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The van der Waals ferromagnet (FM), VI$_3$, was studied by muon spin relaxation ($\mu^+$SR) and first principle calculations based on density functional theory (DFT). Temperature dependent zero field muon spin relaxation ($\mu^+$SR)…

Strongly Correlated Electrons · Physics 2022-11-01 Ola Kenji Forslund , Yuqing Ge , Hiroto Ohta , Chennan Wang , Mahmoud Abdel-Hafiez , Jun Sugiyama , Martin Månsson , Yasmine Sassa

The discovery of ordered magnetism in two-dimensional van der Waals materials at the monolayer limit challenges the Mermin-Wagner theorem, which forbids spontaneous breaking of continuous symmetries in two dimensions at finite temperatures.…

Two-dimensional (2D) layered magnetic materials are generating a great amount of interest for the next generation of electronic devices thanks to their remarkable properties associated to spin dynamics. The recently discovered layered…

Van der Waals materials provide a versatile toolbox for the emergence of new quantum phenomena and the fabrication of functional heterostructures. Among them, the trihalide VI3 stands out for its unique magnetic and structural landscape.…

Materials Science · Physics 2024-02-07 A. De Vita , R. Sant , V. Polewczyk , G. van der Laan , N. B. Brookes , T. Kong , R. J. Cava , G. Rossi , G. Vinai , G. Panaccione

Layered van-der-Waals 2D magnetic materials are of great interest in fundamental condensed-matter physics research, as well as for potential applications in spintronics and device physics. We present neutron powder diffraction data using…

We present a combined study of zero-field $^{51}$V and $^{127}$I NMR at ambient pressure and specific heat and magnetization measurements under pressure up to 2.08 GPa on bulk single crystals of the van-der-Waals ferromagnet VI$_3$. At…

Strongly Correlated Electrons · Physics 2019-11-21 Elena Gati , Yuji Inagaki , Tai Kong , Robert J. Cava , Yuji Furukawa , Paul C. Canfield , Sergey L. Bud'ko

We report the magnetic structure and electronic properties of the honeycomb antiferromagnet $\rm NaNi_2BiO_{5.66}$. We find magnetic order with moments along the $c$ axis for temperatures below $T_{c1}=6.3(1)\>{\rm K}$ and then in the…

Strongly Correlated Electrons · Physics 2019-12-25 A. Scheie , K. Ross , P. Peter Stavropoulos , E. Seibel , J. A. Rodriguez-Rivera , J. A. Tang , Yi Li , Hae-Young Kee , R. J. Cava , C. Broholm

We use the synergy of infrared, terahertz, and Raman spectroscopies with DFT calculations to shed light on the magnetic and lattice properties of VI3. The structural transition at TS1 = 79 K is accompanied by a large splitting of polar…

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

We report a comprehensive investigation of the lattice and magnetic structure in van der Waals antiferromagnet VBr3, characterized by a BiI3-type structure at room temperature. Neutron diffraction experiments were performed on both…

Strongly Correlated Electrons · Physics 2024-08-06 Yimeng Gu , Yiqing Hao , Zeyu Kao , Yiqing Gu , Feiyang Liu , Shiyi Zheng , Huibo Cao , Lunhua He , Jun Zhao

Recently discovered ferromagnetism of the layered van der Waals material VI$_3$ attracts much research attention. Despite substantial progress,in the following important aspects no consensus has been reached: (i) a possible deviation of the…

Materials Science · Physics 2021-07-07 L. M. Sandratskii , K. Carva

VI$_{3}$ is a ferromagnet with planar honeycomb sheets of bonded V$^{3+}$ ions held together by van der Waals forces. We apply neutron spectroscopy to measure the two dimensional ($J/J_{c} \approx 17$) magnetic excitations in the…

Strongly Correlated Electrons · Physics 2021-07-23 H. Lane , E. Pachoud , J. A. Rodriguez-Rivera , M. Songvilay , G. Xu , P. M. Gehring , J. P. Attfield , R. A. Ewings , C. Stock

We present comprehensive measurements of the structural, magnetic and electronic properties of layered van-der-Waals ferromagnet VI$_3$ down to low temperatures. Despite belonging to a well studied family of transition metal trihalides,…

We report structural, physical properties and electronic structure of van der Waals (vdW) crystal VI3. Detailed analysis reveals that VI3 exhibits a structural transition from monoclinic C2/m to rhombohedral R-3 at Ts ~ 79 K, similar to…

Materials Science · Physics 2019-06-19 Shangjie Tian , Jian-Feng Zhang , Chenghe Li , Tianping Ying , Shiyan Li , Xiao Zhang , Kai Liu , Hechang Lei

Vanadium Sesquioxide (V$_2$O$_3$) is an antiferromagnetic insulator below $T_{\mathrm N}\approx$ 155 K. The magnetic order is not of C- or G-type as one would infer from the bipartite character of the hexagonal basal plane in the…

Materials Science · Physics 2015-08-19 Daniel Grieger , Michele Fabrizio

Recent years have seen a vast increase in research into van der Waals magnetic materials. In many of these systems, magnetism is introduced via light 3\textit{d}-transition metal elements, combined with chalcogenides or halogens. Despite…

VBr$_3$ is a van der Waals antiferromagnet below the N\'eel temperature of 26.5 K with a saturation moment of 1.2 mB/f.u. above the metamagnetic transitions detected in the in-plane and out-of-plane directions. To reveal the AFM structure…

Layered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI$_3$…

Materials Science · Physics 2020-01-15 Yu Liu , Milinda Abeykoon , C. Petrovic

Van der Waals (vdW) Dirac magnon system CrI$_3$, a potential host of topological edge magnons, orders ferromagnetically (FM) (T$_C=61$ K) in the bulk, but antiferromagnetic (AFM) order has been observed in nanometer thick flakes, attributed…

Materials Science · Physics 2024-05-14 John A. Schneeloch , Luke Daemen , Despina Louca

We report a magnetic and neutron diffraction study on the ground state magnetism and field evolution of single crystal van der Waals multiferroic CuCrP2S6. The ordered moments align along the b axis in the A-type antiferromagnetic…

Strongly Correlated Electrons · Physics 2026-03-30 Jiasen Guo , Ryan P. Siebenaller , Michael A. Susner , Jiaqiang Yan , Zachary Morgan , Feng Ye
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