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Static and dynamic structure factors of Heisenberg ferrimagnetic spin chains are numerically investigated. There exist two distinct branches of elementary excitations, which exhibit ferromagnetic and antiferromagnetic aspects. The…

Statistical Mechanics · Physics 2009-10-31 Shoji Yamamoto , Toru Sakai

Magnetic correlations of two iso-structural quasi-one-dimensional (1D) antiferromagnetic spin-chain compounds Sr$M_2$V$_2$O$_8$ ($M$ = Co, Mn) have been investigated by magnetization and powder neutron diffraction. Two different collinear…

Strongly Correlated Electrons · Physics 2014-12-17 A. K. Bera , B. Lake , W. -D. Stein , S. Zander

SrCr$_2$As$_2$ is an itinerant antiferromagnet in the same structural family as the SrFe$_2$As$_2$ high-temperature superconductors. We report our calculations of exchange-coupling parameters $J_{ij}$ for SrCr$_2$As$_2$ using a static…

The magnetic and thermodynamic properties of a new ferrimagnetic decorated spin-(1/2,1) Heisenberg chain with spin-1 pendant spins are investigated for three cases: (A) J1,J2>0; (B) J1>0, J2<0; and (C) J1<0, J2>0, where J1 and J2 are the…

Strongly Correlated Electrons · Physics 2010-06-23 Shou-Shu Gong , Wei Li , Yang Zhao , Gang Su

With the commutation relations of the spin operators, we first write out the equations of motion of the spin susceptibility and related correlation functions that have a hierarchical structure, then under the "soft cut-off" approximation,…

Strongly Correlated Electrons · Physics 2020-08-25 Yu-Liang Liu

We study the thermodynamics of the spin-$S$ two-dimensional quantum Heisenberg antiferromagnet on the square lattice with nearest ($J_1$) and next-nearest ($J_2$) neighbor couplings in its collinear phase ($J_2/J_1>0.5$), using the…

Strongly Correlated Electrons · Physics 2007-05-23 Luca Capriotti , Tommaso Roscilde , Andrea Fubini , Valerio Tognetti

We have carried out extensive series studies, at T=0 and at high temperatures, of 2-chain and 3-chain spin-half ladder systems with antiferromagnetic intrachain and both antiferromagnetic and ferromagnetic interchain couplings. Our results…

Condensed Matter · Physics 2009-10-28 J. Oitmaa , Rajiv R. P Singh , Zheng Weihong

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin

Deuteronium jarosite, (D_3O)Fe_3(SO_4)_2(OD)_6, contains a kagome lattice of Heisenberg spins, S=5/2, with a coverage of 97+-1%. DC and AC susceptibility measurements show strong in-plane antiferromagnetic exchange (\theta_CW=-1500+-300K)…

Condensed Matter · Physics 2007-05-23 A. S. Wills , A Harrison , S. A. M. Mentink , T. E. Mason , Z. Tun

We report synthesis and magnetic properties of quasi-one-dimensional spin-$\frac{1}{2}$ Heisenberg antiferromagnetic chain compound BaNa$_2$Cu(VO$_4$)$_2$. This orthovanadate has a centrosymmetric crystal structure, $C2/c$, where the…

Nuclear spins are known to experience spontaneous long-range correlations only below 2.5 mili-Kelvin in superfluid $^3$He. Here we present the first evidence of nuclear spin coupling in molecular hydrogen (H$_2$) at 74-92 Kelvin using…

Materials Science · Physics 2016-02-05 Raina J. Olsen , Jon W. Taylor , Cristian I. Contescu , James R. Morris

We report transport and inelastic neutron scattering studies on electronic properties and spin dynamics of the quasi-one-dimensional spin chain antiferromagnet RbFeS$_2$. An antiferromagnetic phase transition at $T_N\approx195$ K and…

Strongly Correlated Electrons · Physics 2021-12-24 Lisi Li , Liangliang Zheng , Benjamin A. Frandsen , Andrew D. Christianson , Dao-Xin Yao , Meng Wang , Robert J. Birgeneau

Sr$_2$CuWO$_6$ is a double perovskite proposed to be at the border between two and three dimensional magnetism, with a square lattice of $S=\frac{1}{2}$ Cu$^{2+}$ ions. We have used inelastic neutron scattering to investigate the spin wave…

Strongly Correlated Electrons · Physics 2016-08-24 H. C. Walker , O. Mustonen , S. Vasala , D. T. Adroja , M. Karppinen

Large single crystals of the new compound SrMn$_2$V$_2$O$_8$ have been grown by the floating-zone method. This transition-metal based oxide is isostructural to SrNi$_2$V$_2$O$_8$, described by the tetragonal space group $I4_1cd$. Magnetic…

Strongly Correlated Electrons · Physics 2011-07-28 Sandra K. Niesen , Oliver Heyer , Thomas Lorenz , Martin Valldor

We have investigated the magnetic diffuse scattering of isostructural $S$ = 5/2 fcc antiferromagnets Ba$_2$MnTeO$_6$ and Ba$_2$MnWO$_6$ using polarized neutrons. Both materials display short-range correlated magnetism above their respective…

To understand spin interactions in materials of the Cu$_2$Sb structure type, inelastic neutron scattering of Fe$_2$As single crystals was examined at different temperatures and incident neutron energies. The experimental phonon spectra…

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

Accurate ab initio calculations on embedded Cu_4O_{12} square clusters, fragments of the La_2CuO_4 lattice, confirm a value of the nearest neighbor antiferromagnetic coupling (J=124 meV) previously obtained from ab initio calculations on…

Strongly Correlated Electrons · Physics 2009-10-31 Carmen J. Calzado , Jean-Paul Malrieu

Exact diagonalization calculations of finite antiferromagnetic spin-1 Heisenberg chains at finite temperatures are presented and compared to a recent inelastic neutron scattering experiment for temperatures T up to 7.5 times the intrachain…

Strongly Correlated Electrons · Physics 2009-11-07 M. Kenzelmann , P. Santini

Neutron spectroscopy and diffuse neutron scattering on herbertsmithite [ZnCu3 (OH)6Cl2], a near-ideal realisation of the s = 1/2 kagome antiferromagnet, reveal the hallmark property of a quantum spin liquid; instantaneous short-ranged…

Strongly Correlated Electrons · Physics 2009-12-21 M. A. de Vries , J. R. Stewart , P. P. Deen , J. O. Piatek , G. J. Nilsen , H. M. Ronnow , A. Harrison