry in electromagnetism. At the interface, polar groups that have polar charges, are indispensable to be considered,…

Soft Condensed Matter · Physics 2022-05-13 Jihong Wang , Yizhou Yang , Jie Jiang , Liuhua Mu , Guosheng Shi , Yongshun Song , Haijun Yang , Peng Xiu , Liang Chen , Haiping Fang

Rare-earth (RE) atoms on top of 2D materials represent an interesting platform with the prospect of tailoring the magnetic anisotropy for practical applications. Here, we investigate the ground state and magnetic properties of selected…

Mesoscale and Nanoscale Physics · Physics 2024-07-25 Johanna P. Carbone , Juba Bouaziz , Gustav Bihlmayer , Stefan Blügel

Based on classical density functional theory (DFT), we investigate the demixing phase transition of a two-dimensional, binary Heisenberg fluid mixture. The particles in the mixture are modeled as Gaussian soft spheres, where one component…

Soft Condensed Matter · Physics 2012-08-31 K. Lichtner , A. J. Archer , S. H. L. Klapp

In this paper, we examine the properties of spin-polarized interfaces consisting of single-molecule magnet bis(cyclopentadienyl)cobalt(II) (cobaltocene) and two-dimensional magnetic materials, semiconducting CrI$_3$ and metallic…

Materials Science · Physics 2026-03-23 Nikola Machacova , Biplab Sanyal

Large-spin two-dimensional magnets are generally expected to develop conventional long-range order once the dominant exchange scale becomes appreciable. The layered spin-$3/2$ maple-leaf compound Na$_2$Mn$_3$O$_7$ defies this expectation:…

Strongly Correlated Electrons · Physics 2026-02-27 Hari Borutta , Tobias Müller , Ronny Thomale , Harald O. Jeschke , Yasir Iqbal

An analytical and numerical study of the one-dimensional double and super-exchange model is presented. A phase separation between ferromagnetic and anti-ferromagnetic phases occurs at low super-exchange interaction energy. When the…

Strongly Correlated Electrons · Physics 2015-06-18 E. Vallejo , F. López-Urías , O. Navarro , M. Avignon

We study crystal melting in two-dimensional antiferromagnets, by analyzing the statistical mechanics of the six-state clock model on a lattice in which defects (dislocations and disclinations) are allowed to appear. We show that the…

Statistical Mechanics · Physics 2018-01-26 Itamar Shamai , Daniel Podolsky

Atomically-thin magnetic crystals have been recently isolated experimentally, greatly expanding the family of two-dimensional materials. In this Article we present an extensive comparative analysis of the electronic and magnetic properties…

Strongly Correlated Electrons · Physics 2019-09-06 Guido Menichetti , Matteo Calandra , Marco Polini

We present systematic quantitative description of the magnetoconductance of the split-gate quantum wires. Accounting for the exchange and correlation interactions within the spin density function theory (DFT) leads to the lifting of the…

Mesoscale and Nanoscale Physics · Physics 2009-05-26 I. V. Zozoulenko , S. Ihnatsenko

The electronic structure of Cu hexafluoroacetylacetonate, crystallized with a stable nitronyl nitroxide radical [Ovcharenko et al., Russ. Chem. Bull. 53, 2406 (2004)], is calculated from first principles within the density functional theory…

Materials Science · Physics 2007-05-23 A. V. Postnikov , A. V. Galakhov , S. Bluegel
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