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Related papers: Fully {\it ab-initio} electronic structure of Ca$_…

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ComDMFT is a parallel computational package designed to study the electronic structure of correlated quantum materials from first principles. Our approach is based on the combination of first-principles methods and dynamical mean field…

Strongly Correlated Electrons · Physics 2024-11-18 Byungkyun Kang , Patrick Semon , Corey Melnick , Mancheon Han , Seongjun Mo , Hoonkyung Lee , Gabriel Kotliar , Sangkook Choi

The multi-tier $GW$+EDMFT scheme is an ab-initio method for calculating the electronic structure of correlated materials. While the approach is free from ad-hoc parameters, it requires a selection of appropriate energy windows for…

Strongly Correlated Electrons · Physics 2024-08-15 Ruslan Mushkaev , Francesco Petocchi , Viktor Christiansson , Philipp Werner

We perform a systematic {\it ab initio} study of the electronic structure of Sr(V,Mo,Mn)O$_3$ perovskites, using the parameter-free $GW$+EDMFT method. This approach self-consistently calculates effective interaction parameters, taking into…

Strongly Correlated Electrons · Physics 2020-02-26 Francesco Petocchi , Fredrik Nilsson , Ferdi Aryasetiawan , Philipp Werner

We give a detailed description of a recently proposed first principles approach to the electronic structure of strongly correlated materials. The method combines the GW approximation with dynamical mean field theory. It is designed to…

Strongly Correlated Electrons · Physics 2007-05-23 Ferdi Aryasetiawan , Silke Biermann , Antoine Georges

The single-layered perovskite Ca$_2$RuO$_4$, characterized by a 4$d^4$ electron configuration, has been studied from first principles using density functional theory (DFT) using the generalized gradient approximation, with inclusion of…

Strongly Correlated Electrons · Physics 2025-11-26 D. A. Kukusta , L. V. Bekenov , P. F. Perndorfer , D. V. Vyalikh , P. A. Buczek , A. Ernst , V. N. Antonov

Strongly correlated transition-metal perovskite oxides pose a fundamental challenge for electronic-structure theory and for large-scale, data-driven materials discovery. While DFT+DMFT provides a quantitatively accurate description of such…

Strongly Correlated Electrons · Physics 2026-05-19 Antik Sihi , Caden Ginter , Kristjan Haule , Subhasish Mandal

The importance of electronic correlation effects in the layered perovskite Sr$_2$RuO$_4$ is evidenced. To this end we use state-of-the-art LDA+DMFT (Local Density Approximation + Dynamical Mean-Field Theory) in the basis of Wannier…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Pchelkina , I. A. Nekrasov , Th. Pruschke , A. Sekiyama , S. Suga , V. I. Anisimov , D. Vollhardt

First-principles descriptions of correlated quantum materials require a simultaneous treatment of strong local many-body effects and nonlocal dynamical screening. We present an efficient fully self-consistent implementation of $GW$+EDMFT…

Strongly Correlated Electrons · Physics 2026-03-16 Chia-Nan Yeh , Francesco Petocchi , Alexander Hampel , Philipp Werner , Olivier Parcollet , Antoine Georges , Miguel Morales

We discuss a parameter-free and computationally efficient ab initio simulation approach for moderately and strongly correlated materials, the multitier self-consistent $GW$+EDMFT method. This scheme treats different degrees of freedom, such…

Strongly Correlated Electrons · Physics 2017-10-02 Fredrik Nilsson , Lewin Boehnke , Philipp Werner , Ferdi Aryasetiawan

Quantitative prediction of electronic properties in correlated materials requires simulations without empirical truncations and parameters. We present a method to achieve this goal through a new ab initio formulation of dynamical mean-field…

Strongly Correlated Electrons · Physics 2021-04-08 Tianyu Zhu , Garnet Kin-Lic Chan

We present a comparative electronic structure study using DFT and various beyond-DFT (DFT+$U$, $G_0W_0$, DFT+DMFT) methods for ferromagnetic Iron (Fe) to find better approach for describing the spectral properties of correlated magnetic…

Strongly Correlated Electrons · Physics 2021-01-01 Antik Sihi , Sudhir K. Pandey

The outstanding optoelectronics and photovoltaic properties of metal halide perovskites, including high carrier motilities, low carrier recombination rates, and the tunable spectral absorption range are attributed to the unique electronic…

Materials Science · Physics 2020-08-14 Shuxia Tao , Xi Cao , Peter Bobbert

The theoretical understanding of emergent phenomena in quantum materials is one of the greatest challenges in condensed matter physics. In contrast to simple materials such as noble metals and semiconductors, macroscopic properties of…

Strongly Correlated Electrons · Physics 2016-08-30 Sangkook Choi , Andrey Kutepov , Kristjan Haule , Mark van Schilfgaarde , Gabriel Kotliar

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

Recently synthesized quadruple perovskite CuCu$_3$Fe$_2$Re$_2$O$_{12}$ possesses strong ferromagnetism and unusual electron properties, including enhanced electronic specific heat. Application of the first principles electronic structure…

Strongly Correlated Electrons · Physics 2025-02-25 A. I. Poteryaev , Z. V. Pchelkina , S. V. Streltsov , Y. Long , V. Yu. Irkhin

The iso-electronic $d^{4}$ compounds of the $4d$ series show rich phase diagrams due to competing spin, charge and orbital degrees of freedom in presence of strong correlations and structural distortions. One such iso-electronic series,…

Strongly Correlated Electrons · Physics 2018-07-10 Swagata Acharya , Dibyendu Dey , T Maitra , A Taraphder

A new layered perovskite-type oxide Ba$_2$RhO$_4$ was synthesized by a high-pressure technique with the support of convex-hull calculations. The crystal and electronic structure were studied by both experimental and computational tools.…

Strongly Correlated Electrons · Physics 2021-02-03 I. Kurata , José A. Flores-Livas , H. Sugimoto , H. Takahashi , H. Sagayama , Y. Yamasaki , T. Nomoto , R. Arita , S. Ishiwata

Theoretical studies of semiconductors and band insulators are usually based on variants of the $GW$ method without full self-consistency, like single-shot $G^0W^0$ or quasiparticle self-consistent $GW$. Fully self-consistent $GW$ provides a…

Strongly Correlated Electrons · Physics 2024-10-28 Viktor Christiansson , Francesco Petocchi , Philipp Werner

While methods based on density-functional perturbation theory have dramatically improved our understanding of electron-phonon contributions to transport in materials, methods for accurately capturing electron-electron scattering relevant to…

We propose a new mechanism for the paramagnetic metal-insulator transition in the layered perovskite Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ (0<x<0.2). The LDA+U approach including spin-orbit coupling is used to calculate the electronic structures. In…

Strongly Correlated Electrons · Physics 2015-05-28 Guo-Qiang Liu
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