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The two opposite concepts - multiphoton and effective photon - readily describing the photoelectric effect under strong irradiation in the case that the energy of the incident light is essentially smaller than the ionisation potential of…

Quantum Physics · Physics 2007-05-23 Volodymyr Krasnoholovets

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We present the extension of the time-dependent configuration interaction singles (TDCIS) method to the computation of the electron kinetic-energy spectrum in photoionization processes. Especially for strong and long ionizing light pulses…

Atomic Physics · Physics 2014-04-17 Antonia Karamatskou , Stefan Pabst , Yi-Jen Chen , Robin Santra

In parallel with the evolution of femtosecond and attosecond laser as well as free-electron laser technology, a variety of theoretical methods have been developed to describe the behavior of atoms, molecules, clusters, and solids under the…

Atomic Physics · Physics 2015-11-12 Kenichi L. Ishikawa , Takeshi Sato

The method has been developed to calculate effects of polarization not only for a atomic core in a field of valent electron, but also polarization of atom as a whole in the electron-hole formalism. A secondary quantized density matrix for…

Quantum Physics · Physics 2007-05-23 Halina V. Grushevskaya , Leonid I. Gurskii

The time-dependent surface flux (t-SURFF) method is introduced for computing of strong-field infrared photo-ionization spectra of atoms by numerically solving the time-dependent Schr\"odinger equation on minimal simulation volumes. The…

Computational Physics · Physics 2015-05-30 Liang Tao , Armin Scrinzi

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo

Atomic undercoordination, charge injection, mechanical and thermal activation mediate the properties of a material intrinsically by bond relaxation from one equilibrium to another while the phonon spectrometrics probes the ever-unexpected…

Materials Science · Physics 2020-01-08 Chang Q Sun

Amino acids are essential to all life. However, our understanding of some aspects of their intrinsic structure, molecular chemistry, and electronic structure is still limited. In particular the nature of amino acids in their crystalline…

Materials Science · Physics 2020-11-02 Anna Regoutz , Marta S. Wolinska , Nathalie K. Fernando , Laura E. Ratcliff

We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

Advantages of introducing the electron structure function (ESF) in electron induced processes are demonstrated. Contrary to the photon structure function it is directly measured in such processes. At present energies a simultaneous analysis…

High Energy Physics - Phenomenology · Physics 2009-01-07 W. Slominski , J. Szwed

Multi-electron screening effects encountered in laboratory astrophysical reactions are investigated by considering the reactants Thomas-Fermi atoms. By means of that model, previous studies are extended to derive the corresponding screening…

Nuclear Theory · Physics 2009-11-06 Theodore E. Liolios

Isotopic substitution in molecular systems can affect fundamental molecular properties including the energy position and spacing of electronic, vibrational and rotational levels, thus modifying the dynamics associated to their coherent…

We show that interference phenomena plays a big role for the electron yield in ionization of atoms by an ultra-short laser pulse. Our theoretical study of single ionization of atoms driven by few-cycles pulses extends the photoelectron…

Quantum Physics · Physics 2009-11-13 Diego Arbo , Emil Persson , Joachim Burgdoerfer

We investigate the kinetic-energy spectrum of electrons emitted from an excited many-electron system, often called photo-electron spectrum (PES). We are particularly interested on the impact of resonant modes of the system on PES. To this…

Atomic and Molecular Clusters · Physics 2015-06-23 P. M. Dinh , P. -G. Reinhard , E. Suraud , P. Wopperer

Frequency-filtered photon correlations have been proven to be extremely useful in grasping how the detection process alters photon statistics. Harnessing the spectral correlations also permits refinement of the emission and unraveling of…

The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Shaul Mukamel , Rafal Oszwaldowski , Lijun Yang

A review is given on the recent spectroscopic studies of the electronic excitation induced processes of large-scale atomic displacements in atomic cryocrystals, including defect formation, atomic and molecular desorption.

Condensed Matter · Physics 2007-05-23 A. N. Ogurtsov

Production of electron-positron pairs from vacuum in strong bichromatic electric fields, oscillating in time with a fundamental frequency and its second harmonic, is studied. Strong-field processes occuring in such field configurations are…

Atomic Physics · Physics 2020-04-15 J. Braß , R. Milbradt , S. Villalba-Chávez , G. G. Paulus , C. Müller