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We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be…

To time-resolve attosecond electronic dynamics in general photoionization processes, the technique that retrieves the phase of emitted electronic wave packets without intercepting the interactions is essential. Here, we theoretically…

Atomic Physics · Physics 2026-04-27 Kunlong Liu , Yidian Tian , Pengcheng Li

Shake-up is a fundamental phenomenon in photoionisation of many-electron systems whereby the ionisation of one electron is accompanied by the simultaneous excitation of another. As a single-photon two-electron excitation, it is the most…

We study high-order harmonic generation (HHG) driven by seeded plasmonic-enhanced fields. On one hand, plasmonic-enhanced fields have shown a great potential to extend the HHG cutoff, an instrumental pre-requisite for the generation of…

Atomic Physics · Physics 2018-12-12 Irfana N. Ansari , M. S. Mrudul , Marcelo F. Ciappina , Maciej Lewenstein , Gopal Dixit

Coherent control over electron dynamics in atoms and molecules using high-intensity circularly-polarized laser pulses gives rise to current loops, resulting in the emission of magnetic fields. We propose and demonstrate with ab-initio…

We review the main research directions ongoing in the development of high-harmonic generation-based extreme ultraviolet sources for the synthesization and application of trains and isolated attosecond pulses to time-resolved spectroscopy. A…

We propose a method for programmable shaping of the amplitude and phase of the XUV and x-ray attosecond pulses produced by high-order harmonic generation. It overcomes the bandwidth limitations of existing spectral filters and enables…

Optics · Physics 2015-06-17 Dane R. Austin , Jens Biegert

Attosecond science has demonstrated that electrons can be controlled on the sub-cycle time scale of an optical wave, paving the way toward optical frequency electronics. Using controlled few-cycle optical waveforms, the study of sub-cycle…

Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. We perform the first temporal…

Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

Ultrafast strong-field laser--plasma physics is shown to offer a promising framework for relativistic nonlinear quantum electrodynamics (QED). As one of its key advantages, this approach to relativistic nonlinear QED does not require an…

Plasma Physics · Physics 2026-04-23 Vedin Dewan , Aleksei M. Zheltikov , Julia M. Mikhailova

Attosecond streaking is one of the most fundamental processes in attosecond science allowing for a mapping of temporal (i.e. phase) information on the energy domain. We show that on the single-particle level attosecond streaking time shifts…

Coherent light beams composed of ultrashort pulses are now increasingly used in different fields of Science, from time-resolved spectroscopy to plasma physics. Under the effect of even simple optical components, the spatial properties of…

Optics · Physics 2013-05-30 H. Vincenti , F. Quéré

Solids exposed to intense electric fields release electrons through tunnelling. This fundamental quantum process lies at the heart of various applications, ranging from high brightness electron sources in DC operation to petahertz vacuum…

The bottleneck for an attosecond science experiment is concluded to be the lack of a high-peak-power isolated attosecond pulse source. Therefore, currently, generating an intense attosecond pulse would be one of the highest priority goals.…

Attosecond pulses produced by High-order Harmonic Generation (HHG) in gases driven by intense laser fields have become a cornerstone technique for probing ultrafast electronic motion in matter. These applications require a good knowledge of…

The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…

Chemical Physics · Physics 2017-02-08 W. A. Bryan , C. R. Calvert , R. B. King , J. B. Greenwood , W. R. Newell , I. D. Williams