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We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

Strongly Correlated Electrons · Physics 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

We introduce THz Stark spectroscopy by using intense single-cycle terahertz pulses as the electric field source and monitoring the induced spectral response of an isotropic molecular ensemble with a coincident femtosecond supercontinuum…

A simple and novel setup for high-frequency dielectric spectroscopy of materials has been developed using a portable vector network analyzer. The measurement principle is based on radio-frequency reflectometry, and both its capabilities and…

Instrumentation and Detectors · Physics 2024-02-02 Aitor Erkoreka , Josu Martinez-Perdiguero

The temperature dependence of ultrafast photoinduced reflectivity transients is reported in Nd$_{0.5}$Sr$_{0.5}$MnO$_{3}$ thin film. The photoinduced reflectivity shows a complex response with very different temperature dependences on…

Condensed Matter · Physics 2009-11-10 T. Mertelj , D. Mihailovic , Z. Jagličič , A. A. Bosak , O. Yu. Gorbenko , A. R. Kaul

We demonstrate resonant detection of rf electric fields from 240 MHz to 900 MHz (very-high-frequency (VHF) to ultra-high-frequency (UHF)) using electromagnetically induced transparency to measure orbital angular momentum $L=3\rightarrow…

This paper is devoted to the theoretical and experimental demonstration of the possibility to perform time-resolved diffusing wave spectroscopy: we successfully registered field fluctuations for selected photon path lengths that can…

Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the…

Optics · Physics 2022-02-10 Tobias Pfeiffer , Jens Klier , Georg von Freymann , Daniel Molter

The serrodyne principle enables shifting the frequency of an electromagnetic signal by applying a linear phase ramp in the time domain [1]. This phenomenon has been exploited to frequency-shift signals in the radiofrequency (RF), microwave…

The successful use of picosecond-pulse free-electron-laser (FEL) radiation for the continuous-wave THz-range electron spin resonance (ESR) spectroscopy has been demonstrated. The combination of two linac-based FELs (covering the wavelength…

Femtosecond coherent multidimensional spectroscopy is demonstrated for an ultracold gas. For this, a setup for phase modulation spectroscopy is used to probe the $3^2\mathrm{S}_{1/2} - 2^2\mathrm{P}_{1/2, 3/2}$ transition in an 800…

Atomic Physics · Physics 2023-01-16 Friedemann Landmesser , Tobias Sixt , Katrin Dulitz , Lukas Bruder , Frank Stienkemeier

Wireless communications in the terahertz band (0.1-10 THz) is a promising and key wireless technology enabling ultra-high data rate communication over multi-gigahertz-wide bandwidths, thus fulfilling the demand for denser networks. The…

Systems and Control · Electrical Eng. & Systems 2024-08-23 Sherif Badran , Arjun Singh , Arpit Jaiswal , Erik Einarsson , Josep M. Jornet

Slow data acquisition in terahertz time-domain spectroscopy (THz-TDS) has hindered the technique's ability to resolve "fast" dynamics occurring on the microsecond timescale. This timescale, arguably too slow to be accessed via standard…

III-V semiconductor mid-infrared photodetectors based on intersubband transitions hold a great potential for ultra-high-speed operation up to several hundreds of GHz. In this work we exploit a ~350nm-thick GaAs/Al0.2Ga0.8As…

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

We developed a phase correction method for broadband terahertz time-domain spectroscopy in reflection geometry, which allows us to obtain quantitative and accurate values for the complex refractive index of materials. The process is…

Transition metal nitrides have recently gained attention in the fields of plasmonics, plasmon-enhanced photocatalysis, photothermal applications, and nonlinear optics because of their suitable optical properties, refractory nature, and…

Ultrafast terahertz spectroscopy accesses the {\em dark} excitonic ground state in resonantly-excited (6,5) SWNTs via internal, direct dipole-allowed transitions between lowest lying dark-bright pair state $\sim$6 meV. An analytical model…

Mesoscale and Nanoscale Physics · Physics 2015-04-09 Liang Luo , Ioannis Chatzakis , Aaron Patz , Jigang Wang

We present a table-top beamline providing a soft X-ray supercontinuum extending up to 350 eV from high-order harmonic generation with sub-13 fs 1300 nm driving pulses and simultaneous production of sub-5 fs pulses centered at 800 nm.…

We report measurements of superradiant optical transition radiation in the 550-800 nm range produced by ultrashort relativistic electron bunches at a dielectric boundary. In the measured optical spectra, we observe photon production with…

We report the first ultrafast pulse radiolysis transient absorption spectroscopy measurements from the Terawatt Ultrafast High Field Facility (TUHFF) at Argonne National Laboratory. TUHFF houses a 20 TW Ti:sapphire laser system that…

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