Related papers: Linear probing of molecules at micrometric distanc…
The high sensitivity of Laser Spectroscopy has made possible the exploration of atomic resonances in newly designed "nanometric" gas cells, whose local thickness varies from 20nm to more than 1000 nm. Following the initial observation of…
Miniaturizing and integrating atomic vapor cells is widely investigated for the purposes of fundamental measurements and technological applications such as quantum sensing. Extending such platforms to the realm of molecular physics is a…
Selective reflection is a high-resolution spectroscopic method that allows the probing of atomic and molecular gases in the near field of dielectric cell windows. It is a sensitive technique for measuring interactions between excited atoms…
Spectroscopy is a unique experimental tool for measuring the fundamental Casimir-Polder interaction between excited state atoms, or other polarizable quantum objects, and a macroscopic surface. Spectroscopic measurements probe atoms at…
We have carried out theoretical research on ultra-high resolution spectroscopy of atoms (or molecules) in the suggested cell with a series of plane-parallel thin gas layers between spatially separated gas regions of this cell for optical…
We demonstrate a hard x-ray probe of laser-aligned small molecules. To align small molecules with optical lasers, high intensities at nonresonant wavelengths are necessary. We use 95 ps pulses focused to 40 mum from an 800 nm Ti:sapphire…
We show that high-resolution laser spectroscopy can probe surface interactions of gas confined in nano-cavities of porous materials. We report on strong line broadening and unfamiliar lineshapes due to tight confinement, as well as signal…
High-resolution gas phase spectroscopy techniques in the microwave, millimeter-wave and terahertz spectral ranges can be used to study complex organic molecules desorbed from interstellar ice analogues surface with a high sensitivity.…
We describe an instrument which can be used to analyze complex chemical mixtures at high resolution and high sensitivity. Molecules are collisionally cooled with helium gas at cryogenic temperatures (~ 4-7 K), and subsequently detected…
We present scanning near-field extinction spectra of single molecules embedded in a solid matrix. By varying the molecule-tip separation, we modify the line shape of the spectra, demonstrating the coherent nature of the interaction between…
We report on high angular resolution observations of the CO(7-6) line and millimeter continuum in the host galaxy of the gravitationally lensed (z~2.8) quasar RXJ0911.4+0551 using the Plateau de Bure Interferometer. Our CO observations…
Spectra in the CH $^2\Pi_{1/2}$, J=1/2, F=1-1 transition at 3335 MHz were obtained in three 5-point crosses centered on the Galactic plane at $\ell =$ 50$\arcdeg$, 100$\arcdeg$, and 110$\arcdeg$. The lines of sight traverse both Giant…
We demonstrate that a method using the derivative of the selective reflection signal from a nanocell is a convenient and robust tool for atomic laser spectroscopy, achieving a nearly Doppler-free spectral resolution. The recorded linewidth…
Spectroscopic gas sensing is both a commercial success and a rapidly advancing scientific field. Throughout the years, massive efforts have been directed towards improving detection limits by achieving long interaction pathlengths.…
In this habilitation thesis, I briefly present my work at Imperial College London on trapping atomic clouds in micro-pyramids fabricated on silicon chips, which led to the fabrication of an on-chip integrated atom source. Next, I describe…
We measure the resonance line shape of atomic vapor layers with nanoscale thickness confined between two sapphire windows. The measurement is performed by scanning a probe laser through resonance and collecting the scattered light. The line…
The ALMA SPECtroscopic Survey in the {\it Hubble} Ultra Deep Field is an ALMA large program that obtained a frequency scan in the 3\,mm band to detect emission lines from the molecular gas in distant galaxies. We here present our search…
Recent spectroscopic observations by sensitive radio telescopes require accurate molecular spectral line frequencies to identify molecular species in a forest of lines detected. To measure rest frequencies of molecular spectral lines in the…
The redshifted spectral line radiation emitted from both atomic fine-structure and molecular rotational transitions in the interstellar medium (ISM) of high-redshift galaxies can be detected in the centimetre, millimetre and submillimetre…
Ubiquitous to most molecular scattering methods is the challenge to retrieve bond distance and angle from the scattering signals since this requires convergence of pattern matching algorithms or fitting methods. This problem is typically…