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Most elemental metals under ambient conditions adopt simple structures such as BCC, FCC and HCP in specific groupings across the Periodic Table, and on compression, many of these elements undergo transitions to surprisingly complex…

Materials Science · Physics 2022-06-27 Yuanhui Sun , Lei Zhao , Chris J. Pickard , Russell J. Hemley , Yonghao Zheng , Maosheng Miao

Organic semiconductors have attracted increasing interest as thermoelectric converters in recent years due to their intrinsically low thermal conductivity compared to inorganic materials. This boom has led to encouraging practical results,…

Materials Science · Physics 2021-03-08 Dorothea Scheunemann , Martijn Kemerink

Thermoelectric materials, which can convert waste heat into electricity or act as solid-state Peltier coolers, are emerging as key technologies to address global energy shortages and environmental sustainability. However, discovering…

Applied Physics · Physics 2024-03-12 Kaidong Song , A. N. M. Tanvir , Md Omarsany Bappy , Yanliang Zhang

Understanding heat transport in organic semiconductors is of fundamental and practical relevance. Therefore, we study the lattice thermal conductivities of a series of (oligo)acenes, where an increasing number of rings per molecule leads to…

Materials Science · Physics 2024-12-09 Lukas Legenstein , Lukas Reicht , Sandro Wieser , Michele Simoncelli , Egbert Zojer

Chalcogenide perovskites provide a promising avenue for non-toxic, stable thermoelectric materials. Here, thermal transport and thermoelectric properties of BaZrS$_3$ as a typical orthorhombic perovskite are investigated. An extremely low…

Materials Science · Physics 2023-12-14 Yu Wu , Ying Chen , Qiaoqiao Li , Kui Xue , Hezhu Shao , Hao Zhang , Liujiang Zhou

Lattice thermal conductivities (LTC) for a subset of polymer crystals from the Polymer Genome Library were investigated to explore high LTC polymer systems. We employed a first-principles approach to evaluating phonon lifetimes within the…

Materials Science · Physics 2020-08-21 Keishu Utimula , Tom Ichibha , Ryo Maezono , Kenta Hongo

The lack of computationally inexpensive and accurate ab-initio based methodologies to predict lattice thermal conductivity, without computing the anharmonic force constants or time-consuming ab-initio molecular dynamics, is one of the…

Materials Science · Physics 2016-07-27 P. Nath , J. J. Plata , D. Usanmaz , C. Toher , M. Fornari , M. Buongiorno Nardelli , S. Curtarolo

We have studied the effects of phonon-boundary scattering on the thermal transport in topological Kondo insulator, SmB$_6$. The studies have been performed by using the $3\omega$ method in the temperature range 300K - 3K. We show that the…

Materials Science · Physics 2022-08-03 Narayan Poudel , Daniel J. Murray , Jason R. Jeffries , Krzysztof Gofryk

Phase change memory devices are typically reset by melt-quenching a material to radically lower its electrical conductance. The high power and concomitantly high current density required to reset phase change materials is the major issue…

A systematic analysis of low temperature magnetic phase diagrams of Ce compounds is performed in order to recognize the thermodynamic conditions to be fulfilled by those systems to reach a quantum critical regime and, alternatively, to…

Strongly Correlated Electrons · Physics 2015-06-04 Julian G. Sereni

PbTe, one of the most promising thermoelectric materials, has recently demonstrated thermoelectric figure of merit ($ZT$) of above 2.0 when alloyed with group II elements. The improvements are due mainly to significant reduction of lattice…

Materials Science · Physics 2018-05-04 Yi Xia , James M. Hodges , Mercouri G. Kanatzidis , Maria K. Y. Chan

In this paper we extend the classical method of lattice dynamics to defective crystals with partial symmetries. We start by a nominal defect configuration and first relax it statically. Having the static equilibrium configuration, we use a…

Materials Science · Physics 2010-04-28 Arash Yavari , Arzhang Angoshtari

Transport properties provide important information about the mobility, elastic and inelastic of scattering of excitations in solids. Heat transport is well understood for phonons and electrons, but little is known about heat transport by…

Strongly Correlated Electrons · Physics 2008-04-11 C. Hess

To synthesize a new superconductor which has a critical temperature, Tc, exceeding the room temperature, one needs to know what chemical components to start with. This chapter presents analysis of experimental data which allow one to draw a…

Superconductivity · Physics 2007-05-23 A. Mourachkine

The glassy thermal conductivities observed in crystalline inorganic perovskites such as Cs$_3$Bi$_2$I$_6$Cl$_3$ is perplexing and lacking theoretical explanations. Here, we first experimentally measure such its thermal transport behavior…

Materials Science · Physics 2024-12-23 Zezhu Zeng , Zheyong Fan , Michele Simoncelli , Chen Chen , Ting Liang , Yue Chen , Geoff Thornton , Bingqing Cheng

Thermoelectric materials, enabling direct waste-heat to electricity conversion, need to be highly electrically conducting while simultaneously thermally insulating. This is fundamentally challenging since electrical and thermal conduction…

Aiming at developing high thermal conductivity copper/diamond composite, an unconventional approach applying self-assembled monolayer (SAM) prior to the high-temperature sintering of copper/diamond composite was utilized to enhance the…

In silicon, lattice thermal conductivity plays an important role in a wide range of applications such as thermoelectric and microelectronic devices. Grain boundaries (GBs) in polycrystalline silicon can significantly reduce lattice thermal…

Computational Physics · Physics 2021-05-26 Susumu Fujii , Atsuto Seko

High lattice thermal conductivity in half-Heusler alloys has been the major bottleneck in thermoelectric applications. Disordered half-Heusler alloys could be a plausible alternative to this predicament. In this paper, utilizing…

Materials Science · Physics 2023-06-27 Mohd Zeeshan , Chandan Kumar Vishwakarma , B. K. Mani

Discovering new materials with ultrahigh thermal conductivity has been a critical research frontier and driven by many important technological applications ranging from thermal management to energy science. Here we have rigorously…

Materials Science · Physics 2021-04-19 Huan Wu , Hang Fan , Yongjie Hu