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High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

The Heisenberg-Euler theory of the quantum vacuum supplements Maxwell's theory of electromagnetism with nonlinear light-light interactions. These originate in vacuum fluctuations, a key prediction of quantum theory, and can be triggered by…

Computational Physics · Physics 2023-09-28 Andreas Lindner , Baris Ölmez , Hartmut Ruhl

We investigate the generation of higher-order harmonics from a quantum optics perspective via the interaction of a semiconductor with a coherent pump field focusing on the regime where strong-field intraband excitations dominate. The…

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

Atomic Physics · Physics 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

The optical phase of the driving field in the process of high harmonic generation and the coherence properties of the harmonics are fundamental concepts in attosecond physics. Here, we consider to drive the process by incoherent classical…

Quantum Physics · Physics 2024-09-16 Philipp Stammer

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

We present a quantum optical generalization of the quantum-matter Lewenstein model of high-harmonic generation (HHG) in gases that contains two channels corresponding to the inter- and intraband HHG in solids. Both channels can be presented…

Atomic Physics · Physics 2025-08-21 Adam Thorpe , Neda Boroumand , Graeme Bart , Lu Wang , Giulio Vampa , Thomas Brabec

We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…

Atomic Physics · Physics 2019-10-23 Sebastian Gemsheim , Jan-Michael Rost

High-order harmonic generation in multiphoton ionization regime is studied theoretically to examine the resonant effects of the generating particle. We solve the time-dependent Schr\"odinger equation for In+ in the laser field by expanding…

Atomic Physics · Physics 2023-12-12 Alexander I. Magunov , Vasily V. Strelkov

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

Plasma Physics · Physics 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

The interaction of electrons with strong laser fields is usually treated with semiclassical theory, where the laser is represented by an external field. There are analytic solutions for the free electron wave functions, which incorporate…

Quantum Physics · Physics 2024-07-09 Sándor Varró

We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…