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In this paper we explore the capabilities of MoS2 and WS2 2D monolayers to produce radiation in the terahertz range by generation of high-order harmonics. This phenomenon, which is a result of the non-linear response of the electronic…

Applied Physics · Physics 2024-02-13 Jose Manuel Iglesias , Elena Pascual , Maria J. Martin , Raul Rengel

Many chemical systems cannot be described by quantum chemistry methods based on a singlereference wave function. Accurate predictions of energetic and spectroscopic properties require a delicate balance between describing the most important…

Chemical Physics · Physics 2018-06-12 Erik Donovan Hedegård , Julien Toulouse , Hans Jørgen Aagaard Jensen

The semiconducting p-n junction is a simple device structure with great relevance for electronic and optoelectronic applications. The successful integration of low-dimensional materials in electronic circuits has opened the way forward for…

Various methods going beyond density-functional theory (DFT), such as DFT+U, hybrid functionals, meta-GGAs, GW, and DFT-embedded dynamical mean field theory (eDMFT), have been developed to describe the electronic structure of correlated…

Strongly Correlated Electrons · Physics 2020-07-16 Subhasish Mandal , Kristjan Haule , Karin M. Rabe , David Vanderbilt

Two-dimensional heterostructure of WSe2/MoS2 atomic layers has unique piezoelectric characteristics which depends on the number of atomic layer, stacking type, and interlayer interaction size. The van der Waals heterostructure of p- and…

Mesoscale and Nanoscale Physics · Physics 2019-12-13 Sheng Yu , Tikaram Neupane , Dulitha Jayakodige , Zhuo Yang

Topological phase transitions in condensed matter systems have shown extremely rich physics, unveiling such exotic states of matter as topological insulators, superconductors and superfluids. Photonic topological systems open a whole new…

Previous works have controversially claimed near-room temperature ferromagnetism in two-dimensional (2D) VSe$_2$, with conflicting results throughout the literature. These discrepancies in magnetic properties between both phases (T and H…

Strongly Correlated Electrons · Physics 2023-07-28 Daniel Wines , Juha Tiihonen , Kayahan Saritas , Jaron Krogel , Can Ataca

Excellent gate electrostatics in field effect transistors (FETs) based on two-dimensional transition metal dichalcogenide (2D TMD) channels can dramatically decrease static power dissipation. Energy efficient FETs operate in enhancement…

Doped transition-metal dichalcogenides monolayers exhibit exciting magnetic properties for the benefit of two-dimensional spintronic devices. Using density functional theory (DFT) incorporating Hubbard-type of correction (DFT$+U$) to…

Materials Science · Physics 2021-05-12 Adlen Smiri , Sihem Jaziri , Samir Lounis , Iann C. Gerber

Piezoelectricity appears in the inversion asymmetric crystal that converts mechanical deformational force to electricity. Two-dimensional transition metal dichalcolgenide (TMDC) monolayers exhibit the piezoelectric effect due to the…

Applied Physics · Physics 2019-12-13 Sheng Yu , Quinton Rice , Tikaram Neupane , Bagher Tabibi , Felix Jaetae Seo

Atomic-scale control of light-matter interactions represent the ultimate frontier for many applications in photonics and quantum technology. Two-dimensional semiconductors, including transition metal dichalcogenides, are a promising…

Mesoscale and Nanoscale Physics · Physics 2024-08-22 John M. Woods , Saroj B. Chand , Enrique Mejia , Takashi Taniguchi , Kenji Watanabe , Johannes Flick , Gabriele Grosso

Plane-wave electronic-structure predictions based upon orbital-dependent density-functional theory (OD-DFT) approximations, such as hybrid density-functional methods and self-interaction density-functional corrections, are severely affected…

Materials Science · Physics 2011-10-19 Yanli Li , Ismaila Dabo

We introduce the unification of dynamical mean field theory (DMFT) and linear-scaling density functional theory (DFT), as recently implemented in ONETEP, a linear-scaling DFT package, and TOSCAM, a DMFT toolbox. This code can account for…

Strongly Correlated Electrons · Physics 2020-05-04 Edward B. Linscott , Daniel J. Cole , Nicholas D. M. Hine , Michael C. Payne , Cédric Weber

In this work we provide an exact and efficient numerical approach to simulate multi-time correlation functions in the Mahan-Nozi\`{e}res-De Dominicis model, which crudely mimics the spectral properties of doped two-dimensional…

Mesoscale and Nanoscale Physics · Physics 2022-06-07 Lachlan P Lindoy , Yao-Wen Chang , David R Reichman

Two-dimensional (2D) layered nanomaterials heterostructures, arising from the combination of 2D materials with other low-dimensional species, feature large surface area to volume ratio, which provides a high density of active sites for…

Materials Science · Physics 2025-02-19 Mengjiao Wang , Michal Langer , Roberto Altieri , Matteo Crisci , Silvio Osella , Teresa Gatti

In this paper, we have done a comparative study of electronic and magnetic properties of iron phthalocyanine (FePc) and cobalt phthalocyanine (CoPc) molecules physisorbed on monolayer of MoS$_2$ and graphene by using density functional…

Materials Science · Physics 2018-09-05 Soumyajyoti Haldar , Sumanta Bhandary , Hakkim Vovusha , Biplab Sanyal

Under temperature or pressure tuning, tetragonal EuPd$_2$Si$_2$ is known to undergo a valence transition from nearly divalent to nearly trivalent Eu accompanied by a volume reduction. Albeit intensive work, its microscopic origin is still…

Strongly Correlated Electrons · Physics 2023-02-24 Young-Joon Song , Susanne Schulz , Kristin Kliemt , Cornelius Krellner , Roser Valentí

The accurate resolution of the chemical properties of strongly correlated systems, such as biradicals, requires the use of electronic structure theories that account for both multi-reference as well as dynamic correlation effects. A variety…

Chemical Physics · Physics 2023-01-03 Jan-Niklas Boyn , David A. Mazziotti

This study presents a comprehensive investigation of hybrid interfaces formed by monolayer MoS$_2$ coupled with the organic molecules perylene (P), perylene diimide (PDI), and perylene orange (PO). Using density functional theory, we…

Materials Science · Physics 2025-09-01 Mohammed El Amine Miloudi , Oliver Kühn

Two-dimensional transition metal dichalcogenides (TMDs) offer tunable optical and electronic properties, making them highly promising for next-generation optoelectronic devices. One effective approach to engineering these properties is…

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