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Using a combination of analytical theory, Monte Carlo simulations, and three dimensional self-consistent field calculations, we study the equilibrium properties and the switching behavior of adsorption-active polymer chains included in a…

Soft Condensed Matter · Physics 2017-11-01 Shuanhu Qi , Leonid I. Klushin , Alexander M. Skvortsov , Alexey A. Polotsky , Friederike Schmid

We investigate diffusion-limited reactions between a diffusing particle and a target site on a semiflexible polymer, a key factor determining the kinetics of DNA-protein binding and polymerization of cytoskeletal filaments. Our theory…

Soft Condensed Matter · Physics 2010-12-08 Yann von Hansen , Roland R. Netz , Michael Hinczewski

Non equilibrium coarse grained, dissipative particle dynamics simulations of complex fluids, made up of polymer brushes tethered to planar surfaces immersed in a solvent yield non monotonic behavior of the friction coefficient as a function…

Soft Condensed Matter · Physics 2017-02-01 E. Mayoral , J. Klapp , A. Gama Goicochea

We use the Bond Fluctuation Model (BFM) to study the pore-blockade times of a translocating polymer of length $N$ in two dimensions, in the absence of external forces on the polymer (i.e., unbiased translocation) and hydrodynamic…

Soft Condensed Matter · Physics 2010-01-05 Debabrata Panja , Gerard T. Barkema

A generalized self-consistent field approach for polymer networks with fixed topology is developed. It is shown that the theory reproduces the localization of crosslinks which is characteristic for gels. The theory is then used to study the…

Soft Condensed Matter · Physics 2015-06-17 Friederike Schmid

Modeling ion correlations in inhomogeneous polymers and soft matters with spatially varying ionic strength or dielectric permittivity remains a great challenge. Here, we develop a new theory which systematically incorporates electrostatic…

Soft Condensed Matter · Physics 2024-07-01 Chao Duan , Nikhil R. Agrawal , Rui Wang

We characterize the fluctuation properties of a polymer chain under external tension and the fluctuation-induced forces between two ring molecules threaded around the chain. The problem is relevant in the context of fluctuation-induced…

Soft Condensed Matter · Physics 2016-09-15 F. M. Gilles , R. Llubaroff , C. Pastorino

Using a finite size scaling form for reunion probability, we show numerically the existence of a binding-unbinding transition for Directed polymers with random interaction. The cases studied are (A1) two chains in 1+1 dimensions, (A2) two…

Condensed Matter · Physics 2009-10-28 Sutapa Mukherji , Somendra M. Bhattacharjee , A. Baumgärtner

A polymer network fractures by breaking covalent bonds, but the experimentally measured strength of the polymer network is orders of magnitude lower than the strength of covalent bonds. We investigate the effect of statistical variation of…

Soft Condensed Matter · Physics 2023-04-26 Manyuan Tao , Shawn Lavoie , Zhigang Suo , Maria K. Cameron

Due to their unique structural and mechanical properties, randomly-crosslinked polymer networks play an important role in many different fields, ranging from cellular biology to industrial processes. In order to elucidate how these…

We investigate polyelectrolyte brushes in the osmotic regime using both theoretical analysis and molecular dynamics simulation techniques. In the simulations at moderate Bjerrum length, we observe that the brush height varies weakly with…

Soft Condensed Matter · Physics 2007-05-23 Ali Naji , Roland R. Netz , Christian Seidel

A new network model is proposed to describe the $1/f^\alpha$ resistance noise in disordered materials for a wide range of $\alpha$ values ($0< \alpha < 2$). More precisely, we have considered the resistance fluctuations of a thin resistor…

Materials Science · Physics 2009-11-13 C. Pennetta , E. Alfinito , L. Reggiani

We explore the effect of random permanent cross-links on a system of directed polymers confined between two planes with their end-points free to slide on them. We treat the cross-links as quenched disorder and we use a semimicroscopic…

Soft Condensed Matter · Physics 2010-02-22 Stephan Ulrich , Annette Zippelius , Panayotis Benetatos

The structure of polymer networks, defined by chain lengths and connectivity patterns, fundamentally influences their bulk properties. While existing polymer network models connect chain properties to emergent network behavior, they are…

Soft Condensed Matter · Physics 2026-03-17 Jason Mulderrig , Michael Buche , Matthew Grasinger

We consider two types of fluctuations in the mass-action equilibrium in protein binding networks. The first type is driven by relatively slow changes in total concentrations (copy numbers) of interacting proteins. The second type, to which…

Molecular Networks · Quantitative Biology 2009-11-13 Koon-Kiu Yan , Dylan Walker , Sergei Maslov

We study an anomalous behavior of the height fluctuation width in the crossover from random to coherent growths of surface for a stochastic model. In the model, random numbers are assigned on perimeter sites of surface, representing pinning…

Statistical Mechanics · Physics 2009-10-28 K. Park , B. Kahng

Following the Flory ideality hypothesis intrachain and interchain excluded volume interactions are supposed to compensate each other in dense polymer systems. Multi-chain effects should thus be neglected and polymer conformations may be…

Soft Condensed Matter · Physics 2009-11-13 H. Meyer , J. P. Wittmer , T. Kreer , P. Beckrich , A. Johner , J. Farago , J. Baschnagel

Polymer melts with chains undergoing reversible crosslinking have distinctively favorable dynamic properties, e.g., self healing and reprocessability. In these situations there are two relevant elementary time scales: the segmental and the…

Soft Condensed Matter · Physics 2025-03-14 Rahul Karmakar , Srikanth Sastry , Sanat K. Kumar , Tarak K. Patra

Shear responsive surfaces offer potential advances in a number of applications. Surface functionalisation using polymer brushes is one route to such properties, particularly in the case of entangled polymers. We report on neutron…

The classical bond-fluctuation model (BFM) is an efficient lattice Monte Carlo algorithm for coarse-grained polymer chains where each monomer occupies exclusively a certain number of lattice sites. In this paper we propose a generalization…

Soft Condensed Matter · Physics 2009-08-12 J. P. Wittmer , A. Cavallo , T. Kreer , J. Baschnagel , A. Johner