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Understanding the reactivity and spectroscopy of aqueous solutions at the atomistic level is crucial for the elucidation and design of chemical processes. However, the simulation of these systems requires addressing the formidable…

Chemical Physics · Physics 2017-02-28 Ondrej Marsalek , Thomas E. Markland

Partially ionized plasma physics has attracted a lot of attention recently due to numerous technological applications made possible by the increased sophistication of computer modelling, the depth of the theoretical analysis, and the…

Plasma Physics · Physics 2026-01-06 Igor Kaganovich , Michael Tendler

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

Electron microscopy based on high-energy electrons allows nanoscopic analytical imaging taking advantage of secondarily generated particles. Especially for cathodoluminescence, the correlation between primary incident electrons and emitted…

Instrumentation and Detectors · Physics 2025-01-28 Sotatsu Yanagimoto , Naoki Yamamoto , Tatsuro Yuge , Hikaru Saito , Keiichirou Akiba , Takumi Sannomiya

Multiphoton interference is an essential phenomenon at the very heart not only of fundamental quantum optics and applications in quantum information processing and sensing but also of demonstrations of quantum computational supremacy in…

Quantum Physics · Physics 2023-12-25 Vincenzo Tamma , Simon Laibacher

Photons strongly coupled to material systems constitute a novel system for studying the dynamics of non-equilibrium quantum many-body systems. We give a fully analytical description of the dynamics of photons coupled to a one-dimensional…

Quantum Physics · Physics 2023-01-04 Björn Schrinski , Anders S. Sørensen

First-principles calculations combining density functional theory and many-body perturbation theory can provide microscopic insight into the dynamics of electrons and phonons in materials. We review this theoretical and computational…

Materials Science · Physics 2016-11-23 Marco Bernardi

We study the statistics of multi-photon absorption/emission processes in a mesoscopic ring threaded by an harmonic time-dependent flux $\Phi(t)$. For this sake, we demonstrate a useful analogy between the Keldysh quantum kinetic equation…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Alessandro Silva , Vladimir E. Kravtsov

The description of excited state dynamics in multichromophoric systems constitutes both a theoretical and experimental challenge in modern physical chemistry. An experimental protocol which can systematically characterize both coherent and…

Quantum Physics · Physics 2011-10-31 Joel Yuen-Zhou , Jacob J. Krich , Masoud Mohseni , Alán Aspuru-Guzik

We introduce a novel computational approach for the investigation of complex correlated electron materials which makes it possible to evaluate interatomic forces and thereby determine atomic displacements and structural transformations…

Strongly Correlated Electrons · Physics 2014-04-24 I. Leonov , V. I. Anisimov , D. Vollhardt

We develop a detailed theoretical model of photo-induced proton-coupled electron transfer (PPCET) processes, which are at the basis of solar energy harvesting in biological systems and photovoltaic materials. Our model enables to analyze…

Chemical Physics · Physics 2021-04-13 Jiaji Zhang , Raffaele Borrelli , Yoshitaka Tanimura

We describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state…

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

Recent results on particle momentum and spin correlations are discussed in view of the role played by the effects of quantum statistics, including multiboson and coherence phenomena, and final state interaction. Particularly, it is…

Nuclear Theory · Physics 2009-11-10 R. Lednicky

Reradiation of a spatially non-uniform ultrashort electromagnetic pulse interacting with the linear chain of multielectron atoms is studied in the framework of sudden perturbation approximation. Angular distributions of the reradiation…

Atomic Physics · Physics 2018-10-16 V. I. Matveev , D. U. Matrasulov

Laser induced plasmas have found numerous applications including plasma-assisted combustion, combustion diagnostics, laser induced breakdown spectroscopy, light detection and ranging techniques (LIDAR), microwave guiding, reconfigurable…

Plasma Physics · Physics 2017-10-11 A. Sharma , M. N. Slipchenko , M. N. Shneider , X. Wang , K. A. Rahman , A. Shashurin

Formulas to describe the photoabsorption and the photon scattering by a plasma or a liquid metal are derived in a unified manner with each other. It is shown how the nuclear motion, the free-electron motion and the core-electron behaviour…

Materials Science · Physics 2009-10-31 Junzo Chihara

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

In addition to its importance in describing high-energy processes themselves, the dynamics of multiparticle production is part of the general field of non-linear phenomena and complex systems. Multiparticle dynamics is one of the rare…

High Energy Physics - Phenomenology · Physics 2007-05-23 W. Kittel

Photon number distributions from classical and non-classical light sources have been studied extensively, yet their impact on photoemission processes is largely unexplored. In this article, we present measurements of electron…

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