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Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

Materials Science · Physics 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

SrCuTe$_2$O$_6$ consists of a 3-dimensional arrangement of spin-$\frac{1}{2}$ Cu$^{2+}$ ions. The 1st, 2nd and 3rd neighbor interactions respectively couple Cu$^{2+}$ moments into a network of isolated triangles, a highly frustrated…

Strongly Correlated Electrons · Physics 2021-01-04 S. Chillal , A. T. M. N Islam , H. Luetkens , E. Canévet , Y. Skourski , D. Khalyavin , B. Lake

X-ray diffraction, thermodynamic measurements, and density-functional band-structure calculations are used to study the magnetic behavior of BaCuTe$_{2}$O$_{6}$, a member of the $A$CuTe$_2$O$_6$ structural family that hosts complex…

Materials Science · Physics 2021-04-21 P. Bag , N. Ahmed , Vikram Singh , M. Sahoo , A. A. Tsirlin , R. Nath

We report a neutron scattering study of the long-wavelength dynamic spin correlations in the model two-dimensional $S=1/2$ square lattice Heisenberg antiferromagnets Sr$_2$CuO$_2$Cl$_2$ and Sr$_2$Cu$_3$O$_4$Cl$_2$. The characteristic energy…

Strongly Correlated Electrons · Physics 2009-10-31 Y. J. Kim , R. J. Birgeneau , F. C. Chou , R. W. Erwin , M. A. Kastner

The magnetic excitation spectrum and Hamiltonian of the quantum magnet BaCuTe2O6 is studied by inelastic neutron scattering (INS) and density functional theory (DFT). INS on powder and single crystal samples reveals overlapping spinon…

Strongly Correlated Electrons · Physics 2023-05-19 A. Samartzis , S. Chillal , H. O. Jeschke , D. J. Voneshen , Z. Lu , A. T. M. N. Islam , B. Lake

We compute the magnetic susceptibility and specific heat of the spin-1/2 Heisenberg model on the kagome lattice with high-temperature expansions and exact diagonalizations. We compare the results with the experimental data on ZnCu3(OH)6Cl2…

Strongly Correlated Electrons · Physics 2011-11-09 Gregoire Misguich , Philippe Sindzingre

Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…

Strongly Correlated Electrons · Physics 2007-11-14 V. O. Garlea , A. Zheludev , L. -P. Regnault , J. -H. Chung , Y. Qiu , M. Boehm , K. Habicht , M. Meissner

This study examines the increasing complexity in the magnetic properties of small $n$ = 3, 4, 5, 6 spin-1/2 quantum rings. Using an exact diagonalization of the isotropic Heisenberg Hamiltonian with nearest and next-nearest neighbor…

Materials Science · Physics 2016-09-21 J. T. Haraldsen

The magnetic structure of the double perovskite compound Sr$_2$CuTeO$_6$ was determined from neutron powder diffraction data. This material is magnetically described as an $S\,{=}\,1/2$ quasi-two-dimensional square-lattice Heisenberg model…

Strongly Correlated Electrons · Physics 2016-03-09 Tomoyuki Koga , Nobuyuki Kurita , Maxim Avdeev , Sergey Danilkin , Taku J. Sato , Hidekazu Tanaka

We present a theoretical and experimental study of a quasi-one-dimensional zigzag antiferromagnet (N_2H_5)CuCl_3, which can be viewed as weakly coupled Heisenberg chains with a frustrated interaction. We first discuss generic features of…

Strongly Correlated Electrons · Physics 2009-11-07 N. Maeshima , M. Hagiwara , Y. Narumi , K. Kindo , T. C. Kobayashi , K. Okunishi

Motivated by the experimental realizations of nearly one-dimensional spin-1/2 Heisenberg model found in chain cuprates SrCuO$_2$ and Sr$_2$CuO$_3$, which remain in a quantum-critical Luttinger liquid state down to temperatures that are much…

Strongly Correlated Electrons · Physics 2016-08-31 A. M. Tsvelik , I. A. Zaliznyak

The electronic and magnetic properties of K$_{2}$CuP$_{2}$O$_{7}$ were investigated by means of susceptibility, specific heat and $^{31}$P nuclear magnetic resonance (NMR) measurements and by LDA band structure calculations. The temperature…

Strongly Correlated Electrons · Physics 2009-11-13 R. Nath , Deepa Kasinathan , H. Rosner , M. Baenitz , C. Geibel

The Heisenberg spin chain compound Sr3CuPtO6 is investigated by magnetic susceptibility and heat capacity measurements. Sr3CuPtO6 has an unconventional chain structure in the sense that i) the spin half copper atoms are arranged in a zigzag…

Strongly Correlated Electrons · Physics 2009-11-10 S. Majumdar , V. Hardy , M. R. Lees , D. McK. Paul , H. Rousseliere , D. Grebille

The spin 1/2 Heisenberg model on a square lattice with antiferromagnetic nearest- and next-nearest neighbour interactions (the $J_1$--$J_2$ model) has long been studied as a paradigm of a two-dimensional frustrated quantum magnet. Only very…

Strongly Correlated Electrons · Physics 2007-05-23 Nic Shannon , Burkhard Schmidt , Karlo Penc , Peter Thalmeier

The double-perovskite compounds Sr$_2$CuTeO$_6$ and Sr$_2$CuWO$_6$ are magnetically described as quasi-two-dimensional spin-1/2 square-lattice $J_1{-}J_2$ Heisenberg antiferromagnets with predominant $J_1$ and $J_2$ exchange interactions,…

Strongly Correlated Electrons · Physics 2018-09-10 Masari Watanabe , Nobuyuki Kurita , Hidekazu Tanaka , Wataru Ueno , Kazuki Matsui , Takayuki Goto

We have investigated the spin dynamics in the strongly correlated chain copper oxide SrCuO$_2$ for energies up to $\gtrsim 0.6$ eV using inelastic neutron scattering. We observe an acoustic band of magnetic excitations which is well…

Strongly Correlated Electrons · Physics 2010-07-28 I. A. Zaliznyak , H. Woo , T. G. Perring , C. L. Broholm , C. D. Frost , H. Takagi

Sr$_2$CuTeO$_6$ presents an opportunity for exploring low-dimensional magnetism on a square lattice of $S=1/2$ Cu$^{2+}$ ions. We employ ab initio multi-reference configuration interaction calculations to unravel the Cu$^{2+}$ electronic…

We report a neutron scattering study of the instantaneous spin correlations in the two-dimensional spin S=5/2 square-lattice Heisenberg antiferromagnet Rb_2MnF_4. The measured correlation lengths are quantitatively described, with no…

Strongly Correlated Electrons · Physics 2009-10-31 Y. S. Lee , M. Greven , B. O. Wells , R. J. Birgeneau , G. Shirane

We report inelastic neutron scattering studies of magnetic excitations in antiferromagnetically ordered SrFe$_{2}$As$_{2}$ ($T_{N}=220$ K), the parent compound of the FeAs-based superconductors. At low temperatures (T=7 K), the spectrum of…

We report detailed neutron scattering studies on Ba$_2$Cu$_3$O$_4$Cl$_2$. The compound consists of two interpenetrating sublattices of Cu, labeled as Cu$_{\rm A}$ and Cu$_{\rm B}$, each of which forms a square-lattice Heisenberg…

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