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We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

High fidelity quantum control over qubits is of crucial importance for realistic quantum computing, and it turns to be more challenging when there are inevitable interactions among qubits. By employing a bandselective shaped pulse, we…

Solid-state nuclear spins surrounding individual, optically addressable qubits provide a crucial resource for quantum networks, computation and simulation. While hosts with sparse nuclear spin baths are typically chosen to mitigate qubit…

Quantum Physics · Physics 2022-03-09 Andrei Ruskuc , Chun-Ju Wu , Jake Rochman , Joonhee Choi , Andrei Faraon

The negatively charged nitrogen-vacancy (NV) center in nano- or micro- diamonds has emerged as a promising magnetic field sensor, as a candidate for hyper-polarizing paramagnetic species, as well as a tool for spin-mechanics at the…

Quantum Physics · Physics 2022-04-06 M. Perdriat , P. Huillery , C. Pellet-Mary , G. Hétet

Solid state defects such as nitrogen vacancy (NV) centers in diamond have been utilized for NMR sensing at ambient temperatures for samples at the nano-scale and up to the micro-scale. Similar to standard NMR, NV-sensitivities can be…

Quantum Physics · Physics 2026-01-28 Oliver T. Whaites , Jaime García Oliván , Jorge Casanova

Nitrogen vacancy (NV) centers in diamond exhibit long spin coherence times, optical initialization, and optical spin readout under ambient conditions, making them excellent quantum sensors. However, the conventional scheme for charge state…

Dephasing and relaxation of the nuclear spins coupled to the nitrogen-vacancy (NV) center during optical initialization and readout is an important issue for various applications of this hybrid quantum register. Here we present both an…

Quantum Physics · Physics 2016-07-15 Ping Wang , Wen Yang

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

We propose a protocol that achieves arbitrary N-qubit interactions between nuclear spins and that can measure directly nuclear many-body correlators by appropriately making the nuclear spins interact with a nitrogen vacancy (NV) center…

Quantum Physics · Physics 2017-09-20 J. Casanova , Z. -Y. Wang , M. B. Plenio

We study the coupling of a single nitrogen-vacancy center in diamond to a nearby single nitrogen defect at room temperature. The magnetic dipolar coupling leads to a splitting in the electron spin resonance frequency of the nitrogen-vacancy…

Quantum Physics · Physics 2007-05-23 R. Hanson , F. M. Mendoza , R. J. Epstein , D. D. Awschalom

We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy…

Quantum Physics · Physics 2013-04-01 Ran Fischer , Andrey Jarmola , Pauli Kehayias , Dmitry Budker

Defects in solid state materials provide an ideal, robust platform for quantum sensing. To deliver maximum sensitivity, a large ensemble of non-interacting defects hosting coherent quantum states are required. Control of such an ensemble is…

Optical spin rotations and cycling transitions for measurement are normally incompatible in quantum dots, presenting a fundamental problem for quantum information applications. Here we show that for a hole spin this problem can be addressed…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Samuel G. Carter , Stefan C. Badescu , Allan S. Bracker , Michael K. Yakes , Kha X. Tran , Joel Q. Grim , Daniel Gammon

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in…

Quantum Physics · Physics 2020-04-22 M. L. Goldman , T. L. Patti , D. Levonian , S. F. Yelin , M. D. Lukin

In quantum information science and sensing, electron spins are often purified into a specific polarisation through an optical-spin interface, a process known as optically-detected magnetic resonance (ODMR). Diamond-NV centres and transition…

Chemical Physics · Physics 2024-11-22 Yong Rui Poh , Joel Yuen-Zhou

The controlled assembly of solid-state spins with nanoscale spatial precision is an outstanding challenge for quantum technology. Here, we combine DNA-based patterning with nitrogen-vacancy (NV) ensemble quantum sensors in diamond to form…

Coherent population trapping (CPT) refers to the steady-state trapping of population in a coherent superposition of two ground states which are coupled by coherent optical fields to an intermediate state in a three-level atomic system.…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Xiaodong Xu , Bo Sun , Paul R. Berman , Duncan G. Steel , Allan S. Bracker , Dan Gammon , L. J. Sham

Population Monte Carlo simulations in the form commonly referred to as population annealing can serve as a useful meta-algorithm for simulating systems with complex free-energy landscapes. In the present paper we provide an easily…

Statistical Mechanics · Physics 2024-01-17 P. L. Ebert , D. Gessert , W. Janke , M. Weigel

Levitated macroscopic particles exhibiting quantum mechanical effects are garnering increased attention as a means for precision sensing and testing quantum mechanics. Defects in diamond, such as the nitrogen-vacancy (NV) centre possess…

Quantum Physics · Physics 2026-03-04 A. A. Wood , D. S. Rice , T. Xie , F. H. Cassells , R. M. Goldblatt , T. Delord , G. Hétet , A. M. Martin