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Chiral circularly polarized (CP) light is central to many photonic technologies, from optical communication of spin information to novel display and imaging technologies. As such, there has been significant effort in the development of…

Materials Science · Physics 2023-07-25 Li Wan , Yizhou Liu , Matthew J. Fuchter , Binghai Yan

Optical activity is a fundamental phenomenon originating from the chiral nature of crystals and molecules. While intrinsic chiroptical responses of ordinary chiral materials to circularly polarized light are relatively weak, they can be…

Parametric X-ray radiation (PXR) from relativistic electrons moving in a crystal along the crystal-vacuum interface is considered. In this geometry the emission of photons is happening in the regime of extremely asymmetric diffraction…

Accelerator Physics · Physics 2017-09-25 O. D. Skoromnik , V. G. Baryshevsky , A. P. Ulyanenkov , I. D. Feranchuk

The high brightness, broad spectral coverage and pulsed characteristics of infrared synchrotron radiation enable time-resolved spectroscopy under throughput-limited optical systems, as can occur with the high-field magnet cryostat systems…

Materials Science · Physics 2015-06-22 Xiaoxiang Xi , R. J. Smith , T. N. Stanislavchuk , A. A. Sirenko , S. N. Gilbert , J. J. Tu , G. L. Carr

We present a computational investigation, in conjunction with synthesis and experimental characterization, into the structural, electronic, and optical properties of layered 2D organic lead bromide perovskites. We contrast materials based…

Materials Science · Physics 2025-10-29 Md Mehdi Masud , Jarek Viera , Azza Ben-Akacha , Biwu Ma , David A. Strubbe

In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter,…

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

Over the past two decades, metamaterials have led to an increasing number of biosensing and nanophotonic applications due to the possibility of a careful control of light propagating through subwavelength features. Chiral nanostructures…

The orbital angular momentum (OAM) of electron states is an essential ingredient for topological and quantum geometric quantities in solids. For example, Dirac surface states with helical spin- and orbital-angular momenta are a hallmark of…

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

The plasmonic chirality has drawn a lot of attention because of the tunable circular dichroism (CD) and the enhancement for the signal of chiral molecules. Different mechanisms have been proposed for explaining the plasmonic CD, however, a…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Li Hu , Xiaorui Tian , Yingzhou Huang , Xinqiang Wang , Yurui Fang

Resonance Raman experiments on doped and photoexcited single crystals of mixed-halide $MX$ complexes ($M$=Pt; $X$=Cl,Br) clearly indicate charge separation: electron polarons preferentially locate on PtBr segments while hole polarons are…

Condensed Matter · Physics 2009-10-22 L. A. Worl , S. C. Huckett , B. I. Swanson , A. Saxena , A. R. Bishop , J. Tinka Gammel

A light beam can carry both spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is commonly evidenced by circular dichroism (CD) experiments {\em i. e.} differential absorption of left and right-handed circularly polarized…

We employ a homogenization technique based on the Lorentz electronic theory to show that planar chiral structures (PCSs) can be described by an effective dielectric tensor similar to that of biaxial elliptically dichroic crystals. Such a…

Optics · Physics 2009-06-25 S. V. Zhukovsky , A. V. Novitsky , V. M. Galynsky

Convergent beam electron diffraction is routinely applied for studying deformation and local strain in thick crystals by matching the crystal structure to the observed intensity distributions. Recently, it has been demonstrated that CBED…

Mesoscale and Nanoscale Physics · Physics 2020-03-31 Tatiana Latychevskaia , Colin Robert Woods , Yi Bo Wang , Matthew Holwill , Eric Prestat , Sarah J. Haigh , Kostya S. Novoselov

The circular dichroism (ICD) induced from interaction of chiral molecules with achiral plasmonic metal nanostructures has improved sensitivity of molecular chirality detection. Although experimental results have presented several orders…

Photodisintegration of the deuteron above $\pi$ threshold is studied in a coupled channel approach including $N \Delta$ and $\pi d$ channels with consideration of pion retardation in potentials and exchange currents. A much improved…

Nuclear Theory · Physics 2009-11-06 Michael Schwamb , Hartmuth Arenhoevel

The lack of long range order in organic semiconductor thin films prevents the unveiling of the complete nature of excitons in optical experiments, because the diffraction limited beam diameters in the bandgap region far exceed typical…

Irradiation of a molecular system by an intense laser field can trigger dynamics of both electronic and nuclear subsystems. The lighter electrons usually move on much faster, attosecond time scale but the slow nuclear rearrangement damps…

Chemical Physics · Physics 2020-08-26 Nikolay V. Golubev , Tomislav Begušić , Jiří Vaníček

We present theoretical and experimental study of plasmonic Hetero-Chiral structures, comprised of constituents with opposite chirality. We devise, simulate and experimentally demonstrate different schemes featuring selective surface plasmon…

Optics · Physics 2014-06-03 Grisha Spektor , Asaf David , Bergin Gjonaj , Lior Gal , Meir Orenstein
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