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We use the perturbed relativistic coupled-cluster theory to compute the static electric dipole polarizabilities of the singly ionized alkali atoms, namely, Na$^+$, $^+$, Rb$^+$, Cs$^+$ and Fr$^+$. The computations use the…

Atomic Physics · Physics 2013-05-01 S. Chattopadhyay , B. K. Mani , D. Angom

We present an implementation of relativistic ionization-potential (IP) equation-of-motion coupled-cluster (EOMCC) with up to 3-hole--2-particle (3h2p) excitations that makes use of the molecular mean-field exact two-component (mmfX2C)…

Chemical Physics · Physics 2025-01-10 Stephen H. Yuwono , Run R. Li , Tianyuan Zhang , Xiaosong Li , A. Eugene DePrince

We report a novel experimental technique for the comparison of ionization processes in ultrafast laser pulses irrespective of pulse ellipticity. Multiple ionization of xenon by 50 fs 790 nm, linearly and circularly polarized laser pulses is…

We study the effects of higher-order electronic correlations in the systems with particle-hole excited states using a relativistic hybrid method that combines configuration interaction and linearized coupled-cluster approaches. We find the…

Atomic Physics · Physics 2018-01-31 M. S. Safronova , U. I. Safronova , M. G. Kozlov

We employ four-component spinor relativistic equation-of-motion coupled-cluster (EOMCC) method within the single- and double- excitation approximation to calculate the single ionization potentials (IPs) and double ionization potentials…

Atomic Physics · Physics 2015-06-11 Himadri Pathak , B. K. Sahoo , Turbasu Sengupta , B. P. Das , Nayana Vaval , Sourav Pal

Ionization of highly charged relativistic ions by neutral atoms and ions is considered. Numerical results of recently developed computer codes based on the relativistic Born and the equivalent-photon approximations are presented. The…

Atomic Physics · Physics 2013-05-29 G. Baur , I. L. Beigman , V. P Shevelko , I. Yu. Tolstikhina , Th. Stoehlker

Analytic expressions are given for the baryonic, electric and strangeness chemical potentials which explicitly show the importance of various terms. Simple scaling relations connecting these chemical potentials are found. Applications to…

Nuclear Theory · Physics 2008-11-26 Aram Z. Mekjian

We have employed the relativistic coupled cluster theory to calculate the magnetic dipole and electric quadrupole hyperfine constants for the ground and low lying excited states of singly ionized magnesium. Comparison with experimental and…

Atomic Physics · Physics 2007-05-23 Chiranjib Sur , Bijaya K. Sahoo , Rajat K Chaudhuri , B. P. Das , D. Mukherjee

The effective potential of electron--electron interaction and the two-particle \textquotedblleft density--density\textquotedblright\ correlation function have been calculated for a simple semiinfinite metal making allowance for the…

Mesoscale and Nanoscale Physics · Physics 2015-03-29 B. M. Markovych , I. M. Zadvorniak

We revisited the electronic structure parameters used to interpret the hyperfine structure of neutral polonium. We used a computational scheme that treats relativistic and high-order electronic correlation effects within the coupled cluster…

Atomic Physics · Physics 2024-03-08 Leonid V. Skripnikov , Anatoly E. Barzakh

We have developed one electron detachment theory from a closed-shell atomic configuration in the relativistic Fock-space coupled-cluster ansatz. Using this method, we determine sensitivity coefficients to the variation of the fine structure…

Atomic Physics · Physics 2013-11-20 D. K. Nandy , B. K. Sahoo

Based on the many-body theory of metals in the third order of the perturbation expansion in electron-ion interaction pseudopotential, the potentials of pair and three-ion interactions are calculated in liquid lead, aluminium and beryllium…

Materials Science · Physics 2007-05-23 E. V. Vasiliu

Atomic polarization phenomena impinge upon a number of areas and processes in physics. The dielectric constant and refractive index of any gas are examples of macroscopic properties that are largely determined by the dipole polarizability.…

Atomic Physics · Physics 2015-05-18 J. Mitroy , M. S. Safronova , Charles W. Clark

We numerically study the magnetization of small metallic clusters. The magnetic susceptibility is enhanced for lower electronic densities due to the stronger influence of electron-electron interactions. The magnetic susceptibility…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Richard Berkovits

We present a theory of local electric polarization in crystalline solids and apply it to study the case of wurtzite group-III nitrides. We show that a local value of the electric polarization, evaluated at the atomic sites, can be cast in…

Materials Science · Physics 2013-12-06 Miguel A. Caro , Stefan Schulz , Eoin P. O'Reilly

The static dipole polarizabilities of group 11 elements (Cu, Ag, and Au) are computed using the relativistic coupled-cluster method with single, double, and perturbative triple excitations. Three types of relativistic effects on dipole…

Atomic Physics · Physics 2025-02-13 YingXing Cheng

Dramatically sharp resonances manifesting stable negative-ion formation characterize Regge pole-calculated low-energy electron elastic total cross sections (TCSs) of heavy multi-electron systems. The novelty of the Regge pole analysis is in…

Atomic Physics · Physics 2022-12-29 Alfred Z. Msezane , Zineb Felfli

We calculate the spectra, electric dipole transition rates and isotope shifts of the super heavy elements Ds (Z=110), Rg (Z=111) and Cn (Z=112) and their ions. These calculations were performed using a recently developed, efficient version…

Atomic Physics · Physics 2020-01-29 B. G. C. Lackenby , V. A. Dzuba , V. V. Flambaum

The notion of strong electronic correlations arose in the context of $d$-metal oxides such as NiO but can be exemplified on systems as simple as the H$_2$ molecule. Here we shed light on correlation effects on B$_6^{2-}$ clusters as found…

Strongly Correlated Electrons · Physics 2022-11-11 Thorben Petersen , Ulrich K. Rößler , Liviu Hozoi

Ionic crystals, such as solid electrolytes and complex oxides, are central to modern technologies for energy storage, sensing, actuation, and other functional applications. An important fundamental issue in the atomic and quantum-scale…

Materials Science · Physics 2026-02-12 Shoham Sen , Yang Wang , Timothy Breitzman , Kaushik Dayal