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The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient…

We applied a tabletop, ultrafast, high-harmonic generation (HHG) source to measure the element-specific ferromagnetic resonance (FMR) in ultra-thin magnetic alloys and multilayers on an opaque Si substrate. We demonstrate a continuous wave…

Materials Science · Physics 2024-04-25 Michael Tanksalvala , Anthony Kos , Jacob Wisser , Scott Diddams , Hans T. Nembach , Justin M. Shaw

Self-diffraction is a non-collinear four-wave mixing technique well-known in optics. We explore self-diffraction in the extreme ultraviolet (EUV) range, taking advantage of intense femtosecond EUV pulses produced by a free electron laser.…

The lack of transmissive photonic components in the extreme ultra-violet (XUV) constitutes a challenge for micro/nano-metric confinement. Here, we theoretically design a novel approach to attain XUV radiation guidance based on the…

Optics · Physics 2023-04-07 Luca Assogna , Carino Ferrante , Alessandro Ciattoni , Andrea Marini

A recent breakthrough in laser-plasma accelerators, based upon ultrashort high-intensity lasers, demonstrated the generation of quasi-monoenergetic GeV-electrons. With future Petawatt lasers ultra-high beam currents of ~100 kA in ~10 fs can…

Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…

Atomic Physics · Physics 2020-08-26 Lorenz Drescher , Marc J. J. Vrakking , Jochen Mikosch

Measurements are reported of the cross-correlation of spectra of differential position signals from the Fermilab Holometer, a pair of co-located 39 m long, high power Michelson interferometers with flat, broadband frequency response in the…

We propose a method for a straightforward characterization of the temporal shape of femtosecond pulses in the extreme-ultraviolet/soft X-ray spectral region. The approach is based on the presence of a significant linear frequency chirp in…

Optics · Physics 2015-06-15 David Gauthier , Benoît Mahieu , Giovanni De Ninno

We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…

A far-ultraviolet (FUV) equivalent-wavelength super-resolution interferometric technique is proposed. This FUV equivalent-wavelength interferometric method combines four demodulated phases from four temporal-sets of visible interferograms.…

Optics · Physics 2018-04-04 Manuel Servin , Moises Padilla , Guillermo Garnica

We investigate, by solving the time-dependent Schr\"{o}dinger equation in the single-active-electron approximation in helium, a two-color scheme for tabletop high-order harmonic generation (HHG) that combines a mid-infrared (MIR) driving…

Dynamic scattering and imaging with coherent, ultrafast, extreme ultraviolet (EUV) light sources can resolve charge, phonon and spin processes on their intrinsic length and time scales. However, full field coherent diffraction imaging…

Despite the multitude of available methods, the characterisation of ultrafast pulses remains a challenging endeavour, especially at the single-photon level. We introduce a pulse characterisation scheme that maps the magnitude of its…

Ultra-intense laser-matter interaction experiments (>10$^{18}$ W/cm$^{2}$) with dense targets are highly sensitive to the effect of laser "noise" (in the form of pre-pulses) preceding the main ultra-intense pulse. These system-dependent…

Instrumentation and Detectors · Physics 2015-06-22 S. Feister , J. A. Nees , J. T. Morrison , K. D. Frische , C. Orban , E. A. Chowdhury , W. M. Roquemore

We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition…

X-ray interferometry provides valuable information in terms of attenuation, small-angle scatter, and differential phase contrast. This multi-modal contrast can aid in many clinical applications, such as lung diseases and breast cancer.…

Optics · Physics 2026-03-12 Murtuza S. Taqi , Joyoni Dey , Hunter C. Meyer

We introduce a wide field hyperspectral microscope using the Fourier-transform approach. The interferometer is based on the Translating-Wedge-Based Identical Pulses eNcoding System (TWINS) [Opt. Lett. 37, 3027 (2012)], a common-path…

Instrumentation and Detectors · Physics 2019-09-26 A. Candeo , B. E. Nogueira de Faria , M. Erreni , G. Valentini , A. Bassi , A. M. de Paula , G. Cerullo , C. Manzoni

The ideal laser source for the emerging research field of nonlinear Terahertz (THz) spectroscopy should offer radiation with a large versatility and deliver both ultra-intense multi-octave spanning single-cycle pulses and user-selectable…

Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics…

Transient X-ray absorption techniques can measure ultrafast dynamics of the elemental edges in a material or multiple layer junction, giving them immense potential for deconvoluting concurrent processes. However, the interpretation of the…

Materials Science · Physics 2021-06-10 Hanzhe Liu , Isabel M. Klein , Jonathan M. Michelsen , Scott K. Cushing